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Synchrotron-Radiation-Based Energy-Domain Mössbauer Spectroscopy, Nuclear Resonant Inelastic Scattering, and Quasielastic Scattering Using Mössbauer Gamma Rays

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Modern Mössbauer Spectroscopy

Part of the book series: Topics in Applied Physics ((TAP,volume 137))

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Abstract

Nuclear resonant scattering spectroscopy using synchrotron radiation (SR) has been applied to a wide variety of scientific applications. An excellent feature of this method is that element (isotope)-specific information on the electronic and phonon states can be obtained using the energy selectivity of SR. The use of high-brilliance SR as an excitation source for Mössbauer spectroscopy allows imaging measurement under extreme conditions, such as high pressures, very high or low temperatures, and strong external magnetic fields. Additionally, diffusion and fluctuation of atoms can be observed by taking advantage of the ultranarrow width of the nuclear excited states. We introduced the concepts of the methods with an emphasis on these excellent features. Furthermore, the unique features involved in the measurements are highlighted and discussed.

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Abbreviations

SR:

Synchrotron radiation

NRIS:

Nuclear resonant inelastic scattering

NIS:

Nuclear inelastic scattering

NRIXS:

Nuclear resonant inelastic X-ray scattering

NRVS:

Nuclear resonant vibrational spectroscopy

PDOS:

Phonon density of states

DFT:

Density functional theory

RSMR:

Rayleigh scattering of Mössbauer radiation

TDI:

Time-domain interferometry

APD:

Avalanche photo diode

NFS:

Nuclear (resonant) forward scattering

SMS:

Synchrotron Mössbauer source

RI:

Radioisotope

FWHM:

Full width at half maximum

DAC:

Diamond anvil cell

QEGS:

Quasielastic γ-ray scattering

RC:

Radiative coupling

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Acknowledgements

The author is grateful to all collaborators and would like to thank all of the staff at the Institute for Integrated Radiation and Nuclear Science, Kyoto University, National Institutes for Quantum and Radiological Science and Technology, Japan Atomic Energy Agency, SPring-8, and the Photon factory of KEK for their support.

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Authors and Affiliations

  1. Institute for Integrated Radiation and Nuclear Science, Kyoto University, Kumatori-Cho, Sennan-Gun, Osaka, 590-0494, Japan

    Makoto Seto, Ryo Masuda & Makina Saito

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  1. Makoto Seto
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  2. Ryo Masuda
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  3. Makina Saito
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Correspondence to Makoto Seto .

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  1. Shizuoka Institute of Science and Technology, Fukuroi, Shizuoka, Japan

    Yutaka Yoshida

  2. University of Leuven, Leuven, Belgium

    Guido Langouche

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Seto, M., Masuda, R., Saito, M. (2021). Synchrotron-Radiation-Based Energy-Domain Mössbauer Spectroscopy, Nuclear Resonant Inelastic Scattering, and Quasielastic Scattering Using Mössbauer Gamma Rays. In: Yoshida, Y., Langouche, G. (eds) Modern Mössbauer Spectroscopy. Topics in Applied Physics, vol 137. Springer, Singapore. https://doi.org/10.1007/978-981-15-9422-9_2

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