Skip to main content

Advertisement

Log in

Innovative device to assay leachate production in non-sanitary landfills

  • ORIGINAL ARTICLE
  • Published:
Journal of Material Cycles and Waste Management Aims and scope Submit manuscript

Abstract

Improper landfills (waste dumps) are common waste disposal systems in developing countries and represent sources of environmental pollution. These sites defy researchers and managers because they lack structures to collect liquid, solid and gaseous samples, which make it challenging to monitor local environmental quality. In this work, we show one device for sample collection to monitor leachate quality in a closed waste dump in Brazil. During the installation of this device (Leachate Monitoring Station, LMS), interesting facts about the structural, physical, and chemical composition of an old dump could be visualized. Two different kinds of leachate were found: the accumulated leachate (AL), a thick dark fluid entrapped above non-degraded material, and the mobile leachate (ML), a lighter liquid which flowed into the LMS, and thus was not stagnant like AL. In the AL, the chemical oxygen demand and total ammoniacal nitrogen average concentrations were about 21,500 mg/L and 1000 mg/L, respectively, which were considerably higher than the ML concentrations, of about 1100 mg/L and 200 mg/L, respectively, for the same parameters. Thus, despite the lower concentrations of hazardous substances in the ML, the waste body stores pockets of leachate (AL) with significant concentrations of hazardous compounds, even after 15 years of the dumpsite closure. Moreover, waste solubilization assays showed that the solid material could not be considered inert according to the Brazilian Standard Norm NBR 10004/2004. The installation of the LMS enabled a new understanding about pollutant accumulation inside waste deposits and provided an effective, low-cost tool to monitor leachate production in non-sanitary landfills. The results warn about the risks that old dumpsites still pose to the environment and reinforce the need for a post-care action plan for managing uncontrolled waste deposits.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1

Source: Modified from [60]

Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6

Similar content being viewed by others

Notes

  1. https://www.atlas.d-waste.com/

References

  1. Blight GE (1996) (1996) Report: standards for landfills in developing countries. Waste Manag Res 14(4):399–408. https://doi.org/10.1177/0734242X9601400407

    Article  Google Scholar 

  2. Johannessen LM, Boyer G (1999) Observations of solid waste landfills in developing countries: Africa, Asia and Latin America—Urban Waste Management Thematic Group. Waste Management Anchor Team. 1st edn. The World Bank, Washington, DC. https://documents.worldbank.org/curated/en/393531468741627673/pdf/multi-page.pdf. Accessed 7 Aug 2020

  3. Singh RK, Datta M, Nema AK (2009) A new system for groundwater contamination hazard rating of landfills. J Environ Manage 91(2009):344–357. https://doi.org/10.1016/j.jenvman.2009.09.003

    Article  Google Scholar 

  4. Bidone FRA, Povinelli J (2010) Basics of solid waste, 2nd edn. University of São Paulo, São Carlos (in Portuguese)

    Google Scholar 

  5. Aharoni I, Siebner H, Dahan O (2017) Application of vadose-zone monitoring system for real-time characterization of leachate percolation in and under a municipal landfill. Waste Manag 67(2017):203–213. https://doi.org/10.1016/j.wasman.2017.05.012(ISSN 0956-053X)

    Article  Google Scholar 

  6. ABRELPE (2017) Overview of solid waste in Brazil in 2016. Organized by the Brazilian Association of Public Cleaning and Special Waste Companies (ABRELPE) (in Portuguese). São Paulo, Brazil. https://abrelpe.org.br/panorama/. Accessed 7 Aug 2020

  7. Brazil (2010) Brazilian federal law nº 12305: national policy on solid waste. Brasília, Brazil. https://www.planalto.gov.br/ccivil_03/_ato2007-2010/2010/lei/l12305.htm. Accessed 7 Aug 2020

