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Oceanography pp 163-191 | Cite as

Radioactive Tracers in the Sea

  • Hugh D. Livingston
  • William J. Jenkins
Conference paper

Abstract

The oceans are a critical component of our environment. Physically, they modify climate, not only on a regional and local scale, but on a planetary scale as well. A significant fraction of the intrahemispheric heat flux is caused by oceanic circulation. The high productivity regions of the ocean represent an important source of food. The oceans not only exert a long time-scale control over the geochemical cycling of many elements, but they play an increasingly important role in the disposal of mankind’s unwanted byproducts.

Keywords

International Atomic Energy Agency Nuclear Fuel Radioactive Tracer North Atlantic Deep Water Global Fallout 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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References

  1. Aller, R. C., and J. K. Cochran. 1976 234Th/238U disequilibrium in nearshore sediment: particle reworking and diagenetic time scales. Earth Planet. Sci. Lett. 29, 37–50.CrossRefGoogle Scholar
  2. Armi, L. 1978. Some evidence for boundary mixing in the deep ocean. J. Geophys. Res. 83, 1971–1979.CrossRefGoogle Scholar
  3. Aston, S. R., and D. A. Stanners. 1979. The determination of estuarine sedimentation rates by 134Cs/137Cs and other artificial radionuclide profiles. Estuarine Coastal Mar. Sci. 9, 529–541.CrossRefGoogle Scholar
  4. Bennett, C. L., R. P. Beukens, M. R. Clover, D. Elmore, H. E. Gove, L. Kilius, A. E. Litherland, and K. H. Purser, 1978. Radiocarbon dating with electrostatic accelerators: dating of milligram samples. Science 20, 345–346.CrossRefGoogle Scholar
  5. Benninger, L. K., R. C. Aller, J. K. Cochran, and K. K. Turekian. 1979. Effects of biological sediment mixing on the 210Pb chronology and trace metal distribution in a Long Island Sound sediment core. Earth Planet. Sci. Lett. 43, 241–259.CrossRefGoogle Scholar
  6. Bowen, V. T., and H. D. Livingston. 1981. Radionuclide distributions in sediment cores retrieved from marine radioactive waste dump sites. In: Impacts of Radionuclide Releases into the Marine Environment. IAEA, Vienna, pp. 33–63.Google Scholar
  7. Bowen, V. T., and W. Roether. 1973. Vertical distributions of Strontium-90, Cesium-137 and tritium near 45° North in the Atlantic. J. Geophys. Res. 78, 6277–6285.CrossRefGoogle Scholar
  8. Bowen, V. T., V. E. Noshkin, H. L. Volchok, H. D. Livingston, and K. M. Wong. 1974. Cesium-137 to strontium-90 ratios in the Atlantic Ocean 1966 through 1972. Limnol. Oceanog. 19, 670–681.CrossRefGoogle Scholar
  9. Bowen, V. T., H. D. Livingston, and J. C. Burke. 1976. Distributions of transuranium nuclides in sediment and biota of the North Atlantic Ocean. In: Transuranium Nuclides in the Environment. IAEA, Vienna, pp. 107–120.Google Scholar
  10. Bowen, V. T., V. E. Noshkin, H. D. Livingston, and H. L. Volchok. 1980. Fallout radionuclides in the Pacific Ocean: horizontal and vertical distributions, largely from GEOSECS stations. Earth Planet. Sci. Lett. 49, 411–434.CrossRefGoogle Scholar
  11. Broecker, W. S., and H. G. Ostlund. 1979. Property distributions along the O q = 26.8 isopycnal in the Atlantic Ocean. J. Geophys. Res. 84, 1145–1154.CrossRefGoogle Scholar
  12. Broecker, W. S., and T-H. Peng. 1980. The radiocarbon age of North Atlantic deep water revisited. J. Geophys. Res. Submitted.Google Scholar
  13. Broecker, W. S., T-H. Peng, and M. Stuiver. 1978. An estimate of the upwelling rate in the equatorial Atlantic based on the distribution of bomb radiocarbon. J. Geophys. Res. 83, 6179–6186.CrossRefGoogle Scholar
  14. Broecker, W. S., T-H. Peng, and R. Engh. 1980. Modelling the carbon system. Radiocarbon 22(3). In press.Google Scholar
  15. Bruland, K. W. 1980. Oceanographic distributions of cadmium, zinc, nickel and copper in the North Pacific. Earth Planet. Sci. Lett. 47, 176–198.CrossRefGoogle Scholar
  16. Clarke, W. B., W. J. Jenkins, and Z. Top. 1976. Determination of tritium by mass spectrometric measurement of 3He. Intl. J. Appl. Rad. Isotopes 27, 515–522.CrossRefGoogle Scholar
  17. Craig, H. 1969. Abyssal carbon and radiocarbon in the Pacific. J. Geophys. Res. 74,5491–5506.CrossRefGoogle Scholar
  18. Deutches Hydrographisches Institut. 1980. Meerwasser. In: Umweltradioak- tivitat und Strahlenbelasting. Jahresbericht, 1977. Der Bundeminister des Innern, Bonn, pp. 58–63.Google Scholar
  19. Dreisigacker, E., and W. Roether. 1978. Tritium and 90Sr in North Atlantic surface water. Earth Planet. Sci. Lett. 38, 301–312.CrossRefGoogle Scholar
  20. Duursma, E. K., and M. G. Gross. 1971. Marine sediments and radioactivity. In: Radioactivity in the Marine Environment (A. H. Seymour, Ed.). U.S. Natl. Acad. Sci., Nat. Res. Council, Washington, D.C., pp. 147–160.Google Scholar
  21. Dyer, R. 1976. Environmental surveys of two deep-sea radioactive waste disposal sites using submersibles. In: Proceedings of an International Symposium on Management of Radioactive Wastes from the Nuclear Fuel Cycle. Vol. 2. IAEA, Vienna, pp. 317–338.Google Scholar
  22. Elderfield, H., and A. Hepworth. 1975. Diagenesis, metals and pollution in estuaries. Mar, Pollut. Bull. 6, 85–87.CrossRefGoogle Scholar
  23. Farges, L., F. Patti, R. Gros, and P. Bourgeon. 1974. Activité du krypton-85 dans l’air hemispheres nord et sