Abstract
Rydberg wave packets have been the object of intense experimental and theoretical study over the past decade due to their many fascinating semiclassical and quantum characteristics. Long-lived wave packets localized in both the radial and angular dimensions have now been produced in alkali metal atoms.1–4 The methods of quantum control can also be applied to calculate the optimally shaped laser pulse which creates a wave packet having a desired distribution in phase space at a specified “target” time.5 Such wave packets can take the form, for instance, of “Schrödinger cat” states,6 or coherent superpositions of macroscopically distinct electronic states.
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References
Parker and C. R. Stroud, Jr., Coherence and decay of Rydberg wave packets, Phys. Rev. Lett. 56: 716 (1986).
ten Wolde, L. D. Noordam, A. Lagendijk, and H. B. van Linden van den Heuvell. Observation of radially localized electron wave packets, Phys. Rev. Lett. 61: 2099 (1988).
A. Yeazell, M. Mallalieu, J. Parker, and C. R. Stroud, Jr., Classical periodic motion of atomic-electronic wave packets, Phys. Rev. A 40: 5040 (1989).
Maciej Kalinski and J. H. Eberly, New states of hydrogen in a circularly polarized electromagnetic field, Phys. Rev. Lett. 77: 2420 (1996).
J. L. Krause, K. J. Schafer, and M. Ben-Nun, Creating and detecting shaped Rydberg wave packets, Phys. Rev. Lett. in press (1997).
M. Noel and C. R. Stroud, Jr., Young’s double slit experiment within an atom, Phys. Rev. Lett. 75:1252 (1995); Excitation of an atomic electron to a coherent superposition of macroscopically distinct states, Phys. Rev. Lett. 77: 1913 (1996).
R. Jones, C. S. Raman, D. W. Schumacher, and P. H. Bucksbaum, Ramsey interference in strongly driven Rydberg systems, Phys. Rev. Lett. 71: 2575 (1993).
R. Jones, D. You, and P. H. Bucksbaum, Ionization of Rydberg atoms by subpicosecond half-cycle electromagnetic pulses, Phys. Rev. Lett. 70: 1236 (1993).
G. M Lankhuijzen and L. D. Noordam, Streak-camera probing a rubidium wave packet decay in an electric field, Phys. Rev. Lett., 76: 1784 (1996).
J.M. Schins, P. Breger, P. Agostini, R. C. Constantinescu, H. G. Muller, A. Bouhal, G. Grillon, A. Antonetti, and A. Mysyrowicz, Cross-correlation measurements of femtosecond extreme-ultraviolet high-order harmonics, JOSA B, 13: 197 (1996).
JT. Randall. The diffraction of X-rays and electrons by amorphous solids, liquids, and gases, John Wiley and Sons, New York, 1934.
EO. Wollan, Scattering of x-rays from gases. Phys. Rev. 37: 862 (1931).
LWaller and D. R. Hartree, Proc. Roy. Soc. A 124: 119 (1929).
C. Williamson, M. Dantus, S. B. Kim, and A. H. Zewail, Ultrafast diffraction and molecular structure, Chem. Phys. Lett. 196: 529 (1992).
Anderson, I. V. Tomov, and P. M. Rentzepis, A high repetition rate, picosecond hard x-ray system, and its application to time-resolved x-ray diffraction, J. Chem. Phys. 99: 869 (1993).
Ben-Nun, T. J. Martinez, P. M. Weber, and K. R. Wilson, Direct imaging of excited electronic states using diffraction techniques: Theoretical considerations, Chem. Phys. Lett. 262: 405 (1996).
Zhou, J. Peatross, M. M. Murnane, and H. C. Kapteyn, Enhanced high-harmonic generation using 25 fs laser pulses, Phys. Rev. Lett. 76: 752 (1996).
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Schafer, K.J., Krause, J.L. (1998). Ultrafast Diffraction from Rydberg Wave Packets Using High Harmonics. In: DiMauro, L., Murnane, M., L’Huillier, A. (eds) Applications of High-Field and Short Wavelength Sources. Springer, Boston, MA. https://doi.org/10.1007/978-1-4757-9241-6_29
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DOI: https://doi.org/10.1007/978-1-4757-9241-6_29
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