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Multiphoton Spectroscopy

  • Chapter
Progress in Atomic Spectroscopy

Part of the book series: Physics of Atoms and Molecules ((PAMO))

Abstract

In this chapter, a class of electronic transitions in atoms involving the simultaneous absorption or emission of more than one photon is discussed. In describing Raman scattering in atoms as a two-photon process, in which one photon of frequency ω1 is absorbed and one of frequency ω2 (≠ω1) is emitted, Kramers and Heisenberg(1) pointed out that an entirely new process may take place, namely, singly stimulated two-photon emission. A bound electron in an excited state | 〉 can reach a lower state |f〉 via the emission of two photons. The presence of a photon field of frequency ω1 stimulates the simultaneous emission of one photon having the same frequency and of a second photon of frequency ω 2 = ω fi — ω 1. This process is greatly enhanced in the presence of real intermediate states and was therefore observed first under these conditions by Yatsiv et al. (2) In the absence of intermediate states, singly stimulated two-photon emission and anti-Stokes Raman scattering in atoms were reported by Bräunlich et al.(3–5)

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  1. Peter Bräunlich

    Present address: Department of Physics, Washington State University, Pullman, Washington, 99163, USA

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  1. Bendix Research Laboratories, Southfield, Michigan, 48076, USA

    Peter Bräunlich

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  1. Ist Institute of Physics, Justus Liebig University, Giessen, Germany

    W. Hanle

  2. Institute of Atomic Physics, University of Stirling, Stirling, Scotland

    H. Kleinpoppen

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Bräunlich, P. (1979). Multiphoton Spectroscopy. In: Hanle, W., Kleinpoppen, H. (eds) Progress in Atomic Spectroscopy. Physics of Atoms and Molecules. Springer, Boston, MA. https://doi.org/10.1007/978-1-4613-3935-9_4

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