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Measurement of radon concentrations and their annual effective doses in soils and rocks of Jaintiapur and its adjacent areas, Sylhet, North-east Bangladesh

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Abstract

The study investigates the measurement of radon concentration in soils and rocks as a natural tracer for exploring uranium mineralization, first of its kind in Bangladesh. The range of radon concentration was measured as 8–4360 Bq/m3 with an average of 851.41 Bq/m3. Among the measured values, 2120–4360 Bq/m3 was observed in the Tertiary sediments whereas 8–584 Bq/m3 was found in the Recent alluvial soil of different bils and haors. These high radon concentrations are explained by geogenic factors such as mineral content in rocks, alluvium cover, sufficient porosity, probable subsurface fault, and flooding by water streamed through adjacent uranium-rich areas in India. The radon values indicate that the rock formations are promising for uranium mineralization. The radon concentration in rocks and soils are well comparable to the similar studies of the other parts of the world. The results are in good agreement with the previous radiometric survey results, suggestive to extensive exploration activities to confirm uranium mineralization in the area. Moreover, the average annual effective dose of 0.008092 mSv/y in the region calculated from the radon values is within the WHO and ICRP safety limits.

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References

  1. Peake R, Schumann R (1993) Regional radon characterizations. In: U.S. Geological Survey (ed) Field Studies of Radon in Rocks, Soils and Water, 1st edn. Florida, United States

  2. Choubey VM, Sharma KK, Ramola RC (1997) Geology of radon occurrence around Jari in Parvati Valley, Himachal Pradesh, India. J Environ Radioact 34(2):139–147. https://doi.org/10.1016/0265-931X(96)00024-0

    Article  CAS  Google Scholar 

  3. Appleton JD, Miles JCH (2010) A statistical evaluation of the geogenic controls on indoor radon concentrations and radon risk. J Environ Radioact 101(10):799–803. https://doi.org/10.1016/j.jenvrad.2009.06.002

    Article  CAS  PubMed  Google Scholar 

  4. Sundal AV, Valen V, Soldal O, Strand T (2008) The influence of meteorological parameters on soil radon levels in permeable glacial sediments. Sci Total Environ 389(2–3):418–428. https://doi.org/10.1016/j.scitotenv.2007.09.001

    Article  CAS  PubMed  Google Scholar 

  5. Zafrir H, Barbosa SM, Malik U (2013) Differentiation between the effect of temperature and pressure on radon within the subsurface geological media. Radiat Meas 49(1):39–56. https://doi.org/10.1016/j.radmeas.2012.11.019

    Article  CAS  Google Scholar 

  6. Alonso H, Rubiano JG, Guerra JG, Arnedo MA, Tejera A, Martel P (2019) Assessment of radon risk areas in the Eastern Canary Islands using soil radon gas concentration and gas permeability of soils. Sci Total Environ 664:449–460. https://doi.org/10.1016/j.scitotenv.2019.01.411

    Article  CAS  PubMed  Google Scholar 

  7. Abbasi A (2013) Calculation of gamma radiation dose rate and radon concentration due to granites used as building materials in Iran. Radiat Prot Dosim 155(3):335–342. https://doi.org/10.1093/rpd/nct003

    Article  CAS  Google Scholar 

  8. Sprinkel DA, Solomon BJ (1990) Radon hazards in Utah: Utah geological and mineral survey, Utah, USA. 81:1–28

  9. Ramola RC, Rawat RBS (1997) Assessment of health risk due to exposure of radon and its daughter products in the lower atmosphere. Curr Sci 73(9):771–774

  10. Erees FS, Yener G, Salk M, Özbal Ö (2006) Measurements of radon content in soil gas and in the thermal waters in Western Turkey. Radiat Meas 41(3):354–361. https://doi.org/10.1016/j.radmeas.2005.06.030

    Article  CAS  Google Scholar 

  11. Abbasi A, Mirekhtiary F (2013) Comparison ofactive and passive methods for radon exhalation from a high-exposure buildingmaterial. Radiat Prot Dosim 157(4):570–574. https://doi.org/10.1093/rpd/nct163

