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Quantum-Resolved Angular Distributions of Neutral Products in Electron-Stimulated Surface Processes

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Desorption Induced by Electronic Transitions DIET V

Part of the book series: Springer Series in Surface Sciences ((SSSUR,volume 31))

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Abstract

Two-dimensional imaging of laser resonance-enhanced multiphoton ionization (REMPI) is used to obtain angular distributions of neutral molecules which are products of electron stimulated desorption (ESD) and dissociation processes on adsorbatecovered surfaces. Quantum resolution allows the angular distributions to be state-specific. We briefly discuss angular distributions for ESD of metastable CO*(a3Πr,ν=0) and ground-state NO from Pt(111); in addition, we discuss distributions for the NO product of NO2 dissociation on clean and O-covered Pt(111). The results are discussed in terms of desorption mechanisms, dissociative forces, site geometries, and disordered coadsorbate layers.

Supported by the U.S. Department of Energy under Contract # DE-AC04-76DP00189.

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References

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Author information

Authors and Affiliations

  1. Department 1114, Sandia National Laboratories, Albuquerque, NM, 87185, USA

    A. R. Burns, E. B. Stechel & D. R. Jennison

Authors
  1. A. R. Burns
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  2. E. B. Stechel
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  3. D. R. Jennison
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Editor information

Editors and Affiliations

  1. Sandia National Laboratories, Albuquerque, P.O. Box 5800, Albuquerque, NM, 87185, USA

    Alan R. Burns , Ellen B. Stechel  & Dwight R. Jennison ,  & 

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© 1993 Springer-Verlag Berlin Heidelberg

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Burns, A.R., Stechel, E.B., Jennison, D.R. (1993). Quantum-Resolved Angular Distributions of Neutral Products in Electron-Stimulated Surface Processes. In: Burns, A.R., Stechel, E.B., Jennison, D.R. (eds) Desorption Induced by Electronic Transitions DIET V. Springer Series in Surface Sciences, vol 31. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-78080-6_27

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  • DOI: https://doi.org/10.1007/978-3-642-78080-6_27

  • Publisher Name: Springer, Berlin, Heidelberg

  • Print ISBN: 978-3-642-78082-0

  • Online ISBN: 978-3-642-78080-6

  • eBook Packages: Springer Book Archive

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