Abstract
The practical applicability of the 1/E1+α epithermal spectrum representation and of the effective resonance energy\(\bar E_r\) in NAA is investigated. Attention is paid to fundamental considerations such as definitions and approximations, error propagation functions, uncertainty statements, reliability of nuclear data and formal dimensioning problems. As to the latter, it is concluded that the applicability of the\(\bar E_r\)-concept is not dependent on the choice of a reference energy. The usefulness of the parameters α and\(\bar E_r\) in NAA is demonstrated by new experimental evidence obtained from α and Q0 determinations in three different reactors: the WWR-M reactor (Budapest, Hungary), the THETIS reactor (Gent, Belgium) and the DR-3 reactor (Risø, Denmark).
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A. SIMONITS, F. DE CORTE, J. HOSTE, J. Radioanal. Chem., 24 (1975) 31.
O. T. HØGDAHL, Neutron Absorption in Pile Neutron Activation Analysis, Rept. MMPP-226-1, Dec. 1962; Proc. Symp. Radiochemical Methods of Analysis, Salzburg, October 19–23, 1964, IAEA Vienna, 1965 p. 23.
L. MOENS, F. DE CORTE, A. DE WISPELAERE, J. HOSTE, A. SIMONITS, A. ELEK, E. SZABÓ, J. Radioanal. Nucl. Chem., 82 (1984) 385.
J. OP DE BEECK, J. Radioanal. Nucl. Chem., 89 (1985) 169.
W. L. ZIJP, E. M. ZSOLNAY, H. J. NOLTHENIUS, E. J. SZONDI, G. C. H. M. VERHAAG, D. E. CULLEN, C. ERTEK, Final Report on the REAL-80 Exercise, Rept. ECN-128, Febr. 1983.
E. M. ZSOLNAY, W. L. ZIJP, H. J. NOLTHENIUS, Effect of Normalization on the Neutron Spectrum Adjustment Procedure, Rept. ECN-139, Oct. 1983.
C. B. BIGHAM, R. M. PEARCE, The Slowing-Down Spectrum in Heterogeneous Reactors, Rept. AECL-1228, 1961.
M. M. R. WILLIAMS, The Slowing-Down and Thermalization of Neutrons, North-Holland, Amsterdam, 1966.
T. B. RYVES, E. B. PAUL, J. Nucl. Energy, 22 (1968) 759.
T. B. RYVES, Metrologia, 5 (1969) 119.
A. AHMAD, Ph. D. Thesis, Univ. of London, 1982.
L. MOENS, F. DE CORTE, A. SIMONITS, A. DE WISPELAERE, J. HOSTE, J. Radioanal. Chem., 52 (1979) 379.
S. JOVANOVIĆ, F. DE CORTE, L. MOENS, A. SIMONITS, J. HOSTE, J. Radioanal. Nucl. Chem., 82 (1984) 379.
S. F. MUGHABGHAB, D. I. GARBER, Neutron Cross Sections, Vol. 1, Resonance Parameters, BNL 325, 3rd ed., 1973.
S. JOVANOVIĆ, The Effective Resonance Energy as a New Parameter in (n,γ) Analysis with Reactor Neutrons, Ph.D. Thesis, Univ. Gent, (1984).
S. F. MUGHABGHAB, M. DIVADEENAM, N. E. HOLDEN, Neutron Cross Sections, Vol. 1, Neutron Resonance Parameters and Thermal Cross Sections, Part A: Z=1–60, Academic Press, New York, 1981.
S. F. MUGHABGHAB, Neutron Cross Sections, Vol. 1, Neutron Resonance Parameters and Thermal Cross Sections, Part B: Z=61–100, Academic Press, New York, 1984.
F. DE CORTE, S. SORDO-EL HAMMAMI, L. MOENS, A. SIMONITS, A. DE WISPELAERE, J. HOSTE, J. Radioanal. Chem., 62 (1981) 209.
F. DE CORTE, S. JOVANOVIĆ, A. SIMONITS, L. MOENS, J. HOSTE, Kernenergie-Kerntechnik, Suppl. to Vol. 44 (1984) 641.
R. KAARLS (Rapporteur), Report of the BIPM Working Group on the Statement of Uncertainties (1st meeting: 21–23 Oct. 1980) to the Comité International des Poids et Mesures.
J. W. MÜLLER, Precision Measurements and Fundamental Constants II, B. N. TAYLOR, W. D. PHILLIPS (Eds), Natl. Bureau of Standards, U.S., Spec. Publ. 617, 1984 p. 375.
J. W. MÜLLER, The Treatment of Measurement Uncertainties, Interregional Training Course on Ensuring Measurement Accuracy, Austrian Research Center, Seibersdorf, 1984.
L. MOENS, F. DE CORTE, A. SIMONITS, J. HOSTE, Proc. 5th Intern. Conf. on Nuclear Methods in Environmental and Energy Research, Mayaguez, Puerto Rico, Apr. 1984, J. R. VOGT, (Ed.), (CONF-840408), p. 525.
J. I. KIM, E. M. GRYNTAKIS, H. J. BORN, Radiochim. Acta, 22 (1975) 20.
F. DE CORTE, L. MOENS, A. SIMONITS, J. HOSTE, J. Radioanal. Nucl. Chem., 92 (1985) 183.
F. W. WALKER, D. G. MILLER, Dr. F. FEINER, Chart of the Nuclides, 13th ed., General Electric Company, San Jose, USA, 1984.
W. MAENHAUT, F. ADAMS, J. HOSTE, J. Radioanal. Chem., 16 (1973) 39.
R. E. HEFT, Proc. Conf. on Computers in Activation Analysis and Gamma-Ray Spectroscopy, Mayaguez, Puerto Rico, Apr. 1979, J. R. VOGT (Ed.) (CONF-780421), p. 1.
P. NIKOLOW, S. NIESE, Isotopenpraxis, 1 (1980) 31.
B. E. WATT, Phys. Rev., 87 (1952) 1037.
L. CRANBERG, G. FRYE, N. NERESON, L. ROSEN, Phys. Rev., 103 (1956) 662.
R. B. LEACHMAN, Determinations des grandeurs de fission importantes pour les piles, Actes de la Conférence Internationale sur l'Utilisation de l'Energie Atomique à des Fins Pacifiques, Vol. 2, Nations Unies, Genève, 1956, p. 223.
J. OP DE BEECK, J. Radioanal. Nucl. Chem., 90 (1985) 167.
A. SIMONITS, F. DE CORTE, L. MOENS, J. HOSTE, J. Radioanal. Chem., 72 (1982) 209.
F. DE CORTE, L. MOENS, A. SIMONITS, A. DE WISPELAERE, J. HOSTE, J. Radioanal. Chem., 52 (1979) 295.
F. DE CORTE, L. MOENS, K. SORDO-EL HAMMAMI, A. SIMONITS, J. HOSTE, J. Radioanal. Chem., 52 (1979) 305.
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De Corte, F., Moens, L., Jovanović, S. et al. Applicability of the 1/E1+α epithermal spectrum representation and the effective resonance energy\(\bar E_r\) in NAA. Journal of Radioanalytical and Nuclear Chemistry, Articles 102, 37–57 (1986). https://doi.org/10.1007/BF02037948
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DOI: https://doi.org/10.1007/BF02037948