Skip to main content
Log in

Local atomic structure of ultra-thin Fe films grown on Cu(100)

  • Published:
Applied Physics A Aims and scope Submit manuscript

Abstract

Ultra-thin epitaxial Fe films grown by thermal deposition on Cu(100) are analyzed by scanning tunneling microscopy. Evidence is presented that the morphological characteristics and magnetic properties are a direct consequence of FCC-to-BCC transitions reminiscent of those occurring in bulk Fe. In contrast to the assumption of a ferromagnetic FCC phase in previous models of the Fe/Cu(100) system, we observe a tightly twinned and strained BCC-like phase termed nanomartensite in films below 5 ML thickness, which encompasses almost the entire film volume of 3 ML films. In addition, the surface of 7–8 ML films reconstructs by forming non-close-packed structures with BCC-like bond angles. The formation of these BCC-like phases is the reason for the expansion of the interlayer spacing observed in these films and correlates perfectly with their ferromagnetic ordering.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. F. Bitter, A.R. Kaufman: Phys. Rev. 56, 1044 (1939)

    Article  ADS  Google Scholar 

  2. C.S. Smith: Phys. Rev. 57, 337 (1940)

    Article  ADS  Google Scholar 

  3. S.C. Abrahams, L. Guttman, J.S. Kasper: Phys. Rev. 127, 2052 (1962)

    Article  ADS  Google Scholar 

  4. U. Gonser, C.J. Meecham, A.H. Muir, H. Wiedersich: J. Appl. Phys. 34, 2373 (1963)

    Article  ADS  Google Scholar 

  5. U. Gradmann, W. Kummerle, P. Tillmanns: Thin Solid Films 34, 249 (1976)

    Article  ADS  Google Scholar 

  6. M.T. Kief, W.F. Egelhoff: Phys. Rev. B 47, 10785 (1993)

    Article  ADS  Google Scholar 

  7. W.A. Jesser, J.W. Matthews: Philos. Mag. 17, 595 (1968)

    Article  ADS  Google Scholar 

  8. W. Keune, R. Halbauer, U. Gonser, J. Lauer, D.L. Williamson: J. Appl. Phys. 48, 2976 (1977)

    Article  ADS  Google Scholar 

  9. W. Becker, H.D. Pfannes, W. Keune: J. Magn. Magn. Mater. 35, 53 (1983)

    Article  ADS  Google Scholar 

  10. J. Thomassen, F. May, B. Feldmann, M. Wuttig, H. Ibach: Phys. Rev. Lett. 69, 3831 (1992)

    Article  ADS  Google Scholar 

  11. D. Pescia, M. Stampanoni, G.L. Bona, A. Vaterlaus, R.F. Willis, F. Meier: Phys. Rev. Lett. 58, 2126 (1987)

    Article  ADS  Google Scholar 

  12. A. Clarke, P.J. Rous, M. Arnott, G. Jennings, R.F. Willis: Surf. Sci. 192, L843 (1987)

  13. S. Müller, P. Bayer, A. Kinne, P. Schmailzl, K. Heinz: Surf. Sci. 322, 21 (1995)

    Article  ADS  Google Scholar 

  14. S. Müller, P. Bayer, C. Reischl, K. Heinz, B. Feldmann, H. Zillgen, M. Wuttig: Phys. Rev. Lett. 74, 765 (1995)

    Article  ADS  Google Scholar 

  15. K. Heinz, S. Müller, P. Bayer: Surf. Sci. 352354, 942 (1996)

    Google Scholar 

  16. R.J. Weiss: Proc. Phys. Soc. 82, 281 (1963)

    Article  ADS  Google Scholar 

  17. M.F. Onellion, C.L. Fu, M.A. Thompson, J.L. Erskine, A.J. Freeman: Phys. Rev. B 33, 7322 (1986)

    Article  ADS  Google Scholar 

  18. V.L. Moruzzi, P.M. Marcus, K. Schwarz, P. Mohn: Phys. Rev. B 34, 1784 (1986)

    Article  ADS  Google Scholar 

  19. V.L. Moruzzi, P.M. Marcus, J. Kübler: Phys. Rev. B 39, 6957 (1989)

    Article  ADS  Google Scholar 

  20. W. Daum, C. Stuhlmann, H. Ibach: Phys. Rev. Lett. 60, 2741 (1988)

    Article  ADS  Google Scholar 

  21. C. Egawa, E.M. McCash, R.F. Willis: Surf. Sci. 215, L271 (1989)

  22. K. Heinz, S. Müller, P. Bayer: Surf. Sci. 337, 215 (1995)

    Article  ADS  Google Scholar 

  23. D. Li, M. Freitag, J. Pearson, Z.Q. Qiu, S.D. Bader: Phys. Rev. Lett. 72, 3112 (1994)

    Article  ADS  Google Scholar 

  24. M. Wuttig, B. Feldmann, J. Thomassen, F. May, H. Zillgen, A. Brodde, H. Hannemann, H. Neddermeyer: Surf. Sci. 291, 14 (1993)

