Abstract
The experimental and theoretical situations for direct single ionization by electron impact are reviewed with special emphasis on triple differential cross sections for impact energies between several hundred eV and threshold. These cross sections can now be determined in absolute units, thus providing a powerful test of calculations. Only the target atoms helium and atomic hydrogen are considered, with quite simple wave functions, in order to focus attention on the correct description of the collision mechanism and to investigate the ranges of validity of various theoretical models. For the higher incident energies, processes with asymmetric energy partitioning and small momentum transfer are emphasized. For a long time these processes (which represent the predominant majority of all ionizing collisions) could not be calculated satisfactorily. Substantial progress in the theoretical treatment of the problem now allows the reproduction of the correct intensities and peak positions in the angular correlations of the outgoing electrons. It is now clear that double collisions, at least, have to be taken into account to describe the dynamics of these collisions. At lower energies both escaping electrons move rather slowly in the field of the ion core and exchange effects can no longer be neglected. Therefore, the theoretical situation is still rather involved. Close to threshold, recent triple differential cross section measurements permit a partial wave analysis, which should challenge theorists to explain these data by ab-initio calculations. The last chapter of this report deals with the progress in the determination of reliable absolute double differential cross sections.
Similar content being viewed by others
References
Tate, J.T., Smith, P.T.: Phys. Rev.39, 270 (1932)
Fite, W.L., Brackmann, R.T.: Phys. Rev.112, 1141 (1958)
Weigold, E., Ugbabe, A., Teubner, P.J.O.: Phys. Rev. Lett.35, 209 (1975)
Ehrhardt, H., Jung, K., Schubert, E.: Coherence and correlation in atomic collisions. Kleinpoppen, H. Williams, J.F. (eds.), Chap. 3. New York: Plenum Publ. Corp. 1980
Pochat, A., Tweed, R.J., Doritch, M., Peresse, J.: J. Phys. B15, 2269 (1982)
Crandall, D.H., Phaneuf, R.A., Gregory, D.C.: Electron impact ionization of multicharged ions. Oak Ridge National Laboratory Report ORNL/TM-7020 (1979) Gregory, D.C., Crandall, D.H., Phaneuf, R.A., Howald, A.M., Dunn, G.H., Falk, R.A., Mueller, D.W., Morgan, T.J.: Oak Ridge National Laboratory Report ORNL/TM-9501
Müller, A., Tinschert, K., Achenbach, C., Becker, R., Salzborn, E.: J. Phys. B18, 3011 (1985)
Kieffer, L.J., Dunn, G.H.: Rev. Mod. Phys.38, 1 (1966)
McDaniel, E.W., Flannery, M.R., Thomas, E.W., Manson, S.T.: At. Data. Nucl. Data Tables33, 1 (1985)
Electron impact ionization. by Märk, T.D., Dunn, G.H. (eds.) Wien, New York: Springer 1985
Tawara, H., Kato, T., Ohnishi, M.: Ionization cross sections of atoms and ions by electron impact. Institute of Plasma Physics, Nagoya University Report IPPJ-AM-37 (1985)
McCarthy, I.E., Weigold, E.: Phys. Rep.27 C, 275 (1976)
Oda, N.: Radiat. Res.64, 80 (1975)
Müller-Fiedler, R., Jung, K., Ehrhardt, H.: (submitted to publication) J. Phys. B
Shyn, T.W., Sharp, W.W., Kim, Y.K.: Phys. Rev. A24, 79 (1981)
Proceedings of the Workshop on Electronic and Ionic Collision Cross Sections needed in the Modeling of Radiation Interactions with Matter. Argonne National Laboratory, Dec. 1983, ANL-84-28
