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Observation of antiferromagnetic spin-flop transition in λ-type BETS salts using AFM microcantilever

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Abstract

Antiferromagnetic spin-flop transitions in a series of λ-(BETS)2FeBrxCl4-x are observed using piezoresistive AFM microcantilever. The measurements are carried out on a tiny single crystal using a sample rotator and the easy axis changes with increasing the bromine content x. The Néel temperature and spin-flop transition field also rise with increasing the bromine content x, suggesting an enhancement of π-d interactions by replacement of chlorine with bromine atoms in this mixed-halide anion system.

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Tanaka, H., Hara, S., Tokumoto, M. et al. Observation of antiferromagnetic spin-flop transition in λ-type BETS salts using AFM microcantilever. J Low Temp Phys 142, 605–608 (2006). https://doi.org/10.1007/BF02679580

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