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A. Peterlin

  • Robert D. Ulrich
Part of the Contemporary Topics in Polymer Science book series (CTPS, volume 1)

Abstract

My Ph. D. thesis work was concerned with the intrinsic viscosity of a suspension of rigid spheroids with symmetry axis al and perpendicular axis a2-1-5 The most important result was the derivation of angular distribution of symmetry axis as function of axial ratio p = al/a2 and dimensionless velocity gradient parameter σ = γ/Dr where γ is the transverse velocity gradient and Dr is the rotational diffusion coefficient of the symmetry axis of the spheroid. The steady state distribution function permits the calculation of the gradient dependence of intrinsic viscosity [n]9 streaming birefringence [Δn] and extinction angle χ. The Intrinsic viscosity calculated according to the then accepted rules of excess energy dissipation by the spheroids exhibited an initial increase with a maximum and subsequent drop to a finite value [η]∞ < [η]o. Much later, Kuhn1 suggested a modification of energy dissipation by inclusions of the contribution of Brownian motion which increased [η]o by a factor 2 and made disappear the initial increase and maximum of intrinsic viscosity. The final formulation of excess energy dissipation by Saito2 was used by Scheraga3 for the correct calculation of gradient dependence of intrinsic viscosity of spheroid suspension.

Keywords

Electron Spin Resonance Intrinsic Viscosity Draw Ratio Hydrodynamic Interaction Amorphous Component 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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Copyright information

© Plenum Press, New York 1978

Authors and Affiliations

  • Robert D. Ulrich
    • 1
  1. 1.Noryl Products DepartmentGeneral Electric Plastics DivisionSelkirkUSA

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