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One Is Not Enough: Intra-Cavity Spectroscopy with Multi-Mode Lasers

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Lasers, Spectroscopy and New Ideas

Part of the book series: Springer Series in Optical Sciences ((SSOS,volume 54))

Abstract

When the laser was discovered more than 25 years ago as the ultimate outgrowth of spectroscopic work, it kept the physics community busy for more than a decade observing, surveying, and classifying all those surprising features of the new type of light and its interactions with matter. The early lasers, lacking technical sophistication, usually oscillated in a vast multitude of radiative modes. These systems were considered overly complex, and accordingly theoretical models and explanations were constructed for ideal single-mode lasers, which, however, barely could be demonstrated in experiments. It is perhaps not so surprising that it took ten years before emission spectra of a real multi-mode laser were subjected to detailed inspection. A close look revealed that the light flux of individual modes in their broad spectral comb did not vary smoothly — as was anticipated — across the full emission band. Instead, crests and crevices, rifts and ridges showed up in the recorded spectra. Soon these observed features were traced to either very weak absorption of matter or spurious interference inside the laser resonator [1]. This interpretation suggested that this ultra-sensitive response to weak extinction could be used for a novel spectroscopic technique.

1986–87 JILA Visiting Fellow. On leave from 1. Institut für Experimentalphysik, Universität Hamburg, D-2 Hamburg 36, F. R. Germany.

On leave from Lebedev Physical Institute, Academy of Sciences of the USSR, Moscow, USSR.

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References

  1. L. A. Pakhomycheva, E. A. Sviridenkov, A. F. Suchkov, L. V. Titova, and S. S. Churilov, ZhETP Pisma Red. 12, 60 (1970)

    ADS  Google Scholar 

  2. L. A. Pakhomycheva, E. A. Sviridenkov, A. F. Suchkov, L. V. Titova, and S. S. Churilov[JETP Lett. 12, 43 (1970)].

    ADS  Google Scholar 

  3. T. P. Belikova, E. A. Sviridenkov, and A. F. Suchkov, Opt. Spektrosk. 37, 654 (1974)

    Google Scholar 

  4. T. P. Belikova, E. A. Sviridenkov, and A. F. Suchkov,[Opt. Spectrosc. 37 372 (1974)].

    Google Scholar 

  5. G. Herzberg, Molecular Spectra and Molecular Structure (Van Nostrand, New York, 1960), p. 427.

    Google Scholar 

  6. N. C. Peterson, M. J. Kurylo, W. Braun, A. M. Bass, and R. A. Keller, J.O.S.A. 61, 746 (1971).

    Article  Google Scholar 

  7. R. J. Thrash, H. von Weyssenhof, and T. S. Shirk, J. Chem. Phys. 55, 4559 (1971).

    Article  Google Scholar 

  8. T. W. Hansen, A. L. Schawlow, and P. E. Toschek, J. Quant. Electron. QE-8, 802 (1972).

    Article  ADS  Google Scholar 

  9. Yu. M. Ajvasjan, V. M. Baev, V. V. Ivanov, S. A. Kovalenko, and E. A. Sviridenkov, Kvantovaja Elektron. 14, No. 2 (1987).

    Google Scholar 

  10. H. Atmanspacher, H., Scheingraber, and V. M. Baev, Phys. Rev. A 35, 142 (1987).

    Article  ADS  Google Scholar 

  11. V. M. Baev, T. P. Belikova, E. A. Sviridenkov, and A. F. Suchkov, Zh. Eksp. Teor. Fiz. M., 43 (1978)

    Google Scholar 

  12. V. M. Baev, T. P. Belikova, E. A. Sviridenkov, and A. F. Suchkov,[Sov. Phys.-JETP 74, 21 (1978)].

    ADS  Google Scholar 

  13. V. M. Baev, T. P. Belikova, S. A. Kovalenko, E. A. Sviridenkov, and A. F. Suchkov, Kvantovaja Elektron. 7, 903 (1980)

    Google Scholar 

  14. V. M. Baev, T. P. Belikova, S. A. Kovalenko, E. A. Sviridenkov, and A. F. Suchkov,[Sov. J. Quantum Electron. 10, 517 (1980)].

