Abstract
Different from the regular method with peak-shape function fitting, in this work, the idea of alpha-spectra analysis using non-negative iterative deconvolution method is proposed. Two non-negative iterative algorithms, the Boosted Gold and the Boosted Richardson–Lucy, were applied to unfold and analyze alpha-particle spectra. The detector response matrix was constructed with the AASI, which is a Monte Carlo simulation software specifically for alpha-particle spectra. A \(^{244}\)Cm alpha-particle source was measured and tested for peak-position deconvolution. A \(^{238+239+240}\)Pu alpha-particle spectrum was used to prove the validity of quantitative analysis by deconvolution algorithms. Both the Boosted Gold and the Boosted Richardson–Lucy can get accurate results for peak positions and content ratios. In terms of running speed, the Boosted Gold was faster than the Boosted Richardson–Lucy.
Similar content being viewed by others
References
G.F. Knoll, Radiation detection and measurement (John Wiley & Sons, 2010)
R. Pöllänen, T. Siiskonen, S. Ihantola, H. Toivonen, A. Pelikan, K. Inn, J. La Rosa, B. Bene, Determination of \(^{239}\)pu/\(^{240}\)pu isotopic ratio by high-resolution alpha-particle spectrometry using the adam program. Applied Radiation and Isotopes 70(4), 733–739 (2012)
S.K. Aggarwal, Alpha-particle spectrometry for the determination of alpha emitting isotopes in nuclear, environmental and biological samples: past, present and future. Analytical Methods 8(27), 5353–5371 (2016)
C.W. Sill, Determination of radium-226 in ores, nuclear wastes and environmental samples by high-resolution alpha spectrometry. Nuclear and chemical waste management 7(3–4), 239–256 (1987)
K. Burns, Determination of radium and uranium isotopes in natural waters by sorption on hydrous manganese dioxide followed by alpha-spectrometry. Journal of radioanalytical and nuclear chemistry 264(2), 437–443 (2005)
H. Amano, A. Kasai, T. Matsunaga, Simultaneous measurement of rn and its progeny in cave air by liquid scintillation techniques and \(\alpha \)-ray spectrometry. Health physics 49(3), 509–511 (1985)
S. Furuta, K. Ito, Y. Ishimori, A continuous radon progeny monitor with a vacuum vessel by alpha spectrometry. Radiation protection dosimetry 90(4), 429–436 (2000)
A.M. Sánchez, D.C. Marzal, Experimental study of the curve-shape variations in alpha-particle spectrometry. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 414(2–3), 265–273 (1998)
R. Shi, X.-G. Tuo, H.-L. Li, J.-B. Yang, Y. Cheng, H.-L. Zheng, \(^{239}\)pu alpha spectrum analysis based on pips detector response function and variations with vacuum and distance. Nuclear Science and Techniques 28(1), 4 (2017)
E. Steinbauer, G. Bortels, P. Bauer, J. Biersack, P. Burger, I. Ahmad, A survey of the physical processes which determine the response function of silicon detectors to alpha particles. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 339(1–2), 102–108 (1994)
P. Martin, G.J. Hancock, Peak resolution and tailing in alpha-particle spectrometry for environmental samples. Applied Radiation and Isotopes 61(2–3), 161–165 (2004)
G.A. Marzo, A comparison of different peak shapes for deconvolution of alpha-particle spectra. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 832, 191–201 (2016)
S. Pommé, B.C. Marroyo, Improved peak shape fitting in alpha spectra. Applied Radiation and Isotopes 96, 148–153 (2015)
R. Shi, X. Tuo, J. Yang, Y. Cheng, H. Zheng, Q. Wang, C. Deng, A peak shape model with high-energy tailing for high-resolution alpha-particle spectra. The European Physical Journal A 55(8), 138 (2019)
R. Shi, X. Tuo, H. Zheng, H. Li, Y. Xu, Q. Wang, C. Deng, Fast adaptive particle spectrum fitting algorithm based on moment-estimated initial parameters. Applied Radiation and Isotopes 129, 1–5 (2017)
M. Morháč, J. Kliman, V. Matoušek, M. Veselskỳ, I. Turzo, Efficient one-and two-dimensional gold deconvolution and its application to \(\gamma \)-ray spectra decomposition. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 401(2–3), 385–408 (1997)
M. Morháč, Deconvolution methods and their applications in the analysis of \(\gamma \)-ray spectra. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 559(1), 119–123 (2006)
A. Mohammad-Djafari, J.-F. Giovannelli, G. Demoment, J. Idier, Regularization, maximum entropy and probabilistic methods in mass spectrometry data processing problems. International Journal of Mass Spectrometry 215(1–3), 175–193 (2002)
M. Morháč, V. Matoušek, Complete positive deconvolution of spectrometric data. Digital Signal Processing 19(3), 372–392 (2009)
M. Morháč, V. Matoušek, High-resolution boosted deconvolution of spectroscopic data. Journal of Computational and Applied Mathematics 235(6), 1629–1640 (2011)
T. Siiskonen, R. Pöllänen, Advanced simulation code for alpha spectrometry. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 550(1–2), 425–434 (2005)
S. Ihantola, A. Pelikan, R. Pöllänen, H. Toivonen, Advanced alpha spectrum analysis based on the fitting and covariance analysis of dependent variables. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 656(1), 55–60 (2011)
R. Pöllänen, T. Siiskonen, M. Moring, J. Juhanoja, Direct alpha spectrometry for characterising hot particle properties. Radiation Measurements 42(10), 1666–1673 (2007)
Y. Ranebo, R. Pöllänen, M. Eriksson, T. Siiskonen, N. Niagolova, Characterization of radioactive particles using non-destructive alpha spectrometry. Applied Radiation and Isotopes 68(9), 1754–1759 (2010)
G. Bortels, A. Verbruggen, G. Sibbens, T. Altzitzoglou, Euromet project no 325: Analysis of plutonium alpha-particle spectra, Tech. rep., Internal Report IRMM, GE/R/RN/01/96 (1996)
R.C. Noy, E. Garcıa-Toraño, E. Mainegra, E. López, The winalpha code for the analysis of alpha-particle spectra. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 525(3), 522–528 (2004)
Acknowledgements
This work is supported by the National Natural Science Foundation of China (Grant Nos. 41874213, 41604154, and U19A2086) and the Opening Project of Key Laboratory of Higher Education of Sichuan Province for Enterprise Informationalization and Internet of Things (Grant No. 2019WZJ01). The authors would like to thank Dr. Hurtado Santiago (Servicio de Radioisotopos, CITIUS, Universidad de Sevilla, Spain) for providing the EUROMET-5535 reference spectrum.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Shi, R., Tuo, X., Cheng, Y. et al. Applications of non-negative iterative deconvolution method in the analysis of alpha-particle spectra. Eur. Phys. J. Plus 135, 225 (2020). https://doi.org/10.1140/epjp/s13360-020-00100-9
Received:
Accepted:
Published:
DOI: https://doi.org/10.1140/epjp/s13360-020-00100-9