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Application of Mössbauer Spectroscopy to Li-Ion and Na-Ion Batteries

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Modern Mössbauer Spectroscopy

Part of the book series: Topics in Applied Physics ((TAP,volume 137))

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Abstract

Electrochemical energy storage is essential in everyday life and is crucial for energy transition requiring sustainable energy sources and clean transportation. Li-ion batteries are widely used due to their high energy density while other technologies are now emerging, as Na-ion batteries, to offer a variety of energy storage systems. The electrode materials are one of the key components that should be improved for better battery performance. This requires the investigation of the electrochemical reactions that take place within the batteries. Mössbauer spectroscopy is a powerful tool to probe the local environment at the atomic scale in electrode materials. This technique can be used for ex situ analyses or to follow in situ the electrochemical reactions. In this chapter, some general aspects of currently commercialized Li-ion batteries are briefly described to introduce electrode materials, electrochemical mechanisms and their characterizations. The basic concepts of the Mössbauer effect and hyperfine interactions are presented to define the Mössbauer parameters that provide information about structural, electronic and magnetic properties, with a special attention to in situ measurements. Then, some selected examples of insertion, alloying and conversion materials are considered to illustrate the application of 57Fe and 119Sn Mössbauer spectroscopies to elucidate reaction mechanisms in Li-ion and Na-ion batteries.

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Acknowledgements

The author is grateful to all collaborators and students who have contributed to the studies of Li-ion and Na-ion batteries, and in particular, J. C. Jumas, J. Olivier-Fourcade, M. T. Sougrati, M. Womes, L. Aldon, C. Bousquet, M. Chamas, J. Chouvin, R. Dedryvère, S. Difi, Y. He, M. El Khalifi, A. Mahmoud, M. Mouyane, S. Naille, A. Perea and F. Robert.

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  1. Institut Charles Gerhardt, UMR 5253 CNRS Université de Montpellier, Place Eugène Bataillon, 34095 Montpellier Cedex 5, France

    Pierre-Emmanuel Lippens

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Correspondence to Pierre-Emmanuel Lippens .

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  1. Shizuoka Institute of Science and Technology, Fukuroi, Shizuoka, Japan

    Yutaka Yoshida

  2. University of Leuven, Leuven, Belgium

    Guido Langouche

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Lippens, PE. (2021). Application of Mössbauer Spectroscopy to Li-Ion and Na-Ion Batteries. In: Yoshida, Y., Langouche, G. (eds) Modern Mössbauer Spectroscopy. Topics in Applied Physics, vol 137. Springer, Singapore. https://doi.org/10.1007/978-981-15-9422-9_7

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