    Article  CAS  Google Scholar 

  12. Akon E (2013) Exploration of atomic minerals in Bangladesh. Energy Power, Dhaka, pp 105–108

    Google Scholar 

  13. Majumder R, Khalil M, Rashid M (2014) Uranium exploration status in Bangladesh: conceptual feasibility studies. IAEA-CN-216 Abstact 167. http://inis.iaea.org/Search/search.aspx?orig_q=RN:48039517. Accessed 16 Sept 2020

  14. Vilcapoma LL et al (2019) Measurement of radon in soils of Lima city - Peru during the period 2016–2017. Earth Sci Res J 23(3):171–183. https://doi.org/10.15446/esrj.v23n3.74108

    Article  Google Scholar 

  15. Asgharizadeh F, Abbasi A, Hochaghani O, Gooya ES (2012) Natural radioactivity in granite stones used as building materials in Iran. Radiat Prot Dosim 149(3):321–326. https://doi.org/10.1093/rpd/ncr233

    Article  CAS  Google Scholar 

  16. UNSCEAR 2016 Report. United Nations Scientific Committee on the Effects of Atomic Radiation (2017) Sources, effects and risks of ionizing radiation. Report to the General Assembly, with Scientific Annexes. New York, United Nations Sales Publications

  17. Schauer DA, Linton OW (2009) NCRP report no. 160, ionizing radiation exposure of the population of the United States, medical exposure - Are we doing less with more, and is there a role for health physicists? Health Phys 97(1):1–5. https://doi.org/10.1097/01.HP.0000356672.44380.b7

    Article  CAS  PubMed  Google Scholar 

  18. Alam M, Alam MM, Curray JR, Chowdhury MLR, Gani MR (2003) An overview of the sedimentary geology of the Bengal Basin in relation to the regional tectonic framework and basin-fill history. Sediment Geol 155(3–4):179–208. https://doi.org/10.1016/S0037-0738(02)00180-X

    Article  Google Scholar 

  19. Curray JR (1991) Geological history of the Bengal geosyncline. J Assoc Explor Geophys 12:209–219

    Google Scholar 

  20. Curray JR, Munasinghe T (1991) Origin of the Rajmahal Traps and the 85°E Ridge: preliminary reconstructions of the trace of the Crozet hotspot. Geology 19(12):1237–1240. https://doi.org/10.1130/0091-7613(1991)019%3c1237:OOTRTA%3e2.3.CO;2

    Article  Google Scholar 

  21. Royhan Gani M, Mustafa Alam M (2004) Fluvial facies architecture in small-scale river systems in the Upper Dupi Tila formation, northeast Bengal Basin, Bangladesh. J Asian Earth Sci 24(2):225–236. https://doi.org/10.1016/j.jseaes.2003.11.003

    Article  Google Scholar 

  22. Uddin A, Lundberg N (1998) Unroofing history of the eastern himalaya and the indo-burman ranges: heavy-mineral study of cenozoic sediments from the Bengal basin, Bangladesh. J Sediment Res 68(3):465–472. https://doi.org/10.2110/jsr.68.465

    Article  CAS  Google Scholar 

  23. Gibbons AD, Whittaker JM, Müller RD (2013) The breakup of East Gondwana: assimilating constraints from Cretaceous ocean basins around India into a best-fit tectonic model. J Geophys Res Solid Earth 118(3):808–822. https://doi.org/10.1002/jgrb.50079

    Article  Google Scholar 

  24. Hiller K, Elahi M (1984) Structural development and hydrocarbon entrapment in the Surma Basin. In: Bangladesh (northwest Indo-Burman fold belt): Fifth Offshore Southwest Conference, Singapore 6:50–63. https://doi.org/10.2118/12398-MS