    Article  ADS  Google Scholar 

  25. H. Zillgen, B. Feldmann, M. Wuttig: Surf. Sci. 321, 32 (1994)

    Article  ADS  Google Scholar 

  26. T. Detzel, M. Vonbank, M. Donath, N. Memmel, V. Dose: J. Magn. Magn. Mater. 152, 287 (1996)

    Article  ADS  Google Scholar 

  27. A. Biedermann, M. Schmid, P. Varga: Phys. Rev. Lett. 86, 464 (2001)

    Article  ADS  Google Scholar 

  28. A. Biedermann, R. Tscheliessnig, M. Schmid, P. Varga: Phys. Rev. Lett. 87, 086103 (2001)

    Article  ADS  Google Scholar 

  29. A. Biedermann, R. Tscheliessnig, C. Klein, M. Schmid, P. Varga: submitted to Surf. Sci.

  30. D. Qian, X.F. Jin, J. Barthel, M. Klaua, J. Kirschner: Phys. Rev. Lett. 87, 227204 (2001)

    Article  ADS  Google Scholar 

  31. J. Giergiel, J. Shen, J. Woltersdorf, A. Kirilyuk, J. Kirschner: Phys. Rev. B 52, 8528 (1995)

    Article  ADS  Google Scholar 

  32. K. Kalki, D.D. Chambliss, K.E. Johnson, R.J. Wilson, S. Chiang: Phys. Rev. B 48, 18344 (1993)

    Article  ADS  Google Scholar 

  33. W. Pitsch: Philos. Mag. 4, 577 (1959)

    Article  ADS  Google Scholar 

  34. H. Landskron, G. Schmidt, K. Heinz, K. Müller, C. Stuhlmann, U. Beckers, M. Wuttig, H. Ibach: Surf. Sci. 256, 115 (1991)

    Article  ADS  Google Scholar 

  35. M. Zharnikov, A. Dittschar, W. Kuch, C.M. Schneider, J. Kirschner: J. Magn. Magn. Mater. 174, 40 (1997)

    Article  ADS  Google Scholar 

  36. P.J. Cumpson, M.P. Seah: Surf. Interface Anal. 25, 430 (1997)

    Article  Google Scholar 

  37. V. Blum, K. Heinz: Comput. Phys. Commun. 134, 392 (2001)

    Article  ADS  Google Scholar 

  38. A. Brodde, H. Neddermeyer: Surf. Sci. 287288, 988 (1993)

  39. D.D. Chambliss, K.E. Johnson: Phys. Rev. B 50, 5012 (1994)

    Article  ADS  Google Scholar 

  40. T. Detzel, N. Memmel, T. Fauster: Surf. Sci. 293, 227 (1993)

    Article  ADS  Google Scholar 

  41. T. Detzel, N. Memmel: Phys. Rev. B 49, 5599 (1994)

    Article  ADS  Google Scholar 

  42. F. Dulot, B. Kierren, D. Malterre: Surf. Sci. 494, 229 (2001)

    Article  ADS  Google Scholar 

  43. W.A. Hofer, J. Redinger, A. Biedermann, P. Varga: Surf. Sci. 466, L795 (2000)

  44. D. Qian, X. Jin, J. Barthel, M. Klaua, J. Kirschner: Phys. Rev. B 66, 172406 (2002)

    Article  ADS  Google Scholar 

  45. D. Spišák, J. Hafner: Phys. Rev. Lett. 88, 056101 (2002)

    Article  ADS  Google Scholar 

  46. A.G. Every, A.K. McCurdy: in High and Low Frequency Properties of Dielectric Crystals, Vol. III/29a of Landolt-Börnstein Condensed Matter, ed. by D. Nelson (Springer, Berlin 1992) p. 635

  47. G.L. Krasko, G.B. Olson: Phys. Rev. B 40, 11536 (1989)

    Article  ADS  Google Scholar 

  48. H. Hasegawa, D.G. Pettifor: Phys. Rev. Lett. 50, 130 (1983)

    Article  ADS  Google Scholar 

  49. M. Aldén, S. Mirbt, H.L. Skriver, N.M. Rosengaard, B. Johansson: Phys. Rev. B 46, 6303 (1992)

    Article  ADS  Google Scholar 

  50. T. Shinjo, W. Keune: J. Magn. Magn. Mater. 200, 598 (1999)

    Article  ADS  Google Scholar 

  51. R.H. Madjoe, A.N. Koveshnikov, C. Harwell, R. Hall, R.L. Stockbauer, R.L. Kurtz: J. Appl. Phys. 85, 6211 (1999)

    Article  ADS  Google Scholar 

  52. J.V. Barth, D.E. Fowler: Phys. Rev. B 52, 11432 (1995)

    Article  ADS  Google Scholar 

  53. K. Heinz, S. Müller: private communication

  54. D. Spišák, J. Hafner: Phys. Rev. B 61, 16129 (2000)

    Article  ADS  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to P. Varga.

Additional information

PACS

68.55.-a; 64.70.-p; 81.30.-t

Rights and permissions

Reprints and permissions

About this article

Cite this article

Biedermann, A., Tscheliessnig, R., Schmid, M. et al. Local atomic structure of ultra-thin Fe films grown on Cu(100). Appl. Phys. A 78, 807–816 (2004). https://doi.org/10.1007/s00339-003-2435-7

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s00339-003-2435-7

Keywords

Navigation