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Vertical profile of polycyclic aromatic hydrocarbons in a sediment core from a reservoir in Osaka City

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Environmental Geology

Abstract

Concentrations of polycyclic aromatic hydrocarbons (PAHs) were measured in a dated sediment core from a reservoir at Osaka City, Southwest Japan. The sediment core consisted of deposits collected over a period of almost 70 years whose PAH content would serve as a historical record of atmospheric environment at Osaka City. Total PAH concentrations varied from 4.2 to 26 mg kg−1 dry wt, and peaked in the 1940s, reflecting the occurrence of a large fire due to air attacks during World War II. The results indicated that warfare had the largest impact on atmospheric environment in Osaka City. Total PAH concentrations decreased in the post-war period except for a small peak. In the 1950s, there was a downward trend from the 1970s to the present. These trends can be ascribed to the growth of industrial activities and the regulation of atmospheric pollutant emissions, respectively.

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References

  • Baumard P, Budzonski H, Garrigues P (1998) Polycyclic aromatic hydrocarbons in sediments and mussels of the western Mediterranean Sea. Environ Toxicol Chem 17:765–776

    Article  Google Scholar 

  • Blokzijl PJ, Guicherit R (1972) The occurrence of polynuclear aromatic hydrocarbons (PAH) in outdoor air. TNO-news 1972, Nov 653–660

  • Boström CE, Gerde P, Hanberg A, Jernström B, Johansson C, Kyrklund T, Rannug A, Törnqvist M, Victorin K, Westerholm R (2000) Cancer risk assessment, indicators, and guidelines for polycyclic aromatic hydrocarbons in the ambient air. Environ Health Perspect 110:451–488

    Google Scholar 

  • Gschwend PM, Hites RA (1981) Fluxes of polycyclic aromatic hydrocarbons to marine and lacustrine sediments in the northeastern United States. Geochim Cosmochim Acta 45:2359–2367

    Article  Google Scholar 

  • Hirose K, Aoyama M, Katsuragi Y, Sugiyama Y (1987) Annual deposition of Sr-90, Cs-137 and Pu-239, 240 from the 1961–1980 Nuclear Explosions: a Simple Model. J Meteorol Soc Jpn 65:259–277

    Google Scholar 

  • Katahira K, Ishitake M, Moriwaki H, Yoshikawa S, Yamamoto O, Fujita T, Yamazaki H (2006) Method for the estimation of the past illegal dumping recorded in a sediment core. Water Air Soil Pollut (in press)

  • Kawaraya T (1998) Trend and dustribution of polycyclic aromatic hydrocarbon in Osaka from 1967 to 1994. Seikatsu Eisei 42:229–232

    Google Scholar 

  • Kumata H, Sanada Y, Takada H, Ueno T (2000) Historical trends of N-cyclohexyl-2-benzothiazolamine, 2-(4-morpholinyl)benzothiazole, and other anthropogenic contaminants in the urban reservoir sediment core. Environ Sci Technol 34:246–253

    Article  Google Scholar 

  • Mastral AM, Callen MS (2000) Review on polycyclic aromatic hydrocarbon (PAH) emissions from energy generation. Environ Sci Technol 34:3051–3057

    Article  Google Scholar 

  • Moriwaki H, Ishitake M, Yoshikawa S, Miyakoda H, Alary JF (2004) Determination of polycyclic aromatic hydrocarbons in sediment by liquid chromatography-atmospheric pressure photo ionization-mass spectrometry. Anal Sci 20:375–377

    Article  Google Scholar 

  • Moriwaki H, Katahira K, Yamamoto O, Fukuyama J, Kamiura T, Yamazaki H, Yoshikawa S (2005) Historical trends of polycyclic aromatic hydrocarbons in the reservoir sediment core at Osaka. Atmos Environ 39:1019–1025

    Article  Google Scholar 

  • Murakami A, Inoue J (2004) History of fossil fuel combustion during the last 100 years in and around Osaka City, Japan: changes of the spheroidal carbonaceous particles (SCPs) recorded in a moat and in pond sediments. Quaternary Res 43:265–274

    Article  Google Scholar 

  • Okuda K, Nakada N, Isobe T, Nishiyama H, Sanada Y, Sato F, Takada H (2000) Endocrine disruptors in a sediment core collected from Tokyo Bay—the historical trends during the past 50 years. Bull Coast Oceanogr 37:15–24

    Google Scholar 

  • Osaka City (1994) Shinshu-Osakashishi 7, 1068, 33p

  • Peirson DH (1971) Worldwide deposition of long-lived fission products from nuclear explosions. Nature 234:79

    Google Scholar 

  • Sicre MA, Marty JC, Saliot A, Aparicio X, Grimalt J, Albaiges J (1987) Aliphatic and aromatic hydrocarbons in different sized aerosols over the Mediterranean Sea: occurrence and origin. Atmos Environ 21:2247–2259

    Article  Google Scholar 

  • The Institute of Energy Economics, Japan (1997) EDMC/energy and economy statistical report, 304p

  • Tsuji I, Koide K, Moriyama H, Tanabe K, Matsusita H (1985) Analysis of polynuclear aromatic hydrocarbons in shellfishes, seabottom sediments and sea water by high performance liquid chromatography. J Food Hyg Soc Jpn 26:50–55

    Google Scholar 

  • Yunker MB, Snowdon LR, Macdonald RW, Smith JN, Fowler MG, Skibo DN, McLaughlin FA, Danyushevskaya AI, Petrova VI, Ivanov GI (1996) Polycyclic aromatic hydrocarbon composition and potential sources for sediment samples from the Beaufort and Barents Seas. Environ Sci Technol 30:1310–1320

    Article  Google Scholar 

  • Yunker MB, Macdonald RW, Vingarzan R, Mitchell RH, Goyette D, Sylvestre S (2002) PAHs in the Fraser River basin: a critical appraisal of PAH ratios as indicators of PAH source and composition. Org Geochem 33:489–515

    Article  Google Scholar 

Download references

Acknowledgments

The authors are grateful to Dr. Mitamura of Osaka City University for his invaluable comments and advice. Thanks to the staff of the laboratory of natural history of anthropogene at Osaka City University for their advice.

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Correspondence to Miho Ishitake.

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Ishitake, M., Moriwaki, H., Katahira, K. et al. Vertical profile of polycyclic aromatic hydrocarbons in a sediment core from a reservoir in Osaka City. Environ Geol 52, 123–129 (2007). https://doi.org/10.1007/s00254-006-0465-0

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  • DOI: https://doi.org/10.1007/s00254-006-0465-0

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