  25. Worm HU et al (1998) Large sedimentation rate in the Bengal Delta: magnetostratigraphic dating of Cenozoic sediments from northeastern Bangladesh. Geology 26(6):487–490. https://doi.org/10.1130/0091-7613(1998)026%3c0487:LSRITB%3e2.3.CO;2

    Article  Google Scholar 

  26. Goodbred SL, Kuehl SA (2000) The significance of large sediment supply, active tectonism, and eustasy on margin sequence development: Late Quaternary stratigraphy and evolution of the Ganges–Brahmaputra delta. Sediment Geol 133(3–4):227–248. https://doi.org/10.1016/S0037-0738(00)00041-5

    Article  Google Scholar 

  27. Uddin A, Lundberg N (2004) Miocene sedimentation and subsidence during continent-continent collision, Bengal basin, Bangladesh. Sediment Geol 164(1–2):131–146. https://doi.org/10.1016/j.sedgeo.2003.09.004

    Article  Google Scholar 

  28. Johnson SY, Nur Alam AM (1991) Sedimentation and tectonics of the Sylhet trough. Bangladesh. Geol Soc Am Bull 103(11):1513–1527. https://doi.org/10.1130/0016-7606(1991)103%3c1513:SATOTS%3e2.3.CO;2

    Article  Google Scholar 

  29. Evans P (1964) The tectonic framework of Assam. J Geol Soc India 5:80–96

    Google Scholar 

  30. Rahman MJJ, Sayem ASM, Bhuiyan MH (2014) Geochemistry of the plio-pleistocene Dupi Tila sandstones from the Surma Basin, Bangladesh: Implications for provenance, tectonic setting and weathering. Himal Geol 35(2):162–170

    Google Scholar 

  31. Rahman MJJ, Worden RH (2016) Diagenesis and its impact on the reservoir quality of Miocene sandstones (Surma Group) from the Bengal Basin, Bangladesh. Mar Pet Geol 77(July):898–915. https://doi.org/10.1016/j.marpetgeo.2016.07.027

    Article  CAS  Google Scholar 

  32. Michael W, Urban C, Gmbh M (2005) Quantitative morphotectonics of the southern Shillong Plateau (Bangladesh/India). Austrian J Earth Sci 97:82–93

    Google Scholar 

  33. Hossain MS, Xiao W, Khan MSH, Chowdhury KR, Ao S (2020) Geodynamic model and tectono-structural framework of the Bengal Basin and its surroundings. J Maps 16(2):445–458. https://doi.org/10.1080/17445647.2020.1770136

    Article  Google Scholar 

  34. Hossain I, Nahar M (2014) The eocene sylhet limestone of Jaflong and adjoining areas, Sylhet: An endangered geoheritage in Bangladesh. Geoheritage 6(4):317–333. https://doi.org/10.1007/s12371-014-0129-5

    Article  Google Scholar 

  35. Khanam F, Rahman MJJ, Alam MM, Abdullah R (2020) Sedimentology and basin-fill history of the Cenozoic succession of the Sylhet Trough, Bengal Basin, Bangladesh. Int J Earth Sci 012345:6789. https://doi.org/10.1007/s00531-020-01946-1

    Article  CAS  Google Scholar 

  36. Brookins G (1990) The indoor radon problem. Columbia University Press, New York

    Google Scholar 

  37. Bossew P et al (2020) Development of a geogenic radon hazard index—concept, history, experiences. Int J Environ Res Public Health 17(11):1–24. https://doi.org/10.3390/ijerph17114134

    Article  Google Scholar 

  38. Tanner A (1978) Radon migration in the ground: a supplementary review. In: U.S. Geological Survey. 78-1050:5–56. https://doi.org/10.3133/ofr781050

  39. Malmqvist L, Isaksson M, Kristiansson K (1989) Radon migration through soil and bedrock. Geoexploration 26:135–144

    Article  Google Scholar 

  40. Nazaro WW (1992) Radon transport from soil to air. Rev Geophys 30:137

    Article  Google Scholar 

  41. Etiope G, Martinelli G (2002) Migration of carrier and trace gases in the geosphere: an overview. Phys Earth Planet Int 129:185–204

