Abstract
Lab synthesized metal-bearing sludge (LSMS) was used in series of designed lab tests to evaluate impacts of ultrasound on selective separation of heavy metals through acid leaching. The tests eliminated the potential of induced bias generated by utilizing field sludge that were produced from different location sources. The results showed that metal pairs of Cu and Fe, Cu and Cr, and Cr and Fe inside LSMS could be practically separated with one metal being contained in a liquid phase and another in a solid phase through acid leaching processes enhanced by ultrasound. With assistance of ultrasound, the acid leaching demonstrated a more efficient segregation between metals within LSMS than a conventional leaching that doesn’t have ultrasonic enhancement, and the tests provided in a generic means that ultrasonically enhanced acid leaching could cost-efficiently recover heavy metals from metal-containing waste sludge.
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Patent-pending technique.
References
Merian E, Anke M, Ihnat M, Stoeppler M (2004) Elements and their compounds in the environment. Metals and their compounds, vol 2. Wiley-VCH, Weinheim, pp 478–1247
Zouboulis AI, Loukidou MX, Matis KA (2004) Biosorption of toxic metals from aqueous solutions by bacteria strains isolated from metal-polluted soils. Process Biochem 39:909–916
Yu T, Zhang Y, Hu X, Meng W (2012) Distribution and bioaccumulation of heavy metals in aquatic organisms of different trophic levels and potential health risk assessment from Taihu lake, China. Ecotoxicol Environ Saf 81(1):55–64
Silva JE, Paiva AP, Soares D, Labrincha A, Castro F (2005) Solvent extraction applied to the recovery of heavy metals from galvanic sludge. J Hazard Mater 120(1–3):113–118
Silva PTS, Mello NT, Duarte MMM, Montenegro MCBSM, Araújo AN, Neto BB, Silva VL (2006) Extraction and recovery of chromium from electroplating sludge. J Hazard Mater 128(1):39–43
Atanassova A, Dukov IL (2006) Solvent extraction and separation of lanthanoids with mixtures of chelating extractant and 1-(2-pyridylazo)-2-naphthol. Sep Purif Technol 49:101–105
Vegliò F, Quaresima R, Fornari P, Ubaldini S (2003) Recovery of valuable metals from electronic and galvanic industrial wastes by leaching and electrowinning. Waste Manag 23(3):245–252
De Villiers PGR, Van Deventer JSJ, Lorenzen L (1995) The extraction of species from slurries of insoluble solids with ion-exchange resins. Miner Eng 8:1309–1316
Parkpian P, Leong ST, Laortanakul P, Poonpolwatanaporn P (2002) Environmental applicability of chitosan and zeolite for amending sewage sludge. J Environ Sci Health A 37:1855–1870
Chaudry MA, Ahmad S, Malik MT (1997) Supported liquid membrane technique applicability for removal of chromium from tannery wastes. Waste Manag 17(4):211–218
Li J, Lu HZ, Guo J, Xu ZM, Zhou YH (2007) Recycle technology for recovering resources and products from waste printed circuit boards. Environ Sci Technol 41:1995–2000
Wu J, Li J, Xu ZM (2008) Electrostatic separation for recovering metals and nonmetals from waste printed circuit board: problems and improvements. Environ Sci Technol 42:5272–5276
Ryu HW, Moon HS, Lee EY, Cho KS, Choi H (2003) Leaching characteristics of heavy metals from sewage sludge by Acidithiobacillus thiooxidans MET. J Environ Qual 32:751–759
Shanableh A, Omar M (2003) Bio-acidification and leaching of metals, nitrogen, and phosphorus from soil and sludge mixtures. Soil Sediment Contam 12:565–589
Hoquea ME, Philip OJ (2011) Biotechnological recovery of heavy metals from secondary sources—an overview. Mater Sci Eng C Mater 31(2):57–66
Rossini G, Bernardes AM (2006) Galvanic sludge metals recovery by pyrometallurgical and hydrometallurgical treatment. J Hazard Mater 131(1–3):210–216
Dimitrijević M, Kostov A, Tasić V, Milosević N (2009) Influence of pyrometallurgical copper production on the environment. J Hazard Mater 164(2–3):892–899
