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Photoemission in Strongly Correlated Crystalline f-Electron Systems: A Need for a New Approach

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Abstract

The unusual properties of heavy fermion (or heavy electron) materials have sparked an avalanche of research over the last two decades in order to understand the basic phenomena responsible for these properties. The reader is referred to numerous review articles, such as Fisk et al., (1995), Grewe and Steglich (1991), Hess et al., (1993), Lawrence and Mills (1991), Ott and Fisk (1987), Stewart (1984), Thompson and Lawrence (1994). The term heavy fermion refers to materials (thus far only compounds with elements having an unfilled 4f or 5f shells) whose electronic properties suggest that the conduction electrons have a very heavy effective mass. This is inferred from the linear term in the low specific heat (Cp = γT+ OT2) which usually has an upturn at low temperatures and suggests [some of the first discoveries were by Andres et al. (1975), followed by Steglich (1979), Stewart et al (1984), Ott et al. (1983)1 y-values as large as 1500 mJ/mole-K2. deHaas-van Alphen measurements have confirmed the existence of heavy masses [Springford and Reinders (1988), Lonzarich (1988), Onuki (1993)1. The quadratic term in the resistivity and the Pauli susceptibility also indicate the existence of a mass enhancement. It is well established that indeed it is the f-electrons that are responsible for the unusual properties [Grewe and Steglich (1991)].

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References

  • Allen, J.W., 1992, Synchrotron Radiation Research:Advances in Surface and Interface Science, Volume I: Techniques, edited by Z. bachrach, Plenum Press, New York.

    Google Scholar 

  • Allen, J.W., S.-J. Oh, O. Gunnarson, K. Schonhammer, M.B. Maple, M.S. Torikachvili and I. Lindau, 1986, Advances in Physics 35, 275.

    Article  CAS  Google Scholar 

  • Anderson, P.W., 1961, Phys. Rev. 124, 41.

    Article  CAS  Google Scholar 

  • Andres, K., J.E. Graebner and H.R. Ott, 1975, Phys. Rev. Lett. 35, 1779.

    Article  CAS  Google Scholar 

  • Andrews, A.B., J.J. Joyce, A.J. Arko, J.D. Thompson, J. Tang, J.M. Lawrence, and J.C. Hemminger, 1995a, Phys. Rev. B 51, Rapid Comm., 3277.

    Google Scholar 

  • Andrews, A.B., J.J. Joyce, A.J. Arko, J.D. Thompson, Z. Fisk, J. Tang, J.M. Law-rence, P. S. Riseborough, and P.C. Canfield, 1995b, Physica B 206 & 207, 83.

    Google Scholar 

  • Andrews, A.B., J.J. Joyce, A.J. Arko, Z. Fisk, and P.S. Riseborough, 1996, Phys. Rev. B 5 3, 3317.

    Article  Google Scholar 

  • Andrews, A.B., R.I.R. Blyth, A.J. Arko, J.J. Joyce, Z. Fisk, J.D. Thompson, R.J. Bartlett, P.C. Canfield, C.G. Olson, P. Benning, and P.S. Riseborough, 1994, Physica B 199&200, 15.

    Article  Google Scholar 

  • Arko, A.J., J.J. Joyce, A.B. Andrews, R.I.R. Blyth, C.G. Olson, P.C. Canfield, P.J. Benning, D. M. Poirier,J.H. Weaver, and P.S. Riseborough, 1994, in Strongly Correlated Electronic Materials,edited by K. Bedell, S.-Y. Huang, A. Balatsky, D.E. Meltzer, and E. Abrahams, (Addison Wesley), pg.101.

    Google Scholar 

  • Arko, A.J., D.D. Koelling, and B. Reihl, 1983, Phys. Rev. B 27, 3955.

