Abstract
Roof runoff is generally perceived as a relatively clean source of water and is therefore often discharged or used without any treatment. Available data from literature however show that roof runoff can be contaminated by a wide range of (micro)pollutants, and in concentrations often exceeding surface water quality and/or drinking water standards. In this review, information on more than 100 contaminants, including trace metals, polycyclic aromatic hydrocarbons, pesticides, phthalates, alkylphenols and alkylphenolethoxylates, is summarized and a meta-analysis provides quantitative proof that roof runoff is a major contributor to stormwater quality deterioration. The two prime sources of roof runoff contamination are leaching from roofing materials and atmospheric deposition. A detailed discussion on material-pollutant relationships is given and a benchmarking method is presented which ranks roofing materials based on their runoff quality. Treated wood roofing and metallic rooftops (copper and zinc) were found to have the highest impact on water quality. Atmospheric deposition is also discussed in detail and includes a summary on the concentration levels in deposition for more than 400 pollutants such as trace metals, pesticides and polycyclic aromatic hydrocarbons. As a conclusion, it can be argued that the general perception on roof runoff quality is inaccurate and that its quality aspects should not be overlooked when roof runoff is used or discharged.
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Abbreviations
- 2,4-D:
-
2,4-Dichlorophenoxyacetic acid
- ACC:
-
Acid copper chromate
- ACQ:
-
Alkaline copper quat
- ACZA:
-
Ammoniacal copper zinc arsenate
- AMPA:
-
Aminomethylphosphonic acid
- AP:
-
Alkylphenol
- APEO:
-
Alkylphenol ethoxylate
- APP:
-
Atactic polypropylene
- BBP:
-
Butyl benzyl phthalate
- BGV:
-
Best guess value
- BPA:
-
Bisphenol A
- CA:
-
Copper azole
- CCA:
-
Chromated copper arsenate
- CBGV :
-
The calculated best guess value
- Cmax ABS :
-
Absolute maximal concentration of a certain pollutant as reported in literature
- Cmax SV :
-
Maximal concentration of the available selected values for a certain pollutant
- Cmean TE :
-
Mean concentration of a certain pollutant based on the triple estimate approach
- Cmean TE, DC :
-
Deposition corrected mean concentration of a certain pollutant based on the triple estimate approach
- Cmin SV :
-
Minimal concentration of the available selected values for a certain pollutant
- COD:
-
Chemical oxygen demand
- DBP:
-
Dibutyl phthalate
- DBPP:
-
Dibutyl phenyl phosphate
- DDD:
-
Dichlorodiphenyldichloroethane
- DDE:
-
Dichlorodiphenyldichloroethylene
- DDT:
-
Dichlorodiphenyltrichloroethane
- DEHP:
-
Bis(2-ethylhexyl) phthalate
- DEP:
-
Diethyl phthalate
- DF:
-
Calculated detection frequency for a certain pollutant
- DIBP:
-
Diisobutyl phthalate
- DIDP:
-
Diisodecyl phthalate
- DINP:
-
Diisononyl phthalate
- DMP:
-
Dimethyl phthalate
- DNOC:
-
Dinitro-ortho-cresol
- DNOP:
-
Di-n-octyl phthalate
- DOC:
-
Dissolved organic carbon
- DWQS:
-
Drinking water quality standards
- DWQSstrictest :
-
Strictest possible drinking water quality standard for a certain pollutant
- EPDM:
-
Ethylene propylene diene monomer
- EVA:
-
Ethylene vinyl acetate terpolymer
- FPO/TPO:
-
Flexible polyolefin/thermoplastic polyolefin
- HBCD:
-
Hexabromocyclododecane
- HCH:
-
Hexachlorocyclohexane
- KOC :
-
Organic carbon–water partitioning coefficient
- KOW :
-
Octanol–water partitioning coefficient
- LLT:
-
Laboratory leaching test
- MCPA:
-
2-Methyl-4-chlorophenoxyacetic acid
- MCPP:
-
Mecoprop
- MI:
-
Material index
- MIDW :
-
Drinking water material index
- MISW :
-
Environmental/surface water material index
- ne :
-
Number of sampled/reported (rain) events
- np :
-
Number of pollutants found in the runoff of a certain material
- NP:
-
Nonylphenol
- NP1EO:
-
Nonylphenol monoethoxylate
- NP2EO:
-
Nonylphenol diethoxylate
- NP3EO:
-
Nonylphenol triethoxylate
- NPEO:
-
Nonylphenol ethoxylate
- nSV :
-
Number of selected values
- OP:
-
Octylphenol
- OP3EO:
-
Octylphenol triethoxylate
- OPEO:
-
Octylphenol ethoxylate
- PAH:
-
Polycyclic aromatic hydrocarbons
- PBDE:
-
Polybrominated diphenyl ether
- PCB:
-
Polychlorinated biphenyl
- PCP:
-
Pentachlorophenol
- PIB:
-
Polyisobutylene
- PMMA:
-
Polymethylmethacrylate
- PVC:
-
Polyvinylchloride
- SBS:
-
Styrene butadiene styrene
- SFA:
-
Substance flow analysis
- SV:
-
Selected value
- SWQS:
-
Surface water quality standards
- SWQSstrictest :
-
Strictest possible surface water quality standard for a certain pollutant
- TBEP:
-
Tris(2-butoxyethyl) phosphate
- TBP:
-
Tributyl phosphate
- TCEP:
-
Tris(2-chloroethyl) phosphate
- TCP:
-
Tris(methylphenyl) phosphate
- TCPP:
-
Tris(2-chloroisopropyl) phosphate
- TDCPP:
-
Tris(1,3-dichloro-2-propyl) phosphate
- TE:
-
Triple estimate approach
- TEP:
-
Triethyl phosphate
- TiBP:
-
Triisobutyl phosphate
- TN:
-
Total nitrogen
- TOC:
-
Total organic carbon
- TP:
-
Total phosphorus
- TPP:
-
Triphenyl phosphate
- TPPO:
-
Triphenyl phosphine oxide
- TPrP:
-
Tripropyl phosphate
- TPU:
-
Thermoplastic polyurethane
- WHO:
-
World Health Organization
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De Buyck, PJ., Van Hulle, S.W.H., Dumoulin, A. et al. Roof runoff contamination: a review on pollutant nature, material leaching and deposition. Rev Environ Sci Biotechnol 20, 549–606 (2021). https://doi.org/10.1007/s11157-021-09567-z
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DOI: https://doi.org/10.1007/s11157-021-09567-z