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Photon Statistics of a Single Photon Source

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Organic Nanophotonics

Part of the book series: NATO Science Series ((NAII,volume 100))

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Abstract

We report on the realization of a single photon source relying on the pulsed excitation of a single organic molecule at room temperature, and the study of its intensity fluctuations over 4 orders of magnitude of the observation time scale. On time scale of a few excitation periods, sub-poissonian statistics is clearly observed and the probability of multiphoton events is 10 times smaller than for equivalent Poissonian pulses. An excess of noise appears on longer timescale, due to the blinking produced by the molecular triplet state.

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References

  1. N. Gisin, G. Ribordy, W. Tittel, and H. Zbinden. Quantum cryptography. Rev. Mod. Phys., 74, 145, 2002.

    Article  ADS  Google Scholar 

  2. Serge Reynaud. Introduction à la réduction du bruit quantique. Ann. Phys. Fr., 15, 63, 1990.

    Article  ADS  Google Scholar 

  3. S. Brattke, B.T.H. Varcoe, and H. Walther. Generation of photon number states on demand via cavity quantum electrodynamics. Phys. Rev. Lett., 86, 3534, 2001.

    Article  ADS  Google Scholar 

  4. A. Kuhn, M. Hennrich, and G. Rempe. Deterministic single-photon source for distributed quantum networking. Phys. Rev. Lett, 89, 067901, 2002.

    Article  ADS  Google Scholar 

  5. J. Kim, O. Benson, H. Kan, and Y. Yamamoto. A single-photon turnstile device. Nature, 397, 500, 1999.

    Article  ADS  Google Scholar 

  6. P. Michler, A. Kiraz, C. Becher, W.V. Schoenfeld, P.M. Petroff, Lidong Shang, E. Hu, and A. Imamoglu. A quantum dot single-photon turnstile device. Science, 290, 2282, 2000.

    Article  ADS  Google Scholar 

  7. C. Santori, M. Pelt on, G. Solomon, Y. Dale, and Y. Yamamoto. Triggered single photons from a quantum dot. Phys. Rev. Lett., 86, 1502, 2001.

    Article  ADS  Google Scholar 

  8. E. Moreau, I. Robert, J.-M. Gérard, I. Abram, L. Manin, and V. Thierry-Mieg. Single-mode solid-state single photon source based on isolated quantum dots in pillar microcavities. Appl. Phys. Lett, 79, 2865, 2001.

    Article  ADS  Google Scholar 

  9. Z. Yuan, B. E. Kardynal, R.M. Stevenson, A.J. Shields, C.J. Lobo, K. Cooper, N.S. Beattie, D.A. Ritchie, and M. Pepper. Electrically driven single-photon source. Science, 295, 102, 2002.

    Article  ADS  Google Scholar 

  10. Ph. Tamarat, A. Maali, B. Lounis, and M. Orrit. Ten years of single molecule spectroscopy. J. Phys. Chem. A, 104, 1, 2000.

    Article  Google Scholar 

  11. C. Brunei, B. Lounis, P. Tamarat, and M. Orrit. Triggered source of single photons based on controlled single molecule fluorescence. Phys. Rev. Lett., 83, 2722, 1999.

    Article  ADS  Google Scholar 

  12. F. De Martini, G. Di Giuseppe, and M. Marrocco. Single—mode generation of quantum photon states by excited single molecules in a microcavity trap. Phys. Rev. Lett., 76, 900, 1996.

    Article  ADS  Google Scholar 

  13. R. Brouri, A. Beveratos, J.-P. Poizat, and P. Grangier. Single-photon generation by pulsed excitation of a single dipole. Phys. Rev. A, 62, 0638177, 2000.

    Article  Google Scholar 

  14. C. Kurtsiefer, S. Mayer, P. Zarda, and H. Weinfurter. Phys. Rev. Lett, 85, 290, 2000.

    Article  ADS  Google Scholar 

  15. R. Brouri, A. Beveratos, J.-Ph. Poizat, and Ph. Grangier. Photon antibunching in the fluorescence of individual colored centers in diamond. Opt Lett, 25, 1294, 2000.

    Article  Google Scholar 

  16. 16. B. Lounis and W. E. Moerner. Single photons on demand from a single molecule at room temperature. Nature, 407, 491, 2000.

    Google Scholar 

  17. L. Fleury, B. Sick, G. Zumofen, B. Hecht, and U. Wild. High photo-stability of single molecules in an organic crystal at room temperature observed by scanning confocal optical microscopy. Molecular Physics, 95, 1333, 1998.

    Article  ADS  Google Scholar 

  18. L. Fleury, J.-M. Segura, G. Zumofen, B. Hecht, and U. Wild. Nonclassical photon statistics in single-molecule fluorescence at room temperature. Phys. Rev. Lett., 84, 1148, 2000.

    Article  ADS  Google Scholar 

  19. F. Treussart, A. Clouqueur, C. Grossman, and J.-F. Roch. Photon antibunching in the fluorescence of a single dye molecule embedded in a thin polymer film. Opt Lett, 26, 1504, 2001.

    Article  ADS  Google Scholar 

  20. A. Beveratos, S. Kühn, R. Brouri, T. Gacoin, J.-P. Poizat, and P. Grangier. Room temperature stable single photon source. Eur. Phys. J. D, 18, 191, 2002.

    ADS  Google Scholar 

  21. S. Nie and R.N. Zare. Optical detection of single molecules. Annu. Rev. Biophys. Biomol. Struct, 26, 567, 1997.

    Article  Google Scholar 

  22. C. Kurtsiefer, P. Zarda, S. Mayer, and H. Weinfurter. Optical detection of single molecules. J. Mod. Opt, 48, 2039–2047, 2001.

    Article  ADS  Google Scholar 

  23. P. Grangier, G. Roger, and A. Aspect. Europhys. Lett, 1, 173, 1986.

    Article  ADS  Google Scholar 

  24. A. Beveratos, R. Brouri, T. Gacoin, A. Villing, J.-P. Poizat, and P. Grangier. Single photon quantum cryptography, to appear in Phys. Rev. Lett, 2002.

    Google Scholar 

  25. L. Mandel. Sub-poissonian photon statistics in resonance fluorescence. Opt. Lett., 4, 205, 1979.

    Article  ADS  Google Scholar 

  26. J.A. Abate, H.J. Kimble, and L. Mandel. Photon statistics of a dye laser. Phys. Rev. A, 14, 788, 1976.

    Article  ADS  Google Scholar 

  27. R. Short and L. Mandel. Observation of sub-poissonian photon statistics. Phys. Rev. Lett, 51, 384, 1983.

    Article  ADS  Google Scholar 

  28. F. Diedrich and H. Walther. Nonclassical radiation of single stored ion. Phys. Rev. Lett, 58, 203, 1987.

    Article  ADS  Google Scholar 

  29. J.A. Veerman, M.F. Garcia-Parajo, L. Kuipers, and N.F. Van Hulst. Time-varying triplet state lifetimes of single molecules. Phys. Rev. Lett., 83, 2155, 1999.

    Article  ADS  Google Scholar 

  30. H. Yang and X.S. Xie. Statistical approaches for probing single-molecule dynamics photon-by-photon, to appear in Chem. Phys., 2002.

    Google Scholar 

  31. V. Barsegov and S. Mukamel. Probing single molecule kinetics by photon arrival trajectories. J. Chem. Phys., 116, 9802, 2002.

    Article  ADS  Google Scholar 

  32. A. Berglund, A. Doherty, and H. Mabuchi. Photon statistics and dynamics of fluorescence resonance energy transfer. Phys. Rev. Lett., 89, 068101, 2002.

    Article  Google Scholar 

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© 2003 Springer Science+Business Media Dordrecht

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Treussart, F., Alléaume, R., Le Floc’h, V., Xiao, L.T., Roch, JF., Courty, JM. (2003). Photon Statistics of a Single Photon Source. In: Charra, F., Agranovich, V.M., Kajzar, F. (eds) Organic Nanophotonics. NATO Science Series, vol 100. Springer, Dordrecht. https://doi.org/10.1007/978-94-010-0103-8_35

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  • DOI: https://doi.org/10.1007/978-94-010-0103-8_35

  • Publisher Name: Springer, Dordrecht

  • Print ISBN: 978-1-4020-1280-8

  • Online ISBN: 978-94-010-0103-8

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