    Article  CAS  Google Scholar 

  • Arko, A.J., J.J. Joyce, A.B. Andrews, J.D. Thompson, J.L. Smith, D. Mandrus, M.F. Hundley, A.L. Cornelius, E.Moshopoulou, Z. Fisk, and P.C. Canfield, Alois Menovsky, 1996, Phys. Rev. B 56, Rapid Corn., R7041.

    Google Scholar 

  • Arko, A.J., J.J. Joyce, A.B. Andrews, J.L. Smith, J.D. Thompson, Z. Fisk, E. Moshopoulou, A. Menovsky and P.C. Canfield, 1997, Physica B 230–232, 16.

    Article  Google Scholar 

  • Arko, A.J., J.J. Joyce, L.E. Cox, L. Morales, J. Sarrao, J.L. Smith, Z. Fisk, A. Menovsky, A. Tahvildar-Zadeh, and M. Jarrell, 1998, J. Alloys and Comp.

    Google Scholar 

  • Arko, A.J., J.J. Joyce, P.C. Canfield, J.D. Thompson, R.J. Bartlett, Z. Fisk, J. Law-rence, J. Tang, and P. Riseborough, 1993, in Vacuum Ultraviolet Radiation Physics, edited by F.J. Wuillemier, Y. Petroff, and I. Nenner, (World Scientific: Singapore), p. 291.

    Google Scholar 

  • Arko, A.J., M.B. Brodsky, G.W. Crabtree, D. Karim, D.D. Koelling, L.R. Windmiller, and J.B. Ketterson, 1975, Phys. Rev. B 12, 4102.

    Article  CAS  Google Scholar 

  • Arko, A.J., M.B. Brodsky, G.W. Crabtree, D. Karim, L.R. Windmiller, and J.B. Ketterson, 1976, in Plutonium 1975 and other Actinides H. Blank and R. Linder, eds. (North Holland, Amsterdam) p. 325.

    Google Scholar 

  • Arko, A.J., P. Armstrong, and M. Wire, 1990, Physica B163, 167.

    Google Scholar 

  • Bickers, N.E., 1987, Rev. Mod. Phys. 59, 845.

    Article  CAS  Google Scholar 

  • Bickers, N.E., D.L. Cox and J.W. Wilkins, 1985, Phys. Rev. Lett. 54, 230.

    Article  CAS  Google Scholar 

  • Bickers, N.E., D.L. Cox and J.W. Wilkins, 1987, Phys. Rev. B 36, 2036.

    Article  Google Scholar 

  • Blyth, R.I.R., J.J. Joyce, A.J. Arko, J. Tang, and J.M. Lawrence, 1992, Phys. Rev. Lett.69, 3418.

    Article  CAS  Google Scholar 

  • Blyth, R.I.R., J.J. Joyce, A.J. Arko, P.C. Canfield, Z. Fisk, J.D. Thompson, R.J. Bartlett, J. Tang, and J.M. Lawrence, 1993, Phys. Rev. B 48, 9497.

    Article  Google Scholar 

  • Fadley, C.F., 1987, Physica Scripta T17, 39.

    Article  CAS  Google Scholar 

  • Fisk, Z., J.L. Sarrao, J.L. Smith, and J.D. Thompson, 1995, Proc. Natl. Acad. Sci. USA, 92, 6663.

    Article  CAS  Google Scholar 

  • Galera, R.M., A.P. Murani, and J. Pierre, 1989, Physica B 156&157, 801.

    Article  Google Scholar 

  • Gamier, M., D. Purdie, K. Breuer, M. Hengsberger, and Y. Baer, 1997, Phys. Rev. B 36, R11399.

    Google Scholar 

  • Grewe, N. and F. Steglich, 1991, Handbook on the Physics and Chemistry of the Rare Earths, K.A. Gschneidner, Jr. and L. Eyerling, editors, (North-Holland, Amsterdam), Vol. 14, pp. 343–474.

    Google Scholar 

  • Grioni, M., D. Malterre, P. Weibel, B. Dardel, and Y. Baer, 1993, Physica B 188, 38.

    Article  Google Scholar 

  • Gunnarson, O., and K. Schonhammer, 1985, Phys. Rev. B 31, 4815.

    Article  Google Scholar 

  • Gunnarson, O., and K. Schonhammer, 1986, in Theory of Heavy Fermions and Valence Fluctuations, T. Kasuya and T. Saso, editors (Springer-Verlag, Berlin, 1986) p. 110.

    Google Scholar 

  • Hess,D.W., P.S. Riseborough, and J.L. Smith, 1993, Encyclopedia of Applied Physics, Vol. 7, George L. Trigg., ed., (VCH Publishers, NY), pp.435–463.

    Google Scholar 

  • Hirsch, J.E., and R.M. Fye, (1989), Phys. Rev. Lett. 56, 2521.

    Article  Google Scholar 

  • Hufner, S., 1986, J. Phys. F 16, L31.

    Article  Google Scholar 

  • Hufner, S., 1992, Z. Phys. B 86, 241.

    Article  Google Scholar 

  • Hufner, S., L. Schlapbach, 1986, Z. Phys. B 64, 417.

    Article  Google Scholar 

  • Jarrell, M., and J.E. Gubernatis, 1996, Physics Reports, Vol. 269, No.3, p133–195.

    Article  Google Scholar 

  • Joyce J.J., and A.J.Arko, 1993a, Phys. Rev. Lett. 70, 1181.

    Article  CAS  Google Scholar 

  • Joyce, J.J., A. J. Arko, J. M. Lawrence, P. C. Canfield, Z. Fisk, R. J. Bartlett, and J. D. Thompson, 1992c, Phys. Rev. Lett. 68 236.

    Article  CAS  Google Scholar 

  • Joyce, J.J., A. J. Arko, J. M. Lawrence, P. C. Canfield, Z. Fisk, R. J. Bartlett, J. D. Thompson, and J. L. Smith, 1992a, J. Less Comm. Met., 181, 161.

    CAS  Google Scholar 

  • Joyce, J.J., A.B. Andrews, A.J. Arko, R.I.R. Blyth, R.J. Bartlett, C.G. Olson, D.M. Poirier, P.C. Canfield,and P.J. Benning, 1996, Phys. Rev. B., to be published.

    Google Scholar 

  • Joyce, J.J., A.J. Arko, A.B. Andrews, and R.I.R. Blyth, 1994a, Phys. Rev. Lett. 72, 1774.

    Article  CAS  Google Scholar 

  • Joyce, J.J., A.J. Arko, A.B. Andrews, R.I.R. Blyth, R.J. Bartlett, J.D. Thompson, Z. Fisk, P.S. Riseborough, P.C. Canfield, C.G. Olson, and P.J. Benning, 1994b, Physica B 205, 365.

    Article  Google Scholar 

  • Joyce, J.J., A.J. Arko, J.L. Sarrao, K.S. Graham, Z. Fisk, and P.S. Riseborough, 1998, submitted to Phys. Rev. Letters.

    Google Scholar 

  • Joyce, J.J., A.J. Arko, J.M. Lawrence, P.C. Canfield, R.J. Bartlett, Z. Fisk, and J.D. Thompson, J. Tang, 1992b, Solid State Comm. 83, 551.

    Article  CAS  Google Scholar 

  • Joyce, J.J., A.J. Arko, P.S. Riseborough, P.C. Canfield, J.M. Lawrence, R.I.R. Blyth, R.J. Bartlett, J.D. Thompson, and Z. Fisk, 1993b, Physica B 186–188, 31.

    Article  CAS  Google Scholar 

  • Kakizaki, A., A. Harasawa, T. Ishii, T. Kashiwakura, A. Kamata, S. Kunii, 1995, J. Phys. Soc. Japan 64, 302.

    Article  CAS  Google Scholar 

  • Kang, J.S., J.W. Allen, O. Gunnarsson, N.E. Christensen, and O.K. Anderson,Y. Las-sailly, M. B. Maple and M. S. Torkachvilli, 1990, Phys. Rev. B 41, 6610.

