Skip to main content

Where are we going with molecular beams?

  • Chapter
Rarefied Gas Dynamics

Abstract

A love affair with molecular beams spanning nearly a quarter of a century has made this reporter a true believer in their powers. But believers, however true, are not necessarily successful seers. Indeed, more things have happened in those 25 years than were dreamt of in his original philosophy. Even so, when the organizers of this conference handed him the crystal ball with an invitation to peer into the future, he found the temptation irresistible. May whatever honor he might enjoy in his country of molecular beams and rarefied gas dynamics be spared, even though he dares to impersonate a prophet.

This is a preview of subscription content, log in via an institution to check access.

Access this chapter

Chapter
USD 29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD 39.99
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
Softcover Book
USD 54.99
Price excludes VAT (USA)
  • Compact, lightweight edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Institutional subscriptions

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  1. D. R. Miller, J. P. Toennies and K. Winkelmann, 9th RGD Symp. (M. Becker and M. Fiebig, eds.) V 2, C9-1 (DFVLR, Göttingen 1974)

    Google Scholar 

  2. U. Borkenhagen, H. Malthan and J. P. Toennies, J. Chem. Phys. 73173 (1975)

    Article  ADS  Google Scholar 

  3. U. Buck, F. Huisken, J. Schleusener, Phys. Rev. Lett. 38, 680 (1977)

    Article  ADS  Google Scholar 

  4. U. Buck, F. Huisken, J. Schleusener J. Chem. Phys. 72, 1512 (1979)

    Article  ADS  Google Scholar 

  5. J. Andres, U. Buck, F. Huisken, J. Schleusener and F. Torello, J. Chem. Phys. 73, 5620 (1980)

    Article  ADS  Google Scholar 

  6. J. P. Toennies and K. Winkelmann, J. Chem. Phys. 66, 3965 (1977)

    Article  ADS  Google Scholar 

  7. R. Compargue, A. Lebehot, J. C. Lemonnier and D. Marette, 12th RGD, Prog. Astro. Aero.(S.S. Fisher,ed)74, 823(AIAA,NY 1981 )

