Abstract
Since 1985, monitoring activities have been conducted in a network of 43 lakes comprising the Québec portion of the Long-Range Transport of Airborne Pollutants (LRTAP) program. The results to date indicate that Québec lakes generally are responding positively to the generalized decline in precipitation sulfate (SO 2−4 ), with 40 of the 43 lakes now showing steep declines in SO4 2− concentrations. The drop in SO 2−4 was associated with a significant decrease in Ca2+ concentrations in 77% of the lakes (67% for Mg2+ concentrations). overall, the acid-neutralizing capacity was increasing in 19 lakes and decreasing only in three, while 21 lakes showed no temporal trends. Compared with previous trend studies of the LRTAP-Québec network for the period of 1985–1993, the longer period (1985–1999) shows a clear improvement, with the proportion of lakes that were acidifying changing from 24 to 7% and with the proportion of lakes that were recovering changing from 16 to 35%. These observations suggest that the recent drop in SO 2−4 deposition in the northeastern U.S. and eastern Canada was significant enough to allow chemical recovery for a significant proportion of Québec lakes.
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References
Berryman, D., Bobée, B., Cluis, D. and Haemmerli, J.: 1988, ‘Nonparametric tests for trend detection in water quality time series’, Water Res. Bull. 24, 545–556.
Bobée, B., Lachance, M., Haemmerli, J., Tessier, A., Charrette, J. Y. and Kramer, J.: 1983, ‘Évaluation de la sensibilité à l’acidification des lacs du sud du Québec et incidences sur le réseau d’acquisition de données’, Report NO. 157, INRS-Eau, Sainte-Foy, Québec.
Bouchard, A.: 1997, ‘Recent lake acidification and recovery trends in southern Québec, Canada’, Water, Air, Soil Pollut. 94, 225–245.
Clair, T. A., Dillon, P. J., Ion, J., Jeffries, D. S., Papineau, M. and Vet, R. J.: 1995, ‘Regional precipitation and surface water chemistry trends in southeastern Canada (1983-1991)’, Can. J. Fish. Aquat. Sci. 52, 197–212.
Cluis, D., Langlois, C., van Coillie, R. and Laberge, C.: 1989, ‘Development of a software package for trend detection in temporal series: Application to water and industrial effluent quality data for the St. Lawrence River’, Environ. Monit. Assess. 12, 429–441.
Cronan, C. S.: 1979, Determination of sulfate in organically colored water samples’, Anal Chem. 51, 1333–1335.
Driscoll, C. T., Likens, G. E., Hedin, L. O., Eaton, J. S. and Bormann, F. H.: 1989, ‘Changes in the chemistry of surface waters’, Environ. Sci. Technol. 23, 137–142.
Driscoll, C. T., Postek, K. M., Kretser, W. and Raynal, D. J.: 1995, ‘Long-term trends in the chemistry of precipitation and lake water in the Adirondack region of New York, U.S.A.’, Water, Air, Soil Pollut. 85, 583–588.
Dupont, J.: 1997, ‘Projet Noranda Phase III-Effet des réductions d’émissions de So2 sur la qualité de l’eau des lacs de l’ouest québécois’, Envirodoq EN980066, Report NO. PA-53/1. Ministère de l’Environnement et de la Faune du Québec, Direction des écosystèmes aquatiques, Québec.
Environment Canada: 1994, Manual of Analytical Methods. Volume 2: Trace Metals. Canada Centre for Inland Waters, National Laboratory of Environmental Testing, Burlington, Ontario.
Galloway, J. N., Norton, S. A. and Church, M. R.: 1983, ‘Freshwater acidification from atmospheric deposition of sulfuric acid: A conceptual model’, Environ. Sci. Technol. 17, 541–545.
Hedin, L. O., Granat, L., Likens, G. E., Buishand, T. A., Galloway, J. N., Butler, T. J. and Rodhe, H.: 1994, ‘Steep declines in atmospheric base cations in regions of Europe and North America’, Nature 367, 351–354.
Hirsch, R. M. and Slack, J. M.: 1984, ‘A nonparametric trend test for seasonal data with serial dependence’, Water Resour. Res. 20, 727–732.
Houle, D. and Carignan, R.: 1995, ‘Role of So4 2- adsorption and desorption in the long term S budget of a coniferous catchment on the Canadian Shield’, Biogeochemistry 28, 161–182.