Ehrhardt, H., Schulz, M., Tekaat, T., Willmann, K.: Phys. Rev. Lett.22, 89 (1969)
Van der Wiel, M.J., Brion, C.E.: J. Electron Spectrosc.1, 309 and 443 (1973)
Camilloni, R., Giardini-Guidoni, A., McCarthy, I.E., Stefani, G.: Phys. Rev. A17, 1634 (1978)
Weigold, E., Noble, C.J., Hood, S.T., Fuss, I.: J. Phys. B12, 291 (1979)
Wingerden, B., van, Kimman, J.T.N., Tilburg, M., van, Heer, F.J., de, J. Phys. B14, 2475 (1981)
Lahman-Bennani, A., Wellenstein, H.F., Duguet, A., Lecas, M.: Rev. Sci. Instrum.56, 43 (1985)
Ehrhardt, H., Fischer, M., Jung, K.: Z. Phys. A — Atoms and Nuclei304, 119 (1982)
Beaty, E.C., Hesselbacher, K.H., Hong, S.P., Moore, J.H.: J. Phys. B10, 611 (1977)
Ehrhardt, H., Hesselbacher, K.H., Jung, K., Willmann, K.: J. Phys. B5, 1559 (1972)
Weigold, E., Hood, S.T., McCarthy, I.E.: Phys. Rev. A11, 566 (1975)
Brion, C.E., Hood, S.T., Suzuki, I.H., Weigold, E., Williams, G.R.J.: J. Electron Spectrosc.21, 71 (1980)
Opal, C.D., Beaty, E.C., Peterson, W.K.: At. Data4, 209 (1972)
Rudd, M.E., Dubois, R.D.: Phys. Rev. A16, 26 (1977)
Shyn, T.W., Sharp, W.E.: Phys. Rev. A19, 557 (1979)
Brion, C.E., Hamnett, A.: The excited state in chemical physics. McGowan, J.W. (ed.), Part 2, Vol. 45. New York: Wiley 1981
Cook, J.P.D., McCarthy, I.E., Stelbovics, A.T., Weigold, E.: J. Phys. B17, 2339 (1984)
Walraven, J.T.M., Silvera, I.F.: Rev. Sci. Instrum.53, 1167 (1982)
Este, G.O., Knight, G., Scoles, G.: Chem. Phys.35, 421 (1978)
Wise, H., Wood, B.J.: Adv. At. Mol. Phys.3, 291 (1967)
Hood, S.T., Dixon, A.J., Weigold, E.: J. Phys. E11, 948 (1978)
Lohmann, B., McCarthy, I.E., Stelbovics, A.T., Weigold, E.: Phys. Rev. A30, 758 (1984)
Nesbet, R.K.: Phys. Rev. A20, 58 (1979)
Stefani, G., Camilloni, R., Giardini-Guidoni, A.: Phys. Lett.64 A, 364 (1978)
Jung, K., Müller-Fiedler, R., Schlemmer, P., Ehrhardt, H., Klar, H.: J. Phys. B18, 2955 (1985)
Bethe, H.: Ann. Phys.5, 325 (1930)
Inokuti, M.: Rev. Mod. Phys.43, 297 (1971)
Lassettre, E.N., Skerbele, A., Dillon, M.A.: J. Chem. Phys.50, 1829 (1969)
Fano, U.: Phys. Rev. A2, 353 (1970)
Starace, A.F.: Corpuscles and Radiation in Matter I. Handbuch der Physik. Flügge, S., (ed.), Vol. 31. Berlin, Heidelberg, New York: Springer 1982
Jacobs, V.L.: Phys. Rev. A10, 499 (1974)
Huo, W.M.: J. Chem. Phys.71, 1593 (1979)
Samson, J.A.R.: Adv. At. Mol. Phys.2, 177 (1966)
Samson, J.A.R.: Phys. Rep.28 C, 303 (1976)
Müller-Fiedler, R., Schlemmer, P., Jung, K., Ehrhardt, H.: Z. Phys. A — Atoms and Nuclei320, 89 (1985)
Ehrhardt, H., Knoth, G., Schlemmer, P., Jung, K.: Phys. Lett.110 A, 92 (1985)
Oda, N., Nishimura, F., Tahira, S.: J. Phys. Soc. Jpn.33, 462 (1972)
Wannier, G.H.: Phys. Rev.90, 817 (1953)
Rau, A.R.P.: Phys. Rev. A4, 207 (1971)
Rau, A.R.P.: J. Phys. B9, L 283 (1976)
Rudge, M.R.H.: Rev. Mod. Phys.40, 564 (1968)
Schulz, M.: J. Phys. B6, 2580 (1973)
Phillips, D.H., McDowell, M.R.C.: J. Phys. B6, L 165 (1973)
Joachain, C.J., Piraux, B., Potvliege, R.M., Furtado, F., Byron, F.W. Jr.: Phys. Lett. A (submitted for publication)
Glassgold, A.E., Ialongo, G.: Phys. Rev.175, 151 (1968)
Veldre, V. Ya., Damburg, R. Ya., Peterkop, R.K.: Atomic collisions. London: Butterworths 1966
Peterkop, R.P.: Phys. Rev.164, 1220 (1967)
Ehrhardt, H., Hesselbacher, K.H., Jung, K., Willmann, K.: Case Studies in Atomic Collision Physics II, 159 (1972)
Lahmam-Bennani, A., Wellenstein, H.F., Dal Capello, C., Roualt, M., Duguet, A.: J. Phys. B16, 2219 (1983)