    Google Scholar 

  8. G. Brusdeylins, R. B. Doak and J. P. Toennies, Phys. Rev. Lett. 46, 437 (1981)

    Article  ADS  Google Scholar 

  9. G. Brusdeylins, R. B. Doak and J. P. Toennies, J. Chem. Phys. 75, 1784, 1793 (1981)

    Article  ADS  Google Scholar 

  10. M. Faubel, K. H. Kohl and J. P. Toennies, 12th RGD, Prog. Astro. Aero. 74862 (1981)

    Google Scholar 

  11. M. Faubel, K. H. Kohl and J. P. Toennies, J. Chem. Phys. 73, 2506 (1980)

    Article  ADS  Google Scholar 

  12. H. Ashkenas and F. S. Sherman, 4th RGD (J. H. Deleeus, ed) V284, Academic Press, NY (1966)

    Google Scholar 

  13. J. B. Anderson and J. B. Fenn, Phys. Fluids8, 780 (1965)

    Article  ADS  Google Scholar 

  14. O. F. Hagena and W. Henkes, Z. Naturforsch. 15A, 851 (1960)

    ADS  Google Scholar 

  15. E. P. Muntz, Phys. Fluids580 (1962)

    Article  ADS  Google Scholar 

  16. P. V. Marrone, Univ. Toronto IAS Report 113 (1967)

    Google Scholar 

  17. F. Robben and L. Talbot, Phys. Fluids9, 653 (1966)

    Article  ADS  Google Scholar 

  18. D. R. Miller and R. P. Andres, J. Chem. Phys.,46, 3418 (1967)

    Article  ADS  Google Scholar 

  19. N. V. Karelov, A. K. Rebrov, R. G. Sharafutdinov, 11th RGD Symp. (R Campargue, ed.) v2, 1131 (CEA Paris 1919 )

    Google Scholar 

  20. M. P. Sinha, C. D. Caldwell and R. N. Zare, J. Chem. Phys. 61, 491 (1974)

    Article  ADS  Google Scholar 

  21. R. E. Smalley, L. Wharton and D. H. Levy, J. Chem. Phys. 63.,4977 (1975)

    Article  ADS  Google Scholar 

  22. R. E. Smalley, L. Wharton and D. H. Levy, Accts. Chem. Res. 10, 139 (1977)

    Article  Google Scholar 

  23. R. E. Smalley, J. Phys. Chem. 86, 3504 (1982)

    Article  Google Scholar 

  24. E. W. Becker and W. Henkes, Z. Phys. 146, 333 (1956)

    Article  ADS  Google Scholar 

  25. O. F. Hagena in “Mol. Beams and Low Density Gas Dyn.” (P. P.Wegener, ed.) p 93 ( Dekker, N.Y. 1974 )

    Google Scholar 

  26. P. Kebarle, Ann. Rev. Phys. Chem. 28, 445 (1977)

    Article  ADS  Google Scholar 

  27. A. W. Castleman, Jr., in “Kinetics of Ion Molecule Reactions”, p. 295 (Plenum, N. Y. 1979); P. M. Holland and — J. Chem. Phys. 76, 4204 (1982)

    Book  Google Scholar 

  28. A. W. Castleman, Jr., in “Kinetics of Ion Molecule Reactions”, p. 295 (Plenum, N. Y. 1979); P. M. Holland and — J. Chem. Phys. 76, 4204 (1982)

    Article  ADS  Google Scholar 

  29. J. Gspann, This Symp. — and H. Vollmar, J. Physique39,C-6 330 (1978)

    Google Scholar 

  30. J. Farges, J. Cryst. Growth31,79 (1975); B. G. DeBoer and G. D. Stein, Surf. Sci. 106, 84 (1981)

    Article  Google Scholar 

  31. J. Farges, J. Cryst. Growth31,79 (1975); B. G. DeBoer and G. D. Stein, Surf. Sci. 106, 84 (1981)

    Article  ADS  Google Scholar 

  32. O. F. Hagena and W. Obert, J. Chem. Phys. 56, 1793 (1972)

    Article  ADS  Google Scholar 

  33. A. Hermann, E. Schumacher and L. Wöste, Helv. Chim. Acta 6l, 453 (1978); see also Ref. 46

    Article  Google Scholar 

  34. A. Hermann, E. Schumacher and L. Wöste, Helv. Chim. Acta 6l, 453 (1978); see also Ref. 46

    Article  ADS  Google Scholar 

  35. A. Hermann, E. Schumacher and L. Wöste, Helv. Chim. Acta 6l, 453 (1978); see also Ref. 46

    Article  Google Scholar 

  36. I. F. Silvera, F. Tommasini and R. J. Wijngaarden, 10th RGD (J.L. Potter, ed.) v2, 1295 (1976) and unpublished work.

    Google Scholar 

  37. A. Van Deursen, A. van Lumig and J. Reuss, Int. J. Mass Spect. Ion Phys. 18, 129 (1975); H. Vehmeyer, R. Feltgen, P. Chakrahorti, M. Dukov, F. Torello and H. Pauly, Chem.Phys.Lett. 42, 597 (1976)

    Article  Google Scholar 

  38. A. Van Deursen, A. van Lumig and J. Reuss, Int. J. Mass Spect. Ion Phys. 18, 129 (1975); H. Vehmeyer, R. Feltgen, P. Chakrahorti, M. Dukov, F. Torello and H. Pauly, Chem.Phys.Lett. 42, 597 (1976)

    Article  ADS  Google Scholar 

  39. D. H. Levy, Adv. Chem. Phys. 47, 323 (l98l)

    Article  Google Scholar 

  40. K. Sattler, This symp.

    Google Scholar 

  41. F. M. Devienne and M. Teisseire, This symp.

    Google Scholar 

  42. D. J. Surman, J. C. Vickerson, J. Chem. Soc.Chem.Comm. 324 (1981)

    Google Scholar 

  43. M. Barker, R. S. Bordol, R. D. Sedgwick and A.N. Tyler ibid. 325

    Google Scholar 

  44. P. G. Bentley, Nature190, 432 (1961)

    Article  ADS  Google Scholar 

  45. W. Henkes, Z. Naturforsch. 16a, 842 (1961)

    ADS  Google Scholar 

  46. R. E. Leckenby, E. J. Robbins and P. Trevalion, Proc. Roy. Soc. A286, 409 (1964)

    ADS  Google Scholar 

  47. T. A. Milne, A. E. Vandegrift, F.T. Greene, J. Chem. Phys. 52, 1552 (1970); ibid. 47, 4095 (1967) and57, 2221 (1972)

    Article  ADS  Google Scholar 

  48. T. A. Milne, A. E. Vandegrift, F.T. Greene, J. Chem. Phys. 52, 1552 (1970); ibid. 47, 4095 (1967) and57, 2221 (1972)

    Article  ADS  Google Scholar 

  49. T. A. Milne, A. E. Vandegrift, F.T. Greene, J. Chem. Phys. 52, 1552 (1970); ibid. 47, 4095 (1967) and57, 2221 (1972)

    Article  ADS  Google Scholar 

  50. D. Golomb, R. E. Good, R. F. Brown, J. Chem. Phys. 52, 1545 (1970)

    Article  ADS  Google Scholar 

  51. A. J. Gordon, Y. T. Lee and D. R. Herschbach, J. Chem. Phys. 54, 2393 (1971)

    Article  ADS  Google Scholar 

  52. J. M. Calo, J. Chem. Phys. 62, 4904 (1974)

    Article  ADS  Google Scholar 

  53. K. C. Janda, J. C. Hemminger, J. S. Winn, S. E. Novick, S. J. Harris and W. Klemperer, J. Chem. Phys. 63, 1419 (1979)

    Article  ADS  Google Scholar 

  54. M. P. Sinha, A. Schulty, R. N. Zare, J. Chem. Phys. 58, 549 (1973)

    Article  ADS  Google Scholar 

  55. K. Bergmann, U. Hefter and P. Hering, Chem.Phys. 32, 329 (1978); ibid. 20, 391 (1976)

    Article  Google Scholar 

  56. K. Bergmann, U. Hefter and P. Hering, Chem.Phys. 32, 329 (1978); ibid. 20, 391 (1976)

    Google Scholar 

  57. P. M. Dehmer, J. Chem. Phys. 76, 1263,3433 (1982); 75, 5625 (1981)

    Article  ADS  Google Scholar 

  58. P. M. Dehmer, J. Chem. Phys. 76, 1263,3433 (1982); 75, 5625 (1981)

    Article  Google Scholar 

  59. D. H. Levy, This symp.

    Google Scholar 

  60. J. Tusa, M. Sulkes and S. A. Rice, J. Chem. Phys. 70, 3136 (1979);72, 5733 (1980)

    Article  ADS  Google Scholar 

  61. J. Tusa, M. Sulkes and S. A. Rice, J. Chem. Phys. 70, 3136 (1979);72, 5733 (1980)

    Google Scholar 

  62. M. Yamashita, T. Sano, S. Kotake, J. Fenn, J. Chem. Phys. 75, 5355 (1981)

    Article  ADS  Google Scholar 

  63. D. R. Worsnop, S. Bülow and D. R. Herschbach, in press

    Google Scholar 

  64. A. Rebrov, This symp.

    Google Scholar 

  65. O. F. Hagena, Z. f. Angewandte Phys. 16, 183 (1963);17, 542 (1964)

    Google Scholar 

  66. O. F. Hagena, Z. f. Angewandte Phys. 16, 183 (1963);17, 542 (1964)

    Google Scholar 

  67. W. R. Gentry, C. F. Giese, Rev. Sci. Inst. 49, 595 (1978).

    Article  ADS  Google Scholar 

  68. W. R. Gentry, C. F. Giese, J. Chem. Phys. 67, 5389 (1977)

    Article  ADS  Google Scholar 

  69. A. Amirav, U. Even and J. Jortner, Chem. Phys. Lett. 83, 1 (1981)

    Article  ADS  Google Scholar 

  70. J. B. Cross, J. J. Valentini, Rev. Sci. Inst. 51, 38 (1982); T. E. Adains, B. H. Rockney, R. J. Morrison and E. R. Grant, ibid. 52, 1469 (1981); C. E. Otis and P.M. Johnson, ibid. 51, 1128 (1980); A. Auerbach and R. McDiarmid, ibid. 51, 1273; F. M. Behlen and S. A. Rice, J. Chem. Phys. 75, 5673; J. Tusa, M. Sulkes, S. A. Rice, C. Jouvet, ibid. 76, 3573 (1982)

    Article  ADS  Google Scholar 

  71. J. B. Cross, J. J. Valentini, Rev. Sci. Inst. 51, 38 (1982); T. E. Adains, B. H. Rockney, R. J. Morrison and E. R. Grant, ibid. 52, 1469 (1981); C. E. Otis and P.M. Johnson, ibid. 51, 1128 (1980); A. Auerbach and R. McDiarmid, ibid. 51, 1273; F. M. Behlen and S. A. Rice, J. Chem. Phys. 75, 5673; J. Tusa, M. Sulkes, S. A. Rice, C. Jouvet, ibid. 76, 3573 (1982)

