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Free-Standing Carbon Nanotube Thin Film for Multifunctional Halide-Perovskite Optoelectronics

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Bulletin of the Russian Academy of Sciences: Physics Aims and scope

Abstract

Carbon nanotube thin (CNT) films have been extensively studied in optoelectronics for the past two decades. Regarding its chemical inertness they have been successfully integrated with halide-perovskites for next-generation flexible optoelectronics. Following this approach, a few perovskite-based devices have been created, namely solar cells, photodetectors, and light-emitting diodes. However, the synthesis of a high-quality halide-perovskite material directly on carbon nanotube thin films has not been demonstrated. Here, we for the first time show a simple one-step synthesis of CsPbBr3 microcrystals directly on the substrate-free, free-standing carbon nanotube thin film. We show that the as-synthesized microcrystals show optical lasing at a threshold fluence 140 μJ cm–2. Our simple approach allows to further study substrate-free perovskite lasers on a carbon nanotube thin film. Furthermore, the proposed design will be perspective for multifunctional optoelectronics, where both CNT film and perovskite crystals may respond various applied stimuli.

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Funding

The work was supported by the RF Ministry of Science and Higher Education (project no. 075-15-2021-1349). A.G.N. acknowledges Russian Science Foundation (project no. 22-13-00436) (for synthesis of carbon nanotubes).

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Authors and Affiliations

  1. ITMO University, School of Physics and Engineering, 197101, St. Petersburg, Russia

    A. A. Marunchenko, D. I. Markina, A. P. Pushkarev, M. A. Baranov & S. V. Makarov

  2. Skolkovo Institute of Science and Technology, 121205, Moscow, Russia

    A. G. Nasibulin

Authors
  1. A. A. Marunchenko
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  2. D. I. Markina
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  3. A. P. Pushkarev
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  4. M. A. Baranov
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  5. A. G. Nasibulin
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  6. S. V. Makarov
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Corresponding author

Correspondence to A. A. Marunchenko.

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Marunchenko, A.A., Markina, D.I., Pushkarev, A.P. et al. Free-Standing Carbon Nanotube Thin Film for Multifunctional Halide-Perovskite Optoelectronics. Bull. Russ. Acad. Sci. Phys. 86 (Suppl 1), S127–S130 (2022). https://doi.org/10.3103/S1062873822700538

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  • DOI: https://doi.org/10.3103/S1062873822700538

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