    Article  ADS  Google Scholar 

  15. E. N. Antonov, V. G. Koloshnikov, and V. R. Mironenko, Opt. Comm. 15, 99 (1975).

    Article  ADS  Google Scholar 

  16. F. Stoeckel, M. A. Melieres, and M. Chenevier, J. Chem. Phys. 76, 2191 (1982).

    Article  ADS  Google Scholar 

  17. T. P. Belikova, B. K. Dorofeev, E. A. Sviridenkov, and A. F. Suchkov, Kvantovaja Elektron. 2, 1325 (1975)

    ADS  Google Scholar 

  18. T. P. Belikova, B. K. Dorofeev, E. A. Sviridenkov, and A. F. Suchkov,[Sov. J. Quantum Electron. 5, 722 (1975)].

    Article  ADS  Google Scholar 

  19. N. A. Raspopov, A. N. Savchenko, and E. A. Sviridenkov, Kvantovaja Elektron. 4, 736 (1977)

    ADS  Google Scholar 

  20. N. A. Raspopov, A. N. Savchenko, and E. A. Sviridenkov,[Sov. J. Quantum Electron. 7, 409 (1977)].

    Article  ADS  Google Scholar 

  21. S. A. Kovalenko, Kvantovaja Elektron. 8, 1271 (1981)

    ADS  Google Scholar 

  22. S. A. Kovalenko,[Sov. J. Quantum Electron. 11, 759 (1981)].

    Article  ADS  Google Scholar 

  23. V. R. Mironenko and V. J. Yudson, Opt. Comm. 34, 397 (1980).

    Article  ADS  Google Scholar 

  24. V. M. Baev, G. Gaida, H. Schroder, and P. E. Toschek, Opt. Comm. 38 309 (1981).

    Article  ADS  Google Scholar 

  25. S. J. Harris, J. Chem. Phys. 71, 4001 (1979).

    Article  ADS  Google Scholar 

  26. E. N. Antonov, A. A. Kachanov, V. R. Mironenko, and T. V. Plakhotnik, Opt. Comm. 46, 126 (1983).

    Article  ADS  Google Scholar 

  27. S. J. Harris, Appl. Opt. 23, 1311 (1984).

    Article  ADS  Google Scholar 

  28. H. Atmanspacher, H. Scheingraber, and C. R. Vidal, Phys. Rev. A 32, 254 (1985).

    Article  ADS  Google Scholar 

  29. H. Atmanspacher, H. Scheingraber, and C. R. Vidal, Phys. Rev. A 33, 1052 (1986).

    Article  ADS  Google Scholar 

  30. F. Stoeckel, G. H. Atkinson, Appl. Opt. 29, 3591 (1985).

    Article  ADS  Google Scholar 

  31. Yu. M. Ajvasjan, V. M. Baev, A. A. Kachanov, and S. A. Kovalenko, Kvantovaja Elektron. 13, 1723 (1986).

    Google Scholar 

  32. Yu. M. Ajvasjan, V. M. Baev, T. P. Belikova, S. A. Kovalenko, E. A. Sviridenkov, and O. I. Yushchuk, Kvantovaja Elektron. 13 612 (1986)

    Google Scholar 

  33. Yu. M. Ajvasjan, V. M. Baev, T. P. Belikova, S. A. Kovalenko, E. A. Sviridenkov, and O. I. Yushchuk,[Sov. J. Quantum Electron. 16, 397 (1986)].

    Article  ADS  Google Scholar 

  34. V. R. Mironenko, Kvantovaja Elektron. 7, 2069 (1980).

    Google Scholar 

  35. W. Brunner and H. Paul, Opt. Quantum Electron. 12, 393 (1980).

    Article  Google Scholar 

  36. V. M. Baev, T. P. Belikova, M. B. Ippolitov, E. A. Sviridenkov, and A. F. Suchkov, Opt. Spektrosk. 45, 58 (1978)

    ADS  Google Scholar 

  37. V. M. Baev, T. P. Belikova, M. B. Ippolitov, E. A. Sviridenkov, and A. F. Suchkov,[Opt. Spectrosc. 45, 31 (1978)].

    ADS  Google Scholar 

  38. A. A. Kachanov and T. V. Plakhotnik, Opt. Comm. 47, 257 (1983).

    Article  ADS  Google Scholar 

  39. Y. H. Meyer and M. N. Nenchev, Opt. Comm. 41, 292 (1982).

    Article  ADS  Google Scholar 

  40. V. M. Baev, T. P. Belikova, O. P. Varnavskij , V. F. Gamalij, S. A. Kovalenko, and E. A. Sviridenkov, ZhETP Pisma Red. 42, 416 (1985)

    ADS  Google Scholar 

  41. V. M. Baev, T. P. Belikova, O. P. Varnavskij , V. F. Gamalij, S. A. Kovalenko, and E. A. Sviridenkov,[JETP Lett. 42, 514 (1985)].

    ADS  Google Scholar 

  42. T. S. Zeilikovich, S. A. Pulkin and L. S. Gaida, Zh. Eksp. Teor. Fiz. 87, 125 (1984)

    Google Scholar 

  43. T. S. Zeilikovich, S. A. Pulkin and L. S. Gaida,[Sov. Phys.-JETP 60, 72 (1984)].

    Google Scholar 

  44. W. T. Hill III, T. W. Hänsch, and A. L. Schawlow, Appl. Opt. 24, 3718 (1985).

    Article  ADS  Google Scholar 

  45. V. S. Egorov and I. A. Chekhonin, Opt. Spektrosk. 52, 591 (1982)

    Google Scholar 

  46. V. S. Egorov and I. A. Chekhonin,[Opt. Spectrosc. 52, 355 (1982)].

    ADS  Google Scholar 

  47. M. Chenevier, M. A. Melieres, and F. Stoeckel, Opt. Comm. 45, 385 (1983).

    Article  ADS  Google Scholar 

  48. W. T. Hill, R. A. Abreu, T. W. Hänsen, and A. L. Schawlow, Opt. Comm. 32, 96 (1980).

    Article  ADS  Google Scholar 

  49. H. Schroder, K. Schultz, and P. E. Toschek, Opt. Comm. 60, 159 (1986).

    Article  ADS  Google Scholar 

  50. Ya. I. Khanin, A. G. Kagan, V. P. Novikov, M. A. Novikov, I. N. Polushkin, and A. I. Shcherbakov, Opt. Comm. 32 456 (1980).