    Article  ADS  Google Scholar 

  72. J. B. Cross, J. J. Valentini, Rev. Sci. Inst. 51, 38 (1982); T. E. Adains, B. H. Rockney, R. J. Morrison and E. R. Grant, ibid. 52, 1469 (1981); C. E. Otis and P.M. Johnson, ibid. 51, 1128 (1980); A. Auerbach and R. McDiarmid, ibid. 51, 1273; F. M. Behlen and S. A. Rice, J. Chem. Phys. 75, 5673; J. Tusa, M. Sulkes, S. A. Rice, C. Jouvet, ibid. 76, 3573 (1982)

    Article  ADS  Google Scholar 

  73. A. Auerbach and R. McDiarmid, Rev. Sci. Inst. 51, 1273;

    Google Scholar 

  74. F. M. Behlen and S. A. Rice, J. Chem. Phys. 75, 5673;

    Google Scholar 

  75. J. B. Cross, J. J. Valentini, Rev. Sci. Inst. 51, 38 (1982); T. E. Adains, B. H. Rockney, R. J. Morrison and E. R. Grant, ibid. 52, 1469 (1981); C. E. Otis and P.M. Johnson, ibid. 51, 1128 (1980); A. Auerbach and R. McDiarmid, ibid. 51, 1273; F. M. Behlen and S. A. Rice, J. Chem. Phys. 75, 5673; J. Tusa, M. Sulkes, S. A. Rice, C. Jouvet, ibid. 76, 3573 (1982)

    Google Scholar 

  76. Beam Dynamics, 623 E. 57th St. Minneapolis, MN 55417; Laser Technics, 6007 Osuna Rd. N.E.,Albuquerque, NM 87109; Quanta Ray, 1250 Charleston Rd., Mt. View, Cal. 94043

    Google Scholar 

  77. H. W. Lülf and P. Andresen, This Symp.

    Google Scholar 

  78. K. L. Saenger, J. Chem. Phys75, 2467 (l98l)

    Article  ADS  Google Scholar 

  79. L. Dunoyer, Compt. Rend. 151, 1068 (1913); Le Radium10,400(1913)

    Google Scholar 

  80. L. Dunoyer, Compt. Rend. 151, 1068 (1913); Le Radium10,400(1913)

    Article  Google Scholar 

  81. D. J. Marsden, 4th RGD (J. H. DeLeeuw, ed)v 2, 565 (Academ. 1966 )

    Google Scholar 

  82. G. M. McClelland, G. D. Kubrak, H. G. Rennagel and R. N. Zare, Phys. Rev. Lett. 46, 831 (1981)

    Article  ADS  Google Scholar 

  83. D. Ettinger, K. Honma, M. Keil and J. C. Polanyi, Chem. Phys. Lett. 87, 413 (1981); J. W. Hepburn, F. J. Northrup, G. Ogram, J. C.Polanyi and J. M. Williamson, Chem. Phys. Lett. 85., 127(1982)

    Article  ADS  Google Scholar 

  84. D. Ettinger, K. Honma, M. Keil and J. C. Polanyi, Chem. Phys. Lett. 87, 413 (1981); J. W. Hepburn, F. J. Northrup, G. Ogram, J. C.Polanyi and J. M. Williamson, Chem. Phys. Lett. 85., 127(1982)

    Article  ADS  Google Scholar 

  85. F. Frankel, J. Hager, W. Kruger, H. Walther, C. T. Campbell, G. Ertl, H. Kuipers and K. Segner, Phys.Rev. Lett. 46, 152 (1981)

    Article  ADS  Google Scholar 

  86. R. R. Cavanagh and D. S. King, Phys.Rev. Lett. 47, 1829 (1981)

    Article  ADS  Google Scholar 

  87. A. W. Kleyn, A. C. Luntz and D. J. Auerbach, Phys. Rev. Lett. 47,1169 (1981); Surf. Sci. 171, 33 (1982); J. Chem. Phys. 76, 1, (1982)

    Article  ADS  Google Scholar 

  88. A. W. Kleyn, A. C. Luntz and D. J. Auerbach, Phys. Rev. Lett. 47,1169 (1981); Surf. Sci. 171, 33 (1982); J. Chem. Phys. 76, 1, (1982)

    Article  Google Scholar 

  89. A. W. Kleyn, A. C. Luntz and D. J. Auerbach, Phys. Rev. Lett. 47,1169 (1981); Surf. Sci. 171, 33 (1982); J. Chem. Phys. 76, 1, (1982)

