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Dynamics of Glassy, Crystalline and Liquid Ionic Conductors pp 89–250Cite as

Electrical Response of Ionic Conductors

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Part of the book series: Topics in Applied Physics ((TAP,volume 132))

Abstract

In spite of the vast amount of studies devoted during the past decades to understanding the dynamics of ions in ionically conducting materials, it is still unsettled to remain an open and challenging problem [1–4]. Since the charge transport in these materials is mainly due to the mobile ions, the measurement, analysis, and theoretical interpretation of their response to an applied electric field constitute the method as well as the key to gain insights into the dynamics of the mobile ions [1–6], which ultimately determines the conductivity. Most remarkable is the fact that, overall, the electrical response in all molten, glassy, liquid, or even crystalline ionically conducting materials, shows similar properties and universal features [3, 7, 8]. Though at the present time there is not a generally accepted theory for the description of the microscopic motion of ions, it is generally agreed that a disordered structure and Coulomb interactions among ions play an essential role in determining the dynamics of mobile ions and its complex properties and behaviour [1, 9–11]. Note that even in the case of crystalline ionic conductors the mobile ions experience a disordered potential landscape since there are significantly fewer ions than available sites with similar energies for them to occupy, and the mobile ions are usually randomly distributed in the structure, like in an ionic glass or molten salt [1]. This is true at least for fast ionic conductors with a high density of mobile ions and vacant available unoccupied sites.

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Authors and Affiliations

  1. Tokyo Institute of Technology, Yokohama, Kanagawa, Japan

    Junko Habasaki

  2. Facultad de Fisica, Universidad Complutense Madrid, Madrid, Spain

    Carlos León

  3. IPCF, CNR, Pisa, Italy

    K. L. Ngai

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Habasaki, J., León, C., Ngai, K.L. (2017). Electrical Response of Ionic Conductors. In: Dynamics of Glassy, Crystalline and Liquid Ionic Conductors. Topics in Applied Physics, vol 132. Springer, Cham. https://doi.org/10.1007/978-3-319-42391-3_4

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