Abstract
Carbon dioxide and methane emissions are major greenhouse gases contributing to global warming, thus calling for rapid techniques of sequestration. For instance, dry reforming of methane transforms CO2 and CH4 into syngas, a mixture of H2 and CO, yet the reaction catalyst becomes inactivated by carbon formation and metal sintering. Here, we review catalytic systems used for dry reforming of methane. Improved catalysts of high catalytic performance and stability are obtained by selecting the active metal, supporting materials, promoters and preparation techniques. We found a strong correlation between the support morphology, physicochemical properties and catalytic performances. In particular, fibrous structures show optimal metal–support interaction, distribution, particle size, basicity, storage of oxygen space, surface area and porosity, resulting in high performance of anti-coking and anti-sintering.
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copyright 2020 Elsevier
copyright 2020 Elsevier
copyright 2020 Elsevier
copyright 2020 Elsevier (Abdulrasheed et al. 2020)
copyright 2019 Elsevier
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Abbreviations
- CCUS:
-
Capture of carbon, use and storage
- MCM-41:
-
Mobil Composition of Matter No. 41 mesoporous via a hierarchical structure
- SBA-15:
-
Santa Barbara amorphous-type material mesoporous silica sieve based on uniform hexagonal pores
- TEOS:
-
Tetraethyl orthosilicate
- EISA:
-
Evaporation-induced self-assembly process
- KCC-1:
-
Fibrous silica
- Ni/KCC-1(IP):
-
Nickel on nitridated fibrous silica by one-pot hydrothermal technique
- Ni/KCC-1(IM):
-
Nickel on nitridated fibrous silica by wet impregnation method
- HZSM-5:
-
Aluminosilicate zeolite
- FmZSM-5:
-
Fibrous silica mesoporous ZSM-5
- DFSBA-15:
-
Dendritic fibrous SBA-15
- HSi@ZSM-5:
-
Mesostructured fibrous silica@ZSM-5
- RWGS:
-
Reverse water–gas shift reaction
- FESEM:
-
Field emission scanning electron microscope
- FTIR:
-
Fourier transform infrared
- TPD-CO2 :
-
Temperature-programmed desorption of carbon dioxide
- TPD-NH3 :
-
Temperature-programmed desorption of ammonia
- CTAB:
-
Cetyltrimethyl ammonium bromide
- EFAl:
-
Extra-framework aluminum species in zeolite
- CARiACT Q:
-
Principally formulated silica with average pores 3 and 50 nm Q-50 and Q-3
- NiCe/NFA:
-
Nickel-supported cerium nanofibers
- NiCe/NGA:
-
Nickel-supported cerium nanograins
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This work was supported by the financial support of Universiti Teknologi Malaysia through Transdisciplinary Research Grant (Grant Nos. 06G52 and 06G53).
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Owgi, A.H.K., Jalil, A.A., Hussain, I. et al. Catalytic systems for enhanced carbon dioxide reforming of methane: a review. Environ Chem Lett 19, 2157–2183 (2021). https://doi.org/10.1007/s10311-020-01164-w
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DOI: https://doi.org/10.1007/s10311-020-01164-w