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The geographical distribution and temporal variations of acidic deposition in Eastern North America

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Abstract

Data from two national precipitation chemistry monitoring networks, and several regional air and precipitation chemistry networks are used to describe some broad-scale features of acidic deposition in eastern North America. In northeastern North America, the coefficient of variation is shown to increase from 10–16% for annual averages to nearly 100% for daily values. There is a strong annual cycle in H+, SO sup=inf4 and NH sup+inf4 deposition and some of the other ions although these cycles are not all in phase. The wet NO sup−inf3 deposition contributes relatively more than SO sup=inf4 to the acidity of snow as compared to rain. Wet deposition is highly “episodic” with about 50% to 70% of the total annual deposition of SO sup=inf4 and NO sup−inf3 accumulating in the highest 20% of the days. Estimates made in various ways indicate that, over eastern North America as a whole, dry deposition is approximately equal to wet for both SO sup=inf4 and NO sup−inf3 . Dry may exceed wet in the high emissions zone but drops to about 20% of the total deposition in more remote areas. Deposition via fog or low cloud impaction is an important input to high elevation forests, but more data are required to quantify the magnitude and regional extent of this.

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References

  • Achtemeier, G.L., Hildebrand, P.H., Schickedanz, P.T., Ackerman, B., Changnon, Jr., S.A., and Semonin, R.G.,: 1977, ‘Illinois Precipitation Enhancement Program Design and Evaluation Techniques for High Plains Cooperative Program’, Ill, State Water Survey Final Report on Contract 14-06-D-7197, Appendix B.

  • Barnes, S.L.: 1964, J. Appl. Meteorol., 3, 396.

    Google Scholar 

  • Barnes, S.L.: 1973, ‘Mesoscale objective map analysis using weighted time-series observations“. NOAA Tech. Memo. 62, NSSL, 60 pp.

  • Barrie, L.A. and Sirois,A.: 1982, ”An Analysis and Assessment of Precipitation Chemistry Measurements made by CANSAP (The Canadian Network for Sampling Precipitation): 1977–1980“. Report AQRB-82-003-T, Atmospheric Environment Service, Toronto, Canada, 163pp.

    Google Scholar 

  • Barrie, L.A. and Sirois, A.: 1986, J. Water, Air and Soil Poll., 22, in press.

  • Barrie, L.A. and Hales, J.M.: 1984, Tellus., 36B, 333.

    Google Scholar 

  • Bowersox, V.C. and dePena, R.G.:1980, J. Geophys. Res., 85, 5614.

    Google Scholar 

  • Bowersox, V.C. and Stensland, G.J.: 1981, “Seasonal Patterns of Sulfate and Nitrate in Precipitation in the United States”. Proc. 74th Annual Meeting of APCA, Philadelphia, PA, June 1981.

  • Bowersox, V.C. and Stensland, G.J.: 1985, “Seasonal Variations in the Chemistry of Precipitation in the United States”, Proc. 78th Annual Meeting, Air Pollution Control Assoc. Detroit, Mich., June 1985.

  • Castillo, R.A., Juisto,J.E., and McLaren, E.: 1983, Atmos. Env., 17, 1497.

    Google Scholar 

  • Castillo, R.A., Kadlecek, J. and McLaren, S.: 1985, J. Water, Air and Soil Poll., 24, 323.

    Google Scholar 

  • Chan, W.H., Tang, A.J.S., Chung, D.H.S., Kirk, R.W. and Lusis, M.A.: 1986, Atmos. Env., 20, in press.

  • Falconer, R.E. and Falconer, P.D.: 1980, J. Geophys. Res., 85, 7465.

    Google Scholar 

  • Galloway, J.N. and Whelpdale, D.M.: 1980, Atmos. Env., 14, 409.

    Google Scholar 

  • Galloway, J.N., Whelpdale, D.W., and Wolff, G.T.: 1984, Atmos. Env., 18, 2595.

    Google Scholar 

  • Kurtz, J., Tang, A.J.S., Kirk, R.W. and Chan, W.H.: 1984, “Analysis of an Acid Deposition Episode at Dorset, Ontario”, Atmos. Env., 18, 387–394.

    Google Scholar 

  • Lindberg, S., Bigelow, D., Bowersox, V., Knapp, W. and Olsen, T.: 1985, ‘NADP Annual Data Summary, Precipitation Chemistry in the United States, 1982”. Chapter II - Data Selection Criteria, Natural Resource Ecology Laboratory, Ft. Collins, Co., pp. 3–8.

    Google Scholar 

  • Logan, J.A.: 1984, J. Geophys. Res., 88, 10, 785.

    Google Scholar 

  • Lovett, G.M.: 1984, Atmos. Env., 18, 361.

    Google Scholar 

  • MAP3S/RAINE Research Community.: 1982, Atmos. Env., 16, 1603.

    Google Scholar 

  • Munn, R.E., Whelpdale, D.M., Oehlert, G.W., and Summers, P.W.: 1986, Atmos. Env., 20, in press.

  • National Academy of Sciences: 1983, “Acid Deposition: Atmospheric Processes in Eastern North Americard, National Academy Press, Washington, D.C., 375 pp.

    Google Scholar 

  • Newcombe, C.P.: 1985, Env. Management, 9, 277.

    Google Scholar 

  • Sheih, C.M., Wesley, M.L. and Hicks, B.B.: 1979, Atmos. Env., 13, 1361.

    Google Scholar 

  • Siccama, T.G.: 1974, Ecol. Mon., 44, 325.

    Google Scholar 

  • Stensland, G.J., Semonin, R.G. Peden, M.E., Bowersox, V.C. McGurk, F.F., Skowron, L.M., Slater, M.J. and Stahlhut, R.K.: 1980, “NADP Quality Assurance Report - Central Analytical Laboratory, 1979 National Atmospheric Deposition Program, Illinois State Water Survey, Champaign, Ill., U.S.A.

    Google Scholar 

  • Voldner, E.C., Sirois, A. and Clark, T.L.: 1984, “Data Screening and Calculation Procedures for the North American Precipitation Chemistry Data to be Used in the International Sulfur Deposition Model Evaluation“. Proceedings of the APCA/ASQC Specialty Conference on Quality Assurance in Air Pollution Measurements, Air Pollution Control Assoc., Pittsburgh, PA, 13 pp.

    Google Scholar 

  • Voldner, E. and Sirois, A.: 1986, J. Water Air and Soil Poll., 22, in press.

  • Watson, C.R. and Olsen, A.R.: 1984, “Acid Deposition System (ADS) for Statistical Reporting: System Design and User's Code Manual”. EPA-600-8-84-023, U.S. Environmental Protection Agency, Research Triangle Park, N.C.

  • Wesley, M.L. and Hicks, B.B.: 1977, J. Air Poll. Control Assoc., 27, 1110.

    Google Scholar 

  • Whelpdale, D.M. and Barrie, L.A.: 1982, J. Water, Air and Soil Poll., 18, 7.

    Google Scholar 

  • Wilson, J.W., and Mohnen, V.A.: 1982, J. Water, Air and Soil Poll., 18, 199.

    Google Scholar 

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Summers, P.W., Bowersox, V.C. & Stensland, G.J. The geographical distribution and temporal variations of acidic deposition in Eastern North America. Water, Air, and Soil Pollution 31, 523–535 (1986). https://doi.org/10.1007/BF00284210

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