  8. Zolnikov TR, Silva RC, Tuesta AA, Marques CP, Cruvinel VRN (2018) Ineffective waste site closures in Brazil: a systematic review on continuing health conditions and occupational hazards of waste collectors. Waste Manag 80:26–39. https://doi.org/10.1016/j.wasman.2018.08.047

    Article  Google Scholar 

  9. Cetrulo TB, Marques RC, Cetrulo NM, Silva F, Moreira RM, Cortés DM, Malheiros TF (2018) Effectiveness of solid waste policies in developing countries: a case study in Brazil. J Clean Prod 205:179–187. https://doi.org/10.1016/j.jclepro.2018.09.094

    Article  Google Scholar 

  10. Government of Brazil (2017) Government of Brazil Audit Report of the Union's Office of the General Comptroller: current stage of implementation of the Brazilian Solid Waste Policy. https://auditoria.cgu.gov.br/download/9805.pdf. Accessed 23 Mar 2019

  11. Farquhar GJ, Rovers FA (1973) Gas production during refuse decomposition. Water Air Soil Pollut 2(4):483–495. https://doi.org/10.1007/BF00585092(ISSN 1573-2932)

    Article  Google Scholar 

  12. Shen S, Chen Y, Zhan L, Xie H, Bouazza A, He F, Zuo X (2018) Methane hotspot localization and visualization at a large-scale Xi'an landfill in China: effective tool for landfill gas management. J Environ Manage 225:232–241. https://doi.org/10.1016/j.jenvman.2018.08.012

    Article  Google Scholar 

  13. Valencia RG, Rodriguez FM, Cristóbal J, Thalasso F (2016) Hotspot detection and spatial distribution of methane emissions from landfills by a surface probe method. Waste Manag 55:299–305. https://doi.org/10.1016/j.wasman.2016.03.004

    Article  Google Scholar 

  14. Christensen TH, Kjeldsen P, Bjerg PL, Jensen DL, Christensen JB, Baun A, Albrechtsen H-J, Heron G (2001) Biogeochemistry of landfill leachate plumes: review. Appl Geochem 16(7–8):659–718. https://doi.org/10.1016/S0883-2927(00)00082-2

    Article  Google Scholar 

  15. Szczepańska J, Twardowska I (2004) Principles of vadose and saturated zones monitoring in solid waste sites exemplified in mining waste dumps. In: Irena Wardowska HEAAAFK, William JL (eds) Waste management series, vol 4. Elsevier, Amsterdam, pp 551–575

    Google Scholar 

  16. Mookiah M, Thiagarajan S, Ganesan Dr (2012) Detection of groundwater contamination by solid waste leachate using electrical resistivity method and geochemical analysis. In: Groundwater modeling and management under uncertainty. CRC Press. p 307–312. https://www.routledge.com/Groundwater-Modeling-and-Management-under-Uncertainty-Proceedings-of-the/Hadi-Copty/p/book/9781138000124. Accessed 7 Aug 2020

  17. Fetter CW, Boving T, Kreamer D (2018) Contaminant hydrogeology, 3rd edn. Waveland Press, Illinois

    Google Scholar 

  18. Gautam A, Pathak G, Sahni A (2011) Assessment of ground water quality at municipal solid waste dumping site-Sewapura, Jaipur. Curr World Environ 6:279–282. https://doi.org/10.12944/CWE.6.2.12

    Article  Google Scholar 

  19. WHO—World Health Organization. Progress on sanitation and drinking water—2015 update and Millennium Development Goals (MDG) assessment. ISBN 978 92 4 150914 5. https://data.unicef.org/wp-content/uploads/2015/12/Progress-on-Sanitation-and-Drinking-Water_234.pdf. Accessed 7 Aug 2020

  20. Mavakala BK, Le Faucheur S, Mulaji CK, Laffite A, Devarajan N, Biey EM, Giuliani G, Otamonga JP, Kabatusuila P, Mpiana PT, Poté J (2016) Leachates draining from controlled municipal solid waste landfill: detailed geochemical characterization and toxicity tests. Waste Manag 55:238–248. https://doi.org/10.1016/j.wasman.2016.04.028(ISSN 0956-053X)

