Abstract
As is well-known, repulsive excited states may lead to desorption only if their life-time is long enough to allow for the desorbing particle to escape from the FRANCK-CONDON region. States with two localized holes are good examples of long-lived excited states. Recent work has shown |1| that electron correlations in the ground state are vital to bring these two-hole states into the picture. These states have been very useful in providing an explicit mechanism for desorption which complements, rather than contradicts, the MGR model |2|.
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Rubio, J., López Sancho, J.M., Refolio, M.C., López Sancho, M.P. (1985). Scattering Approach to Two-Hole Final States. In: Brenig, W., Menzel, D. (eds) Desorption Induced by Electronic Transitions DIET II. Springer Series in Surface Sciences, vol 4. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-82547-7_5
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DOI: https://doi.org/10.1007/978-3-642-82547-7_5
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