Abstract
It is presented a consistent relativistic approach to calculation of the energy, spectroscopic, radiation decay (excitation, ionization) characteristics of the Rydberg atomic systems in a Black-body radiation field. The approach is based on an advanced relativistic energy approach (in a single-electron approximation realization) and formalism of the relativistic many-body perturbation theory with the zeroth density functional approximation. The key features of the approach are connected with an accurate treatment of the complex exchange-correlation effects (interelectron polarization interaction through the Fermi sea, continuum pressure, the non-Coulomb grouping of levels in the heavy Rydberg spectra and others) and application of the optimized bases of relativistic wave functions, and correspondingly, fulfilling the principle of gauge invariance in calculation of the radiative decay characteristics. As illustration, we present the results of calculation of the spectroscopic characteristics (ionization rate, effective lifetime values etc.) for sodium Rydberg atoms in a Black-body radiation field for different states and temperatures. The obtained spectroscopic data are compared with available experimental and alternative theoretical results.
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Acknowledgements
The authors are grateful to the Chair of QSCP-XXIII, Prof. Liliana Mammino, and the Cochair Prof. Jean Maruani, for their generous invitation to present this work in the Proceedings of the XXIII International workshop on Quantum Systems in Chemistry, Physics and Biology.
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Glushkov, A.V., Ternovsky, V.B., Kuznetsova, A.A., Tsudik, A.V. (2020). Spectroscopy of Rydberg Atomic Systems in a Black-Body Radiation Field. In: Mammino, L., Ceresoli, D., Maruani, J., Brändas, E. (eds) Advances in Quantum Systems in Chemistry, Physics, and Biology. QSCP 2018. Progress in Theoretical Chemistry and Physics, vol 32. Springer, Cham. https://doi.org/10.1007/978-3-030-34941-7_3
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