    Article  Google Scholar 

  21. Belevi H, Baccini P (1989) Long-term behavior of municipal solid waste landfills. Waste Manag Res 7:43–56

    Article  Google Scholar 

  22. Rees JF (1980) The fate of carbon compounds in the landfill disposal of organic matter. J Chem Technol Biotechnol 30(1980):161–175. https://doi.org/10.1002/jctb.503300121

    Article  Google Scholar 

  23. Ehrig HJ (1983) Quality and quantity of sanitary landfill leachate. Waste Manag Res 1:53–68 (ISBN: 9780323144865)

    Article  Google Scholar 

  24. McBean EA, Rovers FA, Farquhar GJB (1995) Solid waste landfill engineering and design. Prentice Hall, Englewood Cliffs

    Google Scholar 

  25. Souto GDAB, Povinelli J (2011) Tables of typical characteristics of the leachate from landfills in Brazil: acidic and methanogenic phases. In: Congresso Brasileiro de Engenharia Sanitária e Ambiental (Brazilian Conference), p 26

  26. Moody CM, Townsend TG (2017) A comparison of landfill leachates based on waste composition. Waste Manag 63:267–274. https://doi.org/10.1016/j.wasman.2016.09.020

    Article  Google Scholar 

  27. Oloibiri V, Chys M, De Wandel S, Demeestere K, Van Hulle SWH (2017) Removal of organic matter and ammonium from landfill leachate through different scenarios: operational cost evaluation in a full-scale case study of a Flemish landfill. J Environ Manag 203:774–781. https://doi.org/10.1016/j.jenvman.2016.09.055

    Article  Google Scholar 

  28. Dia O, Drogui P, Buelna G, Dubé R (2018) Hybrid process, electrocoagulation-biofiltration for landfill leachate treatment. Waste Manag 75:391–399. https://doi.org/10.1016/j.wasman.2018.02.016

    Article  Google Scholar 

  29. Poblete R, Oller I, Maldonado MI, Cortes E (2019) Improved landfill leachate quality using ozone, UV solar radiation, hydrogen peroxide, persulfate and adsorption processes. J Environ Manag 232:45–51. https://doi.org/10.1016/j.jenvman.2018.11.030

    Article  Google Scholar 

  30. Hozle I (2019) Contaminant patterns in soils from landfill mining. Waste Manag 83:151–160. https://doi.org/10.1016/j.wasman.2018.11.013

    Article  Google Scholar 

  31. Bjerg PL, Albrechtsen H-J, Kjeldsen P, Christensen TH, Cozzarelli I (2013) The groundwater geochemistry of waste disposal facilities. In: Holland HD, Turekian KK (eds) Environmental geochemistry: treatise on geochemistry. Elsevier Science, Amsterdam

    Google Scholar 

  32. Lopes AA (2007) Study of the integrated management of urban solid waste at the Tietê-Jacaré Basin-UGRHI-13 (in Portuguese). Doctoral Thesis—University of São Paulo, São Carlos, Brazil

  33. Velozo R (2006) Geological-geotechnical characterization of a deactivated dump in São Carlos—SP, with the aid of geophysics (in Portuguese). Masters Dissertation—University of São Paulo, São Carlos, Brazil

  34. PMSC (2011) Detailed environmental assessment—Evaluation of risk to human health. (Report in Portuguese). São Carlos municipal council and GEOAMBIENTE Consulting (ID: GEOSP09022), Curitiba, Brazil

  35. Freitas ALS (1996) Characterization of the Botucatu Aquifer in the São Carlos dump region—SP (in Portuguese). Masters Dissertation—University of São Paulo, São Carlos, Brazil

  36. Gadotti RF (1997) Assessment of contamination of surface water and groundwater adjacent to the São Carlos waste dump (in Portuguese). Masters Dissertation—University of São Paulo, São Carlos, Brazil

