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Nature and Estimation of Functional Groups on Solid Surfaces

  • Chapter
Catalysis

Part of the book series: CATALYSIS — Science and Technology ((CATALYSIS,volume 4))

Abstract

The lattice of a crystal is abruptly terminated at its surface. In consequence, the constituents of the lattice are unsaturated in their coordination, giving rise to the surface energy. Adsorption of substances which are foreign to the lattice may lower the energy of the system and reduce the coordinative “unsaturation”. The interaction of the adsorptive with the adsorbent can very greatly in nature, i.e. from weak interaction by van der Waals forces, leading to physisorption, to strong chemical bonding or chemisorption. Chemisorption of molecules is frequently dissociative and often irreversible as well, that is the adsorptive cannot always be recovered in its original form. An example is the chemisorption of oxygen, O2, on carbon giving rise to surface oxides [1] which yield CO and CO2 on thermal decomposition.

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Authors and Affiliations

  1. Institut für Anorganische Chemie, Universität München, Meiserstraße 1, D-8000, München 2, Germany

    Hanns-Peter Boehm

  2. Institut für Physikalische Chemie, Universität München, Sophienstraße 11, D-8000, München 2, Germany

    Helmut Knözinger

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  1. Hanns-Peter Boehm
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Editors and Affiliations

  1. CSIRO Division of Materials Science Catalysis and Surface Science Laboratory, University of Melbourne, Victoria, Australia

    John R. Anderson

  2. Dept. of Chemical Engineering, Stanford University, Standford, CA, 94305, USA

    Michel Boudart

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Boehm, HP., Knözinger, H. (1983). Nature and Estimation of Functional Groups on Solid Surfaces. In: Anderson, J.R., Boudart, M. (eds) Catalysis. CATALYSIS — Science and Technology, vol 4. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-93229-8_2

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