    Article  Google Scholar 

  90. D. H. Maylotte, J. C. Polanyi, K. B. Woodall, J. Chem. Phys. 57, 1547 (1972); L. T. Cowley, D. S. Horne and J. C. Polanyi, Chem. Phys. Lett. 12, 144 (1971)

    Article  ADS  Google Scholar 

  91. D. H. Maylotte, J. C. Polanyi, K. B. Woodall, J. Chem. Phys. 57, 1547 (1972); L. T. Cowley, D. S. Horne and J. C. Polanyi, Chem. Phys. Lett. 12, 144 (1971)

    Article  ADS  Google Scholar 

  92. D. H. Maylotte, J. C. Polanyi, K. B. Woodall, J. Chem. Phys. 57, 1547 (1972); L. T. Cowley, D. S. Horne and J. C. Polanyi, Chem. Phys. Lett. 12, 144 (1971)

    Article  ADS  Google Scholar 

  93. D. H. Maylotte, J. C. Polanyi, K. B. Woodall, J. Chem. Phys. 57, 1547 (1972); L. T. Cowley, D. S. Horne and J. C. Polanyi, Chem. Phys. Lett. 12, 144 (1971)

    Article  ADS  Google Scholar 

  94. D. A. Mantell, S. B. Ryali, B. Halpern, G. L. Haller and J. B. Fenn, Chem. Phys. Lett. 81, 185 (1981)

    Article  ADS  Google Scholar 

  95. T. E. Gough, R. E. Miller and G. Scoles, Appl.Phys.Lett. 30, 338 (1977) and private communication.

    Article  ADS  Google Scholar 

  96. M. A. Covington, G. N. Liu and K. A. Lincoln, AIAA J15, 1174 (1977); Int. J. Mass. Spect. and Ion Phys16, 191 (1975)

    Article  ADS  Google Scholar 

  97. M. A. Covington, G. N. Liu and K. A. Lincoln, AIAA J15, 1174 (1977); Int. J. Mass. Spect. and Ion Phys16, 191 (1975)

    Article  Google Scholar 

  98. F.Tehranian and D. R. Olander, private communication

    Google Scholar 

  99. S. P. Tang, N. G. Utterback, J. F. Frichnicht, J. Chem. Phys. 64, 3833 (1976); Phys. Fluid. 19, 900 (1976)

    Article  ADS  Google Scholar 

  100. S. P. Tang, N. G. Utterback, J. F. Frichnicht, J. Chem. Phys. 64, 3833 (1976); Phys. Fluid. 19, 900 (1976)

    Article  ADS  Google Scholar 

  101. S. P. Tang, N. G. Utterback, J. F. Frichnicht, J. Chem. Phys. 64, 3833 (1976); Phys. Fluid. 19, 900 (1976)

    Article  ADS  Google Scholar 

  102. S. P. Tang, N. G. Utterback, J. F. Frichnicht, J. Chem. Phys. 64, 3833 (1976); Phys. Fluid. 19, 900 (1976)

    Article  ADS  Google Scholar 

  103. R. Beuhler and L. Friedman, Phys.Rev.Lett. 48, 1097 (1982)

    Article  ADS  Google Scholar 

  104. M. Dole, L.L. Mack, R. L. Hines, R. C. Mobley, L. D. Ferguson, M. B. Alice, J. Chem. Phys. 49, 2240(1968);52, 4977 (1970)

    Article  ADS  Google Scholar 

  105. M. Dole, L.L. Mack, R. L. Hines, R. C. Mobley, L. D. Ferguson, M. B. Alice, J. Chem. Phys. 49, 2240(1968);52, 4977 (1970)

    Article  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Editor information

Editors and Affiliations

Rights and permissions

Reprints and permissions

Copyright information

© 1985 Springer Science+Business Media New York

About this chapter

Cite this chapter

Fenn, J.B. (1985). Where are we going with molecular beams?. In: Belotserkovskii, O.M., Kogan, M.N., Kutateladze, S.S., Rebrov, A.K. (eds) Rarefied Gas Dynamics. Springer, Boston, MA. https://doi.org/10.1007/978-1-4613-2467-6_8

Download citation

  • DOI: https://doi.org/10.1007/978-1-4613-2467-6_8

  • Publisher Name: Springer, Boston, MA

  • Print ISBN: 978-1-4612-9497-9

  • Online ISBN: 978-1-4613-2467-6

  • eBook Packages: Springer Book Archive

Publish with us

Policies and ethics