  37. Wendland E, Barreto C, Gomes LH (2007) Water balance in the Guarani Aquifer outcrop zone based on hydrogeologic monitoring. J Hydrol 342(2007):261–269. https://doi.org/10.1016/j.jhydrol.2007.05.033

    Article  Google Scholar 

  38. CETESB (2017) Contaminated areas list from São Paulo State, Brazil (in Portuguese). https://cetesb.sp.gov.br/areas-contaminadas/wp-content/uploads/sites/17/2018/01/Munic%C3%ADpios.pdf. Accessed 7 Aug 2020

  39. Bertolo RA (2001) Hydrodynamics and hydrogeochemistry of the unsaturated zone of the Adamantine Aquifer in Urania (in Portuguese). Doctoral Thesis—University of São Paulo, São Paulo, Brazil. https://teses.usp.br/teses/disponiveis/44/44133/tde-20012014-174523/pt-br.php. Accessed 7 Aug 2020

  40. Varnier CL (2007) Evaluation of contamination of a deactivated cesspool in the unsaturated zone of the Adamantina aquifer in Urânia—SP (in Portuguese). Doctoral Thesis—University of São Paulo, São Paulo, Brazil

  41. ISO/IEC 17025 (2005) Brazilian standard norms: ISO/IEC 17025—Laboratory accreditation (in Portuguese)—CETESB—São Paulo, Brazil

  42. APHA (2005). Standard Methods for Examination of Water and Wastewater. In: Prepared and published jointly by American Public Health Association (APHA), American Water Works Association (AWWA) and Water Environment Federation Publication (WEFP), 21th edn, Washington, USA

  43. ABNT (2004a) Brazilian standard norms NBR 10006: procedure for obtaining solubilized solid waste extract (in Portuguese). Rio de Janeiro, Brazil

  44. ABNT (1989) Brazilian standard norms NBR 10644: water—determination of residues (solids)—gravimetric method (in Portuguese). Rio de Janeiro, Brazil

  45. Addinsoft (2019) XLSTAT statistical and data analysis solution. Boston, USA. https://www.xlstat.com. Accessed 7 Aug 2020

  46. Ehrig HJ (1989) “Leachate quality” in sanitary landfilling: process, technology, and environmental impact. In: Christensen TH, Cossu R, Stegman R (eds) Sanitary landfilling: process, technology and environmental impact. Academic Press, New York

    Google Scholar 

  47. Masoner JR, Kolpin DW, Furlong ET, Cozzarelli IM, Gray JL, Schwab EA (2014) Contaminants of emerging concern in fresh leachate from landfills in the conterminous United States. Environ Sci Process Impacts 16(10):2335–2354

    Article  Google Scholar 

  48. Abreu AES (2015) Geophysical investigation and shear strength of municipal solid waste with different ages (in Portuguese). Doctoral Thesis—University of São Paulo, São Carlos, Brazil.

  49. Gomes LP (1989) Study of physical characterization and biodegradability of municipal solid waste in landfills (in Portuguese). Masters Dissertation, University of São Paulo, São Carlos, Brazil

  50. Gazoty A, Findaca G, Pedernsen J, Auken E, Christiansen AV, Pedersen JK (2012) Application of time domain induced polarization to the mapping of lithotypes in a landfill site. Hydrol Earth Syst Sci 16(2012):1793–1804. https://doi.org/10.5194/hess-16-1793-2012

    Article  Google Scholar 

  51. Qasim SR, Chiang W (1994) Sanitary landfill leachate: generation, control and treatment. CRC Press, Boca Raton

    Google Scholar 

  52. Kjeldsen P, Barlaz MA, Rooker AP, Baun A, Ledin A, Christensen TH (2002) Present and long-term composition of MSW landfill leachate: a review. Critical Rev Environ Sci Technol 32(4):297–336. https://doi.org/10.1080/10643380290813462

