Abstract
Experimental results of spin-dependent light scattering in 2D magnetically ordered systems are confronted with the theory of Suzuki and Kamimura.
The temperature dependence of the Raman integrated intensity of phonon bands which have become Raman active after magnetic ordering has occurred below the Néel temperature show the behaviour predicted by Suzuki and Kamimura’s theory on spin-dependent phonon Raman scattering. The macroscopic aspect of this theory predicts a temperature dependence of the integrated Raman intensity which is proportional to the nearest neighbor spin correlation function <S 0 . S 1>. This prediction is confirmed experimentally.
Insertion of lithium into 2D magnetically ordered intercalation compounds like FePS3 lowers the Néel temperature. This effect demands further theoretical attention.
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© 1992 Springer Science+Business Media Dordrecht
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Balkanski, M. (1992). Spin-Dependent Light Scattering in Two-Dimensional Magnetically Ordered Systems. In: Aoki, H., Tsukada, M., Schlüter, M., Lévy, F. (eds) New Horizons in Low-Dimensional Electron Systems. Physics and Chemistry of Materials with Low-Dimensional Structures, vol 13. Springer, Dordrecht. https://doi.org/10.1007/978-94-011-3190-2_5
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DOI: https://doi.org/10.1007/978-94-011-3190-2_5
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