Skip to main content

Measurements of the Short-Term Variability of Aqueous-Phase Mass Concentrations in Cloud Droplets

  • Chapter
Acid Deposition at High Elevation Sites

Part of the book series: NATO ASI Series ((ASIC,volume 252))

Abstract

In-situ sampling of clouds with a droplet to aerosol converter allows determination of several important chemical and physical properties of cloud droplets over short spatial and temporal scales. During a measurement programme in July and August 1986 on the Swedish peak Areskutan (1250 m asl), the number concentration, water content, and aerosol light scattering coefficient of evaporated cloud droplets were determined in-situ. These measurements allow estimation of the mass concentration of non-volatile materials dissolved or suspended in the cloud droplets, the average size of the sampled cloud droplets, and the average size of the aerosol particles that result from evaporation of the sampled cloud droplets. The results illustrate the inhomogeneous character of clouds, with substantial variations of droplet number concentration, liquid water content, and residual aerosol light scattering coefficient over distances of less than 1 km. The observed, smaller variations in derived properties such as aqueousphase mass concentration and mean droplet radius may be due to entrainment of subsaturated air causing complete evaporation of some of the droplets.

This is a preview of subscription content, log in via an institution to check access.

Access this chapter

Chapter
USD 29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD 39.99
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
Softcover Book
USD 54.99
Price excludes VAT (USA)
  • Compact, lightweight edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Institutional subscriptions

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  • Armbruster, L., and Zebel, G. 1985. Theoretical and experimental studies for determining the aerosol sampling efficiency of annular slot probes. J. Aerosol Sci. 4, 335–341.

    Article  Google Scholar 

  • Baker, M.B., Breidenthal, R.E., Choularton, T. and Latham, J. 1984. The effects of turbulent mixing in clouds. J. Atmos. Sci. 41, 399–304.

    Article  Google Scholar 

  • Choularton, T.W., Consterdine, I.E., Gardiner, B.A., Gay, M.J., Hill, M.K., Latham, J. and Stromberg, I.M. 1986. Field studies of the optical and microphysical characteristics of clouds enveloping Great Dun Fell. J. R. Met. Soc. 112, 131–148.

    Article  Google Scholar 

  • Fuchs, N.A. 1964. The Mechanics of Aerosols. Pergamon Press, Oxford.

    Google Scholar 

  • Heintzenberg, J. and Backlin, L. 1983. A high sensitivity integrating nephelometer for airborne air pollution studies. Atmos. Environ. 17, 433–436.

    Article  Google Scholar 

  • Noone, K.J., Charlson, R.J., Covert, D.S., Ogren, J.A. and Heintzenberg, J. 1987a. Cloud droplets: solute concentration is size dependent. Submitted to J. Geophys. Res.

    Google Scholar 

  • Noone, K.J., Charlson, R.J., Covert, D.S., Ogren, J.A. and Heintzenberg, J. 1987b. Design and calibration of a counterflow virtual impactor for sampling of atmospheric fog and cloud droplets. Aerosol Sci. Tech., in press.

    Google Scholar 

  • Ogren, J.A., Heintzenberg, J. and Charlson, R.J. 1985. In-situ sampling of clouds with a droplet to aerosol converter. Geophys. Res, Lett. 12, 121–124.

    Article  Google Scholar 

  • Ogren, J.A. and Rodhe, H. 1986. Measurements of the chemical composition of cloudwater at a clean air site in citral Scandinavia. Tellus38B, 190–196.

    Article  Google Scholar 

  • Waggoner, A.P. et al. 1981. Optical characteristics of atmospheric aerosols. Atmos. Environ. 15, 1891–1909.

    Article  Google Scholar 

  • Warner, J. 1969. The microstructure of cumulus clouds. Part I. General features of the droplet spectrum. J. Atmos. Sci. 26, 1049–1059.

    Article  Google Scholar 

  • Whitby, K.T. 1978. Physical characteristics of sulphur aerosols. Atmos. Enviorn. 12, 135–159.

    Article  Google Scholar 

  • Zebel, G. 1978. Some problems in the sampling of aerosols. In Recent Developments in Aerosol Science (ed. D.T. Shaw), pp. 167–185. Wiley, New York.

    Google Scholar 

  • Zuber, A. and Witt, G. 1987. An optical hygrometer using differential absorption of the hydrogen Lyman alpha emission. Appi. Optics 26, 3083–3089.

    Article  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Editor information

Editors and Affiliations

Rights and permissions

Reprints and permissions

Copyright information

© 1988 Kluwer Academic publishers

About this chapter

Cite this chapter

Ogren, J.A. et al. (1988). Measurements of the Short-Term Variability of Aqueous-Phase Mass Concentrations in Cloud Droplets. In: Unsworth, M.H., Fowler, D. (eds) Acid Deposition at High Elevation Sites. NATO ASI Series, vol 252. Springer, Dordrecht. https://doi.org/10.1007/978-94-009-3079-7_6

Download citation

  • DOI: https://doi.org/10.1007/978-94-009-3079-7_6

  • Publisher Name: Springer, Dordrecht

  • Print ISBN: 978-94-010-7883-2

  • Online ISBN: 978-94-009-3079-7

  • eBook Packages: Springer Book Archive

Publish with us

Policies and ethics