    Article  Google Scholar 

  53. Mehta R, Barlaz MA, Yasdani R, Augentein D, Bryars M, Sinderson L (2002) Refuse decomposition in the presence and absence of leachate recirculation. J Environ Eng 128(3):2002. https://doi.org/10.1061/(ASCE)0733-9372(2002)128:3(228)

    Article  Google Scholar 

  54. ABNT (2004) Brazilian standard Norm NBR 10.004: classification of solid waste (in Portuguese). Rio de Janeiro, Brazil

  55. Pauli AR, Espizona-Quiñones FR, Trigueros DEG, Módenes AN, Souza ARC, Borba FH, Kroumov AD (2018) Integrated two-phase purification procedure for abatement of pollutants from sanitary landfill leachates. Chem Eng J 334(2018):19–29. https://doi.org/10.1016/j.cej.2017.10.028(ISSN 1385-8947)

    Article  Google Scholar 

  56. Eighmy TT, Crannell BS, Krzanowski JE, Butler LG, Cartledge FK, Emery EF, Eusden JD Jr, Shawe EL, Francis CA (1998) Characterization and phosphate stabilization of dusts from the vitrification of MSW combustion residues. Waste Manag 18(1998):513–524. https://doi.org/10.1016/S0956-053X(98)00139-1

    Article  Google Scholar 

  57. Pohland FG, Harper SR (1985) Critical review and summary of leachate and gas production from landfills. Cincinnati, USEPA, Office of Research and Development. EPA/600/2-86/073. https://nepis.epa.gov/Exe/ZyPDF.cgi/20007KHC.PDF?Dockey=20007KHC.PDF

  58. Brazil (2011) CONAMA Resolution nº430 of May 13th, 2011: regulates effluent discharge standards (in Portuguese). Ministry of Environment (MMA), Brasília, Brazil. https://www.mma.gov.br/port/conama/res/res11/res43011.pdf. Accessed 7 Aug 2020

  59. Farquhar GJ (1989) Leachate: production and characterization. Can J Civ Eng 16(3):317–325. https://doi.org/10.1139/l89-057

    Article  Google Scholar 

  60. Shinzato MPB (2014) Mobilization of pollutants in waste mass of an uncontrolled landfill (in Portuguese). Doctoral Thesis–University of São Paulo, São Carlos, Brazil. https://www.teses.usp.br/teses/disponiveis/18/18138/tde-27012015-085018/pt-br.php. Accessed 7 Aug 2020

  61. El-Fadel M, Bou-Zeid E, Chahine W, Alayli B (2002) Temporal variation of leachate quality from pre-sorted and baled MSW with high organic and moisture content. Waste Manag 22(2002):269–282. https://doi.org/10.1016/S0956-053X(01)00040-X

    Article  Google Scholar 

  62. EPA—U.S. Environmental Protection Agency (2011) Closure and Post-Closure Care Requirements for Municipal Solid Waste Landfills (MSWLFs). https://www.epa.gov/osw/nonhaz/municipal/landfill/financial/mswclose.html. Accessed 7 Aug 2020

Download references

Acknowledgements

This research was supported by the National Council for Scientific and Technological Development (CNPq), Funding Authority for Studies and Projects (FINEP) and by the São Paulo Research Foundation (FAPESP—no 2011/08105-0 and no 2015/03806-1). We wish to express our gratitude to all and the Centre for Natural Resources and Development (CNRD-Germany).

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Natalia de Souza Pelinson.

Ethics declarations

Conflict of interest

The authors declare no conflict of interest.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Electronic supplementary material

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

de Souza Pelinson, N., Shinzato, M.P.B., Morita, A.K.M. et al. Innovative device to assay leachate production in non-sanitary landfills. J Mater Cycles Waste Manag 22, 1985–1998 (2020). https://doi.org/10.1007/s10163-020-01084-5

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10163-020-01084-5

Keywords

Navigation