    Article  ADS  Google Scholar 

  51. Y. H. Meyer, Opt. Comm. 30, 75 (1979).

    Article  ADS  Google Scholar 

  52. A. N. Rubinov, M. V. Belobon, and A. V. Adamushko, Kvantovaja Elektron. 6, 723 (1979)

    ADS  Google Scholar 

  53. A. N. Rubinov, M. V. Belobon, and A. V. Adamushko,[Sov. J. Quantum Electron. 9, 433 (1979)].

    Article  ADS  Google Scholar 

  54. V. M. Baev, V. F. Gamalij, E. A. Sviridenkov, and D. D. Toptygin, Kratk. Soob. po Fiz. No. 8, 6 (1986) [Sov. Phys. Lebedev Institute Report].

    Google Scholar 

  55. W. Neuhauser and P. E. Toschek, Opt. Comm. 11, 331 (1974).

    Article  ADS  Google Scholar 

  56. S. Haroche and F. Hartmann, Phys. Rev. A 6, 1280 (1972).

    Article  ADS  Google Scholar 

  57. M. Sargent III and P. E. Toschek, Appl. Phys. 11 107 (1976).

    Article  ADS  Google Scholar 

  58. B. Stahlberg, V. M. Baev, G. Gaida, H. Schröder, and P. E. Toschek, J. Chem. Soc. Faraday Trans. 81, 207 (1985).

    Article  Google Scholar 

  59. V. M. Baev, S. A. Kovalenko, E. A. Sviridenkov, A. F. Suchkov, and D. D. Toptygin, Kvantovaja Elektron. 7, 1112 (1980)

    Google Scholar 

  60. V. M. Baev, S. A. Kovalenko, E. A. Sviridenkov, A. F. Suchkov, and D. D. Toptygin, [Sov. J. Quantum Electron. 10, 638 (1980)].

    Article  ADS  Google Scholar 

  61. J. P. Reilly and J. H. Clark, Proc. Int. Conf. on Advances in Laser Chemistry, California Institute of Technology, Pasadena, Calif., 1978, ed. by A. W. Zewail (Springer-Verlag, Berlin, 1978), p. 355.

    Book  Google Scholar 

  62. V. M. Baev, T. P. Belikova, V. F. Gamalij, E. A. Sviridenkov, and A. F. Suchkov, Kvantovaja Elektron. 11, 2413 (1984)

    Google Scholar 

  63. V. M. Baev, T. P. Belikova, V. F. Gamalij, E. A. Sviridenkov, and A. F. Suchkov, [Sov. J. Quantum Electron. 14, 1596 (1984)].

    Article  ADS  Google Scholar 

  64. V. M. Baev, V. F. Gamalij, E. A. Sviridenkov, and D. D. Toptygin, Kratk. Soob. po Fiz. No. 8, 3 (1986) [Sov. Phys. Lebedev Institute Report].

    Google Scholar 

  65. J. E. Bjorkholm and P. F. Liao, Phys. Rev. Lett. 33, 128 (1974).

    Article  ADS  Google Scholar 

  66. K. Boller, V. M. Baev, and P. E. Toschek, Opt. Comm., in press.

    Google Scholar 

  67. V. M. Baev, H. Schroder, and P. E. Toschek, Opt. Comm. 36, 57 (1981).

    Article  ADS  Google Scholar 

  68. V. M. Baev, K.-J. Boller, A. Weiler, and P. E. Toschek, Opt. Comm., in press.

    Google Scholar 

  69. D. M. Sarkisov, E. A. Sviridenkov, and A. F. Suchkov, Chimicheskaya Fizika 9, 1155 (1982).

    Google Scholar 

  70. F. Stoeckel, M. Schuh, N. Goldstein, and G. H. Atkinson, Chem. Phys. 95, 135 (1985).

    Article  ADS  Google Scholar 

  71. A. L. Schawlow and C. H. Townes, Phys. Rev. 112, 1940 (1958).

    Article  ADS  Google Scholar 

  72. J. L. Hall, private communication.

    Google Scholar 

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Toschek, P.E., Baev, V.M. (1987). One Is Not Enough: Intra-Cavity Spectroscopy with Multi-Mode Lasers. In: Yen, W.M., Levenson, M.D. (eds) Lasers, Spectroscopy and New Ideas. Springer Series in Optical Sciences, vol 54. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-47872-0_5

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  • DOI: https://doi.org/10.1007/978-3-540-47872-0_5

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