    Article  CAS  Google Scholar 

  • Lawrence, J.M., and D.M. Mills, 1991, Comments Cond. Mat. Phys., 15, 163.

    Google Scholar 

  • Lawrence, J.M., G.H. Kwei, P.C. Canfield, J.G. DeWitt, and A.C. Lawson, 1994, Phys. Rev. B49.

    Google Scholar 

  • Lee, P.A., T.M. Rice, J.W. Serene, L.J. Sham, and J.W. Wilkins, 1986, Corn. Cond. Mat. Phys. 12, 99.

    CAS  Google Scholar 

  • Liu, L.Z., J.W. Allen, O. Gunnarsson, N.E. Christensen, and O.K. Anderson, 1992, Phys. Rev. B 45, 8934.

    Article  CAS  Google Scholar 

  • Liu, S.H., 1993, in Handbook on the Physics and Chemistry of Rare Earths, Vol. 17, Ch. 111 (North Holland, Amsterdam, 1993) pp 87–148.

    Google Scholar 

  • Liu, S.H., 1997, Physica B 240, 49

    Article  CAS  Google Scholar 

  • Lonzarich, G.G., 1988, J. Magn. Magn. Mat. 76–77, 1.

    Google Scholar 

  • Malterre, D., M. Grioni, P. Weibel, B. Dardcl and Y. Baer, 1992a, Europhys. Lett.20, 445.

    Article  CAS  Google Scholar 

  • Malterre, D., M. Grioni, P. Weibel, B. Dardcl and Y. Baer, 1992b, Phys. Rev. Lett. 68, 2656.

    Article  CAS  Google Scholar 

  • Matzdorf, R., G. Meister, and A. Goldmann, 1993, Surf. Sci. 286, 56.

    Article  CAS  Google Scholar 

  • Norman, M.R., 1985, Phys. Rev. B 31, 6261.

    Article  CAS  Google Scholar 

  • Norman, M.R., D.D. Koelling and A.J. Freeman, 1985, Phys. Rev. B 31, 6251.

    Article  CAS  Google Scholar 

  • Nozicres, P., 1985, Ann. de Phys. 10, 19.

    Article  Google Scholar 

  • Oh, S.J., 1993, Physica B 186–188, 637.

    Google Scholar 

  • Oliveira, L.N. and J. Wilkins (1981), Phys. Rev. Lett. 47, 1553.

    Article  Google Scholar 

  • Onuki, Y., 1993, Physica B 186–188, 92.

    Google Scholar 

  • Ott, H.R., and Z. Fisk, 1987, in Handbook on the Physics and Chemistry of the Actinides, A.J. Freeman and G.H. Lander, editors, (North-Holland, Amsterdam), pp. 85–225.

    Google Scholar 

  • Ott, H.R., H. Rudigicr, Z. Fisk, and J.L. Smith, 1993, Phys. Rev. Lett. 50, 1595.

    Article  Google Scholar 

  • Patthey, F., B. Delley, W.D. Schneider, and Y. Baer, 1985, Phys. Rev. Lett. 55, 1518.

    Article  CAS  Google Scholar 

  • Patthey, F., J.-M. Imer, W.-D. Schneider, H. Beck and Y. Baer, 1990, Phys. Rev. B 42, 8864.

    Article  CAS  Google Scholar 

  • Patthey, F., W.-D. Schneider, Y. Baer, and B. Dcllcy, 1987a, Phys. Rev. Lett. 58, 2810.

    Article  CAS  Google Scholar 

  • Patthey, F., W.D. Schneider, M. Grioni, D. Malterre, and Y. Baer, 1993, Phys. Rev. Lett. 70, 1179.

    Article  CAS  Google Scholar 

  • Patthey, F., W.D. Schneider, Y. Baer, and B. Delley, 1986, Phys. Rev. B 34, 2967.