Houle, D., Paquin, R., Camiré, Ouimet, C. R. and Duchesne, L.: 1997, ‘Response of the Lake Clair watershed (Duchesnay, Québec) to changes in precipitation chemistry (1988-1994)’, Can. J. For. Res. 27, 1813–1821.
Jeffries, D. S., Lam, D. C. L., Wong, I. and Moran, M. D.: 2000, ‘Assessment of changes in lake pH in southeastern Canada arising from present levels and expected reductions in acidic deposition’, Can. J. Fish. Aquat. Sci. 57(suppl. 2), 40–49.
Kemp, A.: 1999, ‘Trends in lake water quality in southern Québec following reductions in sulphur emissions’, Scientific and Technical Report STE-212. Environment Canada-Québec Region, Environmental Conservation, St. Lawrence Centre, Montreal, Québec.
Lawrence, G. B., David, M. B., Bailey, S. W. and Shortle, W. C.: 1997, ‘Assessment of soil calcium status in red spruce forests in the northeastern United States’, Biogeochemistry 38, 19–39.
Likens, G. E., Driscoll, C. T. and Buso, D. C.: 1996, ‘Long-term effects of acid rain: Response and recovery of a forest ecosystem’, Science 272, 244–246.
Likens, G. E., Driscoll, C. T., Buso, D. C., Siccama, T. G., Johnson, C. E., Lovett, G. M., Fahey, T. J., Reiners, W A., Ryan, D. F., Martin, C. W and Bailey, S. W.: 1998, ‘The biogeochemistry of calcium at Hubbard Brook’, Biogeochemistry 41, 89–173.
Mallory, M. L., McNicol, D. K., Cluis, D. A. and Laberge, C.: 1998, ‘Chemical trends and status of small lakes near Sudbury ontario, 1983-1995: Evidence of continued chemical recovery’, Can. J. Fish. Aquat. Sci. 55, 63–75.
Mitchell, M. J., Raynal, D. J. and Driscoll, C. T.: 1995, ‘Biogeochemistry of a forested watershed in the central Adirondack Mountains: Temporal changes and mass balances’, Water, Air, Soil Pollut. 88, 355–369.
Molot, L. A. and Dillon, P. J.: 1997, ‘Colour mass balances and colour-dissolved organic carbon relationships in lakes and streams in central ontario’, Can. J. Fish. Aquat. Sci. 54, 2789–2795.
Stainton, M. P., Capel, M. J. and Armstrong, F. A. J.: 1974, ‘The Chemical Analysis of Freshwater’, Fisheries Research Board of Canada, Miscellaneous Special Publication 25.
Stoddard, J. L., Driscoll, C. T., Kahl, J. S. and Kellogg, J. P.: 1998, ‘A regional analysis of lake acidification trends for the Northeastern U.S., 1982-1994’, Environ. Monit. Assess. 51, 399–413.
Stoddard, J. L., Jeffries, D. S., Lukewille, A., Clair, T. A., Dillon, P. J., Driscoll, C. T., Forsius, M., Johannessen, M., Kahl, J. S. Kellogg, J. H., Kemp, A., Mannio, J., Monteith, D. T., Murdoch, P. S., Patrick, S., Rebsdorf, A., Skjelkvale, B. L., Stainton, M. P., Traaen, T., van Dam, H., Webster, K. E., Wieting, J. and Wilander, A.: 1999, ‘Regional trends in aquatic recovery from acidification in North America and Europe’, Nature 401, 575–578.
Vet, R. J., Sukloff, W B., Still, M. E., McNair, C. S., Martin, J. B., Kobelka, W. F. and Gaudenzi, A. J.: 1989, ‘Canadian Air and Precipitation Monitoring Network (CAPMoN): Precipitation Data Summary-1987’, Environment Canada, Atmospheric Environment Service, Air Quality and Interenvironmental Research Branch, Measurements and Analysis Research Division, Downsview, Ontario.
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Houle, D., Gagnon, C., Couture, S., Kemp, A. (2004). Recent Recovery of Lake Water Quality in Southern Québec following Reductions in Sulfur Emissions. In: Wieder, R.K., Novák, M., Vile, M.A. (eds) Biogeochemical Investigations of Terrestrial, Freshwater, and Wetland Ecosystems across the Globe. Springer, Dordrecht. https://doi.org/10.1007/978-94-007-0952-2_18
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