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Role of the Surface Chemistry of Adsorbents and Nature of Molecular Interactions

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Gas-Adsorption Chromatography

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Abstract

The effects of geometrical inhomogeneity in the surfaces and pores may be largely avoided by using crystalline adsorbents, and also amorphous ones with large pores with surfaces modified either chemically or by adsorption. The surface chemistry of the adsorbent will then largely control the adsorption and selectivity of the gas-adsorption column. The surface chemistry determines the nature and energy of the interactions with the adsorbate. Interaction with a homogeneous surface and the state of adsorbed molecules on such a surface (gas-adsorption chromatography) allow more readily of theoretical treatment than do the interactions on a solution in a liquid film (gas-liquid chromatography). All the molecules in a solution are mobile and so interact with fluctuating centers, whereas the molecules adsorbed on a reasonably smooth solid surface interact mainly with the nearest force centers, which are fixed.

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Authors and Affiliations

  1. Department of Chemistry, Moscow University, Russia

    Andrei V. Kiselev

  2. Institute of Physical Chemistry, Academy of Sciences of the USSR, Russia

    Yakov I. Yashin

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Kiselev, A.V., Yashin, Y.I. (1969). Role of the Surface Chemistry of Adsorbents and Nature of Molecular Interactions. In: Gas-Adsorption Chromatography. Springer, Boston, MA. https://doi.org/10.1007/978-1-4899-6503-5_2

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  • DOI: https://doi.org/10.1007/978-1-4899-6503-5_2

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