Geltman, S.: J. Phys. B7, 1994 (1974)
Robb, W.D., Rountree, S.P., Burnett, T.: Phys. Rev. A11, 1193 (1975)
Byron, F.W. Jr., Joachain, C.J., Piraux, B.: J. Phys. B13, L 673 (1980)
Jacobs, V.L.: Phys. Rev. A3, 289 (1971)
Ehrhardt, H., Fischer, M., Jung, K., Byron, F.W. Jr., Joachain, C.J., Piraux, B.: Phys. Rev. Lett.48, 1807 (1982)
Byron, F.W. Jr., Joachain, C.J.: Phys. Rev.146, 1 (1966)
Klar, H., Jung, K., Ehrhardt, H.: Phys. Rev. A29, 405 (1984)
Seaton, M.J.: Proc. Phys. Soc.88, 801 (1966)
Franz, A., Klar, H.: Z. Phys. D — Atoms, Molecules and Clusters1, 33 (1986)
Joachain, C.J.: Quantum collision theory. Amsterdam: North-Holland 1975
Madison, D.H., Calhoun, R.V., Shelton, W.N.: Phys. Rev. A16, 552 (1977)
Bransden, B.H., Smith, J.J., Winters, K.H.: J. Phys. B11, 3095 (1978)
Sloan, I.H.: Proc. R. Soc. London Ser. A281, 151 (1964)
Tweed, R.J.: J. Phys. B13, 4467 (1980)
Byron, F.W. Jr., Joachain, C.J., Piraux, B.: Phys. Lett.99 A, 427 (1983)
Byron, F.W. Jr., Joachain, C.J., Piraux, B.: J. Phys. B15, L 293 (1982)
McGuire, J.H., Hidalgo, M.B., Doolen, G.D., Nuttall, J.: Phys. Rev. A7, 973 (1973)
Roy, A.C., Das, A.K., Sil, N.C.: Phys. Rev. A23, 1662 (1981)
Klar, H., Franz, A., Tenhagen, H.: (to be published)
Roy, A.C., Klar, H., Schlemmer, P., Jung, K., Ehrhardt, H.: (to be published)
Ehrhardt, H., Hesselbacher, K.H., Jung, K., Schulz, M., Willmann, K.: J. Phys. B5, 2107 (1972)
Joachain, C.J.: Private Communication 1984
Popov, Yu. V., Erokhin, V.F.: Phys. Lett.97 A, 280 (1983)
Stefani, G., Avaldi, L., Lahmam-Bennani, A., Duguet, A.: XIV ICPEAC, Contributed papers, 176, Palo Alto (1985)
Schubert, E., Schuck, A., Jung, K., Geltman, S.: J. Phys. B12, 967 (1979)
Baum, G., Kisker, E., Raith, W., Schröder, W., Sillman, U., Zenses, D.: J. Phys. B14, 4377 (1981)
Alguard, M.J., Hughes, V.W., Lubell, M.S., Wainwright, P.F.: Phys. Rev. Lett.39, 334 (1977)
McGowan, J.W., Clarke, E.M.: Phys. Rev.167, 43 (1968)
Marchand, P., Paquet, C., Marmet, P.: Phys. Rev.180, 123 (1969)
Brion, C.E., Thomas, G.E.: Int. J. Mass. Spectrom. Ion Phys.1, 25 (1968)
Vinkalns, I., Gailitis, M.: Latvian Acad. Sci. Rep.4, 17 (1967) Riga
Cvejanovics, S., Read, F.H.: J. Phys. B14, 1841 (1974)
Schubert, E., Jung, K., Ehrhardt, H.: J. Phys. B14, 3267 (1981)
Fournier-Lagarde, P., Mazeau, J., Huetz, A.: J. Phys. B17, L 591 (1984)
Klar, H., Schlecht, W.: J. Phys. B9, 1699 (1976)
Greene, C.H., Rau, A.R.P.: Phys. Rev. Lett.48, 533 (1982)
Greene, C.H., Rau, A.R.P.: J. Phys. B16, 99 (1983)
Altick, P.L.: J. Phys. B18, 1841 (1985)
Read, F.H.: J. Phys. B17, 3965 (1984)
Hammond, P., Read, F.H., Cvejanovics, S., King, G.C.: XIV. ICPEAC, Contributed papers, 158, Palo Alto (1985)
Peterson, W.K., Opal, C.B., Beaty, E.C.: J. Phys. B4, 1020 (1971)
Srivastava, S.K., Chutjian, A., Trajmar, S.: J. Chem. Phys.63, 2659 (1975)
Yong-Ki Kim: Phys. Rev. A28, 656 (1983)
Avaldi, L., Stefani, G.: XIV ICPEAC, Contributed papers, 157, Palo Alto (1985)
Goruganthu, R.R., Wilson, W.G., Bonham, R.A.: XIV ICPEAC, Contributed papers., 691, Palo Alto (1985)
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Ehrhardt, H., Jung, K., Knoth, G. et al. Differential cross sections of direct single electron impact ionization. Z Phys D - Atoms, Molecules and Clusters 1, 3–32 (1986). https://doi.org/10.1007/BF01384654
Received:
Revised:
Issue Date:
DOI: https://doi.org/10.1007/BF01384654