    Article  CAS  Google Scholar 

  42. Choubey VM, Ramola RC (1997) Correlation between geology and radon levels in groundwater, soil and indoor air in Bhilangana Valley, Garhwal Himalaya, India. Environ Geol 32(4):258–262. https://doi.org/10.1007/s002540050215

    Article  CAS  Google Scholar 

  43. Bourai AA et al (2013) Measurements of radon flux and soil-gas radon concentration along the Main Central Thrust, Garhwal Himalaya, using SRM and RAD7 detectors. Acta Geophys 61(4):950–957. https://doi.org/10.2478/s11600-013-0132-2

    Article  Google Scholar 

  44. Duggal V, Rani A, Mehra R (2014) Measurement of soil-gas radon in some areas of northern Rajasthan, India. J Earth Syst Sci 123(6):1241–1247. https://doi.org/10.1007/s12040-014-0473-5

    Article  CAS  Google Scholar 

  45. Mujahid SA, Hussain S, Ramzan M (2010) Measurement of radon exhalation rate and soil gas radon concentration in areas of southern Punjab, Pakistan. Radiat Prot Dosim 140(3):300–303. https://doi.org/10.1093/rpd/ncq119

    Article  CAS  Google Scholar 

  46. Deeba F, Rahman SH, Kabir MZ (2020) Radon concentration in soil and groundwater of West Coastal Area, Bangladesh. Radiat Prot Dosim. https://doi.org/10.1093/rpd/ncaa134

    Article  Google Scholar 

  47. Ali N, Khan EU, Akhter P, Khan F, Waheed A (2010) Estimation of mean annual effective dose through radon concentration in the water and indoor air of Islamabad and Murree. Radiat Prot Dosim 141(2):183–191. https://doi.org/10.1093/rpd/ncq160

    Article  CAS  Google Scholar 

  48. Kumar S, Singh S, Bajwa BS, Sabharwal AD (2011) In situ measurements of radon levels in water and soil and exhalation rate in areas of Malwa belt of Punjab (India). Isotopes Environ Health Stud 47(4):446–455. https://doi.org/10.1080/10256016.2011.622441

    Article  CAS  PubMed  Google Scholar 

  49. Al-hamidawi A, Jabar AA, Mashhadani QS, Bayati HA (2012) Measurement of radon and thoron concentrations of soil–gas in Al-Kufa city using RAD-7 detector. Iraqi J Phys 10(19):110–116

    Google Scholar 

  50. Alharbi WR, Abbady AGE (2013) Measurement of radon concentrations in soil and the extent of their impact on the environment from Al-Qassim, Saudi Arabia. Nat Sci 05(01):93–98. https://doi.org/10.4236/ns.2013.51015

    Article  CAS  Google Scholar 

  51. Tabar E, Kumru MN, Içhedef M, Saç MM (2013) Radioactivity level and the measurement of soil gas radon concentration in Dikili geothermal area, Turkey. Int J Radiat Res 11(4):253

    Google Scholar 

  52. Ka K (2013) Depth and Seasonal Variations for the Soil Radon-Gas Concentration Levels at Wadi Naseib Area, Southwestern Sinai, Egypt. J Phys Chem Biophys. https://doi.org/10.4172/2161-0398.1000123

    Article  Google Scholar 

  53. Mehra R, Bala P (2014) Estimation of annual effective dose due to Radon level in indoor air and soil gas in Hamirpur district of Himachal Pradesh. J Geochemical Explor 142:16–20. https://doi.org/10.1016/j.gexplo.2013.07.005

    Article  CAS  Google Scholar 

  54. Ravikumar P, Davis D, Somashekar RK, Prakash KL (2015) Measurement of radon activity in soil gas using RAD7 in the environs of Chitradurga District, Karnataka, India. Earth Sci 80:31078–31082

