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Quantitative modeling of ultrafast energy transfer dynamics in the photosynthetic apparatus

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Ultrafast Phenomena XII

Part of the book series: Springer Series in Chemical Physics ((CHEMICAL,volume 66))

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Abstract

The dynamics of energy transfer processes in photosynthetic reaction centers and the light harvesting antenna LH2 are elucidated quantitatively using a new prescription for applying Forster theory to complex molecular aggregates. We conclude that the design of highly efficient light harvesting antenna systems generally cannot be predicted by pairwise Förster theory.

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References

  1. Th. Förster Zwischenmolekulare Energiewanderung und Fluoreszenz,″ Ann. Phys. 6, 55–75 (1948).

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  2. G. D. Scholes and G. R. Fleming, ″On the mechanism of light-harvesting in photosynthetic purple bacteria: B800 to B850 energy transfer,″ J. Phys. Chem. 104, 1854–1868 (2000).

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  3. R. J. Stanley, B. King, and S. G. Boxer, “Excited state energy transfer pathways in photosynthetic reaction centers.2. Heterodimer special pair,” J. Phys. Chem. 100, 12052–12059 (1996).

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  4. J. M. Jean, C. -K. Chan, and G. R. Fleming, “Electronic Energy Transfer in Photosynthetic Bacterial Reaction Centers,” Isr. J.Chem. 28, 169–175 (1988).

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© 2001 Springer-Verlag Berlin Heidelberg

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Jordanides, X.J., Scholes, G.D., Fleming, G.R. (2001). Quantitative modeling of ultrafast energy transfer dynamics in the photosynthetic apparatus. In: Ultrafast Phenomena XII. Springer Series in Chemical Physics, vol 66. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-642-56546-5_200

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  • DOI: https://doi.org/10.1007/978-3-642-56546-5_200

  • Publisher Name: Springer, Berlin, Heidelberg

  • Print ISBN: 978-3-642-62512-1

  • Online ISBN: 978-3-642-56546-5

  • eBook Packages: Springer Book Archive

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