Demetrio S, Ahumada J, Angel M, Mast E, Jojas U, Sanhueza J, Reyes P, Morales E (2000) Slag cleaning: the Chilean copper smelter experience. JOM 52(8):20–25
Davenport WG, King M, Schlesinger M, Biswas AK (2002) Extractive metallurgy of copper, 4th edn. Pergamon, Oxford, pp 289–305
Jergensen GV (1999) Copper leaching, solvent extraction, and electrowinning technology. Society for Mining Metallurgy and Exploration, Littleton
Norgate TE, Jahanshahi S, Rankin WJ (2007) Assessing the environmental impact of metal production processes. J Clean Prod 15(8–9):838–848
Hsiao MC, Wang HP, Huang CH, Chang JE, Wei YL (2007) Tracking of copper in contaminated soils. J Electron Spectrosc 156–158:208–210
Ziqi H, Surasak S, Richard TS, Samuel JT, Linda KW (2011) Removal of mercury from sediment by ultrasound combined with biomass (transgenic Chlamydomonas reinhardtii). Chemosphere 83(9):1249–1254
Chiha M, Hamdaoui O, Ahmedchekkat F, Pétrier C (2010) Study on ultrasonically assisted emulsification and recovery of copper(II) from wastewater using an emulsion liquid membrane process. Ultrason Sonochem 17:318–325
Samuel LR, Emmanuel N, Patrick D, Guy M, Jean-François B (2012) Low frequency ultrasound-assisted leaching of sewage sludge for toxic metal removal, dewatering and fertilizing properties preservation. Ultrason Sonochem. doi:10.1016/j.ultsonch.2012.08.001
Xie FC, Li HY, Ma Y, Li CC, Cai TT, Huang ZY, Yuan GQ (2009) The ultrasonically assisted metals recovery treatment of printed circuit board waste sludge by leaching separation. J Hazard Mater 170:430–435
Li CC, Xie FC, Ma Y, Li HY, Cai TT, Huang ZY, Yuan GQ (2010) Multiple heavy metals extraction and recovery from hazardous electroplating sludge waste via ultrasonically enhanced two-stage acid leaching. J Hazard Mater 178:823–833
Xie FC, Cai TT, Ma Y, Li HY, Li CC, Huang ZY, Yuan GQ (2009) Recovery of Cu and Fe from printed circuit board waste sludge by ultrasound: evaluation of industrial application. J Clean Prod 17:1494–1498
Jandová J, tefanová T, Niemczyková R (2000) Recovery of Cu-concentrates from waste galvanic copper sludges. Hydrometallurgy 57(1):77–84
Whillock G, Harvey B (1997) Ultrasonically enhanced corrosion of 304L stainless steel I: the effect of temperature and hydrostatic pressure. Ultrason Sonochem 4:23–31
Suslick KS, Price GJ (1999) Applications of ultrasound to materials chemistry. Annu Rev Mater Sci 29:295–326
Konno A, Kato H, Yamaguchi H, Maeda M (2002) On the collapsing behavior of cavitation bubble clusters. Jpn Soc Mech Eng Int J Ser B Fluids Therm Eng 45(3):631–637
Grénman H, Murzina E, Rönnholm M, Eränen K, Mikkola JP, Lahtinen M, Salmi T, Murzi YD (2007) Enhancement of solid dissolution by ultrasound. Chem Eng Process 46(9):862–869
Kim J, Kaurich TA, Sylvester P, Martin AG (2006) Enhanced selective leaching of chromium from radioactive sludges. Sep Sci Technol 41:179–196
Sridhar P, Puspendu B, Song Y, Blanc RJ, Tyagi RD, Surampalli RY (2011) Ultrasonic pretreatment of sludge: a review. Ultrason Sonochem 18(1):1–18
Godinez JAB, O’Keefe TJ, Watson JL (1992) Effect of ultrasound on acidified brine leaching of double-kiln treated EAF dust. Miner Eng 5:1365–1373
Acknowledgments
The authors are thankful to the Nature Science Foundation of China (20777020), the Enterprise-College-Institute Cooperative Project Foundation of Guangdong Province and Ministry of Education of China (2007B090400037), and the Science and Technology Planning Project Foundation of Guangzhou City (2008Z1-E481) for supporting this work.
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Zhang, P., Ma, Y. & Xie, F. Impacts of ultrasound on selective leaching recovery of heavy metals from metal-containing waste sludge. J Mater Cycles Waste Manag 15, 530–538 (2013). https://doi.org/10.1007/s10163-013-0131-z
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DOI: https://doi.org/10.1007/s10163-013-0131-z