    Google Scholar 

  55. Atif KH (2016) Determination of Natural Radioactivity and Radon, Thoron Concentrations of Soil in Hilla City-Iraq. J Babylon Univ Pure Appl Sci 24:5

    Google Scholar 

  56. Mittal S, Rani A, Mehra R (2016) Estimation of radon concentration in soil and groundwater samples of Northern Rajasthan, India. J Radiat Res Appl Sci 9(2):125–130. https://doi.org/10.1016/j.jrras.2015.10.006

    Article  CAS  Google Scholar 

  57. Amin SA, Al-Obiady AH, Alwan A (2017) Radon level measurements in soil and sediments at oil field area and its impact on the environment. Eng Technol J Part B Technol J Part B 35(1):1–7

    Google Scholar 

  58. Cucoş A et al (2017) Residential, soil and water radon surveys in north-western part of Romania. J Environ Radioact 166:412–416. https://doi.org/10.1016/j.jenvrad.2016.10.003

    Article  CAS  Google Scholar 

  59. Huynh Nguyen PT, Nguyen VT, Vu NB, Nguyen VD, Le Cong H (2018) Soil radon gas in some soil types in the rainy season in Ho Chi Minh City, Vietnam. J Environ Radioact 193–194:27–35. https://doi.org/10.1016/j.jenvrad.2018.08.017

    Article  CAS  PubMed  Google Scholar 

  60. Sharrad AA (2020) Seasonal radon concentration measurements at Sawa Lake, Samawa City-South of Iraq. MS Thesis. Al-Muthana University, Samawah, Iraq

  61. UNSCEAR 2000 Report. United Nations Scientific Committee on the Effects of Atomic Radiation (2000) Sources and effects of ionizing radiation. Report to the General Assembly, with Scientific Annexes. New York, United Nations Sales Publications

  62. Karthik Kumar M, Nagaiah N, Mathews G, Ambika M (2018) Assessment of annual effective dose due to outdoor radon activity in the environment of Bengaluru. Radiat Prot Environ 41(3):115. https://doi.org/10.4103/rpe.rpe_40_18

    Article  Google Scholar 

  63. Gorchev HG, Ozolins G (2004) Guidelines for drinking-water quality, 3rd edition. Who 1:564

    Google Scholar 

  64. ICRP (2007) The 2007 Recommendations of the International Commission on Radiological Protection. ICRP Publication 103, Ann. ICRP 37:1–35

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Acknowledgements

The authors of this paper are sincerely grateful to the scientific and technical personnel of the Institute of Nuclear Minerals of the Bangladesh Atomic Energy Commission for the support during field work. Sincere acknowledgement goes to the local people and administration for their logistic help and cooperation in the field. Constructive suggestions of the anonymous reviewers are thankfully appreciated.

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Field supervision, investigation and review: [Ratan Kumar Majumder]; conceptualization, field investigation, map preparation and writing-original draft: [Sudeb Chandra Das]; funding acquisition and review: [Md. Golam Rasul]; field investigation: [Mohammad Ibrahim Khalil]; data curation: [Nafisa Tamannaya Dina]; methodology, data analysis and review: [Mohammad Zafrul Kabir, Farah Deeba]; review and editing: [Mohammad Rajib]. All authors have read and agreed to the published version of the manuscript.

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Correspondence to Sudeb Chandra Das.

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We confirm that this work is original and has not been published elsewhere nor it currently under consideration for publication elsewhere. All authors of this research paper have directly participated in the planning, execution, or analysis of this study. All authors have seen and approved the final version of the manuscript being submitted. To the best of our knowledge, no conflict of interest, financial or other, exists.

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Majumder, R.K., Das, S.C., Rasul, M.G. et al. Measurement of radon concentrations and their annual effective doses in soils and rocks of Jaintiapur and its adjacent areas, Sylhet, North-east Bangladesh. J Radioanal Nucl Chem 329, 265–277 (2021). https://doi.org/10.1007/s10967-021-07771-3

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