Abstract
In molecular spectroscopy, the introduction of more than one resonant electromagnetic field is a well-established technique applied in the full spectral range between radiofrequency (rf) and ultraviolet.(1) The main motivation for extending single resonance to double or multiple resonance techniques can be twofold: (1) either one wants to increase the sensitivity of detection by “quantum transformation” from low-frequency absorbed quanta to high-frequency detected quanta, or (2) one wants to enhance the resolution of the spectra, i.e., reduce the number of spectral lines in a given frequency range by introducing specific coherent time-dependent interactions that average out unwanted static interactions in the Hamiltonian,(2) by imposing additional “selection rules,”(2) or by exploiting degeneracies of certain transitions.(3)
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Möbius, K., Biehl, R. (1979). Electron-Nuclear-Nuclear TRIPLE Resonance of Radicals in Solutions. In: Dorio, M.M., Freed, J.H. (eds) Multiple Electron Resonance Spectroscopy. Springer, Boston, MA. https://doi.org/10.1007/978-1-4684-3441-5_14
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