    Article  CAS  Google Scholar 

  • Patthey, F., W.D. Schneider, Y. Baer, and B. Delley, 1987b, Phys. Rev. B 35, 5903. Phys. Rev. Lett. 65, 496–9.

    Google Scholar 

  • Pruschke, Th., and N. Grewe (1989), Z. Phys. B 74, 439.

    Article  Google Scholar 

  • Sheng, Q.G. and B.R. Cooper, 1995, Phil. Mag. Lett. 72, 123.

    Article  CAS  Google Scholar 

  • Silver, R.N., J. E. Gubernatis, D. S. Sivia, and Mark Jarrell, 1990

    Google Scholar 

  • Springford, M., and P.H.P. Reinders, 1988, J. Magn. Magn. Mat. 76–77, 11.

    Article  Google Scholar 

  • Steglich, F., J. Aarts, C.D. Bredl, W. Lieke, D. Meschede, W. Franz, and H. Schafer, 1979, Phys. Rev. Lett. 43, 1892.

    Article  CAS  Google Scholar 

  • Steiner, M.M., R. C. Albers, and L. J. Sham, 1994, Phys. Rev. Lett. 72, 2923.

    Article  CAS  Google Scholar 

  • Stewart, G. R., 1984, Rev. Mod. Phys. 56, 755.

    Article  CAS  Google Scholar 

  • Stewart, G.R., Z. Fisk, J.O. Willis, and J.L. Smith, 1984, Phys. Rev. Lett. 52, 679.

    Article  CAS  Google Scholar 

  • Strange, P., and D. M. Newns, J. Phys. F 16, 335.

    Google Scholar 

  • Tahvildar-Zadeh, A.N., M. Jarrell and J.K. Freericks, 1997, Phys. Rev. B 55, R3332.

    Article  CAS  Google Scholar 

  • Tahvildar-Zadeh, A.N., M. Jarrell and J.K. Freericks,1998, In preparation.

    Google Scholar 

  • Takahashi, T., T. Morimoto, T. Yokoya, M. Kohgi, and T. Satoh, 1994, Phys. Rev. B 49, 15688.

    Article  CAS  Google Scholar 

  • Tang, J., J.M. Lawrence, and J.C. Hemminger, 1993, Phys. Rev. B 48, 15342.

    Article  CAS  Google Scholar 

  • Thompson, J.D. and J.M. Lawrence, 1994, Handbook on the Physics and Chemistry of the Rare Earths, K.A. Gschneidner,Jr.and L. Eyerling, editors, (North-Holland, Amsterdam), Vol 19, pp. 383–478.

    Google Scholar 

  • Tjeng, L.H., S.-J. Oh, E.-J. Cho, H.-J. Lin, C.T. Chen, G.-W. Gweon, J.-H. Park, J.W. Allen, T. Suzuki, M.S. Makivic, and D.L. Cox, 1993, Phys. Rev. Lett. 71, 1419.

    Article  CAS  Google Scholar 

  • Weibel, P., M. Grioni, D. Malterre, B. Dardel, Y. Baer, and M. Besnus, 1993, Z. Phys. B 91, 337.

    Article  CAS  Google Scholar 

  • Weschke, E., C. Laubschat, T. Simmons, M. Domke, O. Strebel, and G. Kaindl, 1991, Phys. Rev. B 44, 8304.

    Article  CAS  Google Scholar 

  • Wilson, K.G., (1975), Rev. Mod. Phys. 47, 733.

    Article  Google Scholar 

  • Zwicknagl, Gertrud, 1992, Advances in Physics 41, 203.

    Article  CAS  Google Scholar 

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Arko, A.J. et al. (1999). Photoemission in Strongly Correlated Crystalline f-Electron Systems: A Need for a New Approach. In: Gonis, A., Kioussis, N., Ciftan, M. (eds) Electron Correlations and Materials Properties. Springer, Boston, MA. https://doi.org/10.1007/978-1-4615-4715-0_3

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