Abstract
Isotope effects are small and separation of mixtures of isotopes is correspondingly difficult. The theory of isotope separation is reviewed and necessary terminology introduced. Practical methods of isotope separation are discussed focusing on the fundamentals of multistage processes and cascade design. We discuss the use of distillation, chemical exchange, gaseous diffusion, thermal diffusion, centrifugation, electromagnetic fields, and laser processes for the separation of isotopes from natural abundance feeds. Numerous examples are treated.
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Further Reading
Avery, D. G., Davies, E., 1973 Uranium Enrichment by Gas Centrifuge (London, Mills & Boon, Ltd.)
Benedict, M., Pigford, M., Levi, H. W., 1981 Nuclear Chemical Engineering, 2nd Ed. (New York, McGraw-Hill)
Cohen, K., 1951 The Theory of Isotope Separation (New York, McGraw-Hill)
Ishida, T., Fujii, Y. 2006 Enrichment of Isotopes in Kohen, A., Limbach, H. H. Isotope effects in Chemistry and Biology (Boca Raton, FL, CRC Press, Taylor & Francis)
Kistemaker, J., Bigeleisen, J., Nier, A. O. C., Eds. 1958 Proceedings of the International Symposium on Isotope Separation (Amsterdam, North-Holland)
Klein, E. R., Klein, P. L. Eds. 1979 Proceedings of the 3rd International Conference on Stable Isotopes (New York, Academic) p. 175
London, H., 1961 Separation of Isotopes (London, George Newnes)
Rae, H. K., Ed., 1978. Separation of Hydrogen Isotopes, ACS Symposium Series 68 (Washington, DC, American Chemical Society)
Spindel, W. 1969 Isotope Effects in Chemical Processes, Advances in Chemistry Series 89 (Washington, DC, American Chemical Society)
Spindel, W., Ishida, T.,1990 Isotope Separation, in Lerner, R. G., Trigg, G. L., Eds. Encyclopedia of Physics (New York, VCH Publishers) 2nd Ed.
Van Hook, W. A. 2004 Isotope Separation, in Vertes, A., Nagy, S., Klencsar, Z., Eds. Volume 5, p. 177, Handbook of Isotope Chemistry (Dordrecht, Kluwer)
Villani, S., 1979 Uranium Separation (Berlin, Springer-Verlag)
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Wolfsberg, M., Van Hook, W.A., Paneth, P. (2009). Isotope Separation. In: Isotope Effects. Springer, Dordrecht. https://doi.org/10.1007/978-90-481-2265-3_8
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DOI: https://doi.org/10.1007/978-90-481-2265-3_8
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