Abstract
Some results on the classical mechanics of anharmonic vibrations in several-dimensional systems are summarized, and their relation to unimolecular reaction rate theory and to infrared multiphoton dissociation of molecules is discussed. Quantum connections are considered using semiclassical theory.
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Marcus, R.A., Noid, D.W., Koszykowski, M.L. (1978). Energy Redistribution in Molecules in the Quasi-Periodic and Ergodic Regimes. In: Zewail, A.H. (eds) Advances in Laser Chemistry. Springer Series in Chemical Physics, vol 3. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-67054-1_29
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DOI: https://doi.org/10.1007/978-3-642-67054-1_29
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