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Infrared spectroscopy in supersonic free jets and molecular beams

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Jet Spectroscopy and Molecular Dynamics

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Abstract

In supersonic free jets and molecular beams [1], molecules at moderately high pressures (usually in the range 0.7 to 100 atmospheres) are expanded either neat or in a carrier through a small orifice (nozzle) or planar slit into a region of relatively lower pressure. The expansion cools the translational degrees of freedom of the gaseous mixture which creates a cold translational bath. This can significantly reduce the internal rotational and vibrational population distributions in molecular species of interest. As the expansion progresses the molecular, and thus collisional, density decreases. Subsequently, the rotationally and vibrationally cooled molecules enter an effectively collision-free region where they can be spectroscopically probed with a minimum of intermolecular interactions. This review is concerned with the application of infrared spectroscopic free jets to investigate cold isolated molecular species generated in such supersonic free jets or in molecular beams. For the purpose of this review, we shall define molecular beams as supersonic expansions in which an aperture or skimmer is used to restrict the velocity distribution and collimate the expanding gaseous mixture. If the molecular expansion is probed without such collimation, then it will be considered a supersonic free jet. We shall confine the infrared spectroscopic techniques considered to those which involve either absorption or emission of photons in the infrared spectral region.

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Authors
  1. J. Arnó
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  2. J. W. Bevan
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Editor information

Editors and Affiliations

  1. Department of Chemistry, University of Reading, UK

    J. M. Hollas

  2. Department of Chemistry Imperial College, University of London, UK

    D. Phillips

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© 1995 Springer Science+Business Media New York

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Arnó, J., Bevan, J.W. (1995). Infrared spectroscopy in supersonic free jets and molecular beams. In: Hollas, J.M., Phillips, D. (eds) Jet Spectroscopy and Molecular Dynamics. Springer, Dordrecht. https://doi.org/10.1007/978-94-011-1314-4_2

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  • DOI: https://doi.org/10.1007/978-94-011-1314-4_2

  • Publisher Name: Springer, Dordrecht

  • Print ISBN: 978-94-010-4573-5

  • Online ISBN: 978-94-011-1314-4

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