Abstract
Bodenstein was the first in the field of catalysis identifying correctly the concentrations of the adsorbed species as controlling element for many heterogeneous reaction systems. While failing to be correct in all details, Bodenstein prepared the ground for many others on their way to a detailed understanding of heterogeneous catalysis kinetics.
In this contribution, the interaction between surface and gas-phase reactions and their coupling by molecular transport is investigated numerically. Two examples are discussed more detailed: heterogeneous ignition and diamond formation by chemical vapour deposition.
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Behrendt, F., Deutschmann, O., Ruf, B., Schmidt, R., Warnatz, J. (1996). Simulation of Heterogeneous Reaction Systems. In: Wolfrum, J., Volpp, HR., Rannacher, R., Warnatz, J. (eds) Gas Phase Chemical Reaction Systems. Springer Series in Chemical Physics, vol 61. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-80299-7_21
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DOI: https://doi.org/10.1007/978-3-642-80299-7_21
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