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Photoionization Dynamics of Small Molecules

  • Chapter
Photophysics and Photochemistry in the Vacuum Ultraviolet

Part of the book series: NATO ASI Series ((ASIC,volume 142))

Abstract

The last decade has witnessed remarkable progress in characterizing dynamical aspects of the molecular photoionization process. The general challenge is to gain physical insight into those processes occuring during photo excitation and eventual escape of the photoelectron through the anisotropic molecular field, in terms of various observables such as photoionization cross-sections and branching ratios, photoelectron angular distributions and even newer probes mentioned below. Much of the progress in this field has mirrored earlier work in atomic photoionization dynamics [1] where many key ideas were developed (e.g., channel interaction, quantum defect analysis, potential barrier phenomena and experimental techniques). However, additional concepts and techniques were required to deal with the strictly molecular aspects of the problem, particularly the anisotropy of the multicenter molecular field and the interaction among rovibronic modes.

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Authors and Affiliations

  1. Argonne National Laboratory, Argonne, IL, 60439, USA

    J. L. Dehmer

  2. Department of Chemistry, Boston University, Boston, MA, 02215, USA

    Dan Dill

  3. Synchrotron Ultraviolet Radiation Facility, National Bureau of Standards, Washington, D.C., 20234, USA

    A. C. Parr

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  1. J. L. Dehmer
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  1. Department of Chemistry, Louisiana State University, Baton Rouge, Louisiana, USA

    S. P. McGlynn

  2. Department of Chemistry, New York University, New York, NY, USA

    G. L. Findley

  3. Argonne National Laboratory, Argonne, Illinois, USA

    R. H. Huebner

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Dehmer, J.L., Dill, D., Parr, A.C. (1985). Photoionization Dynamics of Small Molecules. In: McGlynn, S.P., Findley, G.L., Huebner, R.H. (eds) Photophysics and Photochemistry in the Vacuum Ultraviolet. NATO ASI Series, vol 142. Springer, Dordrecht. https://doi.org/10.1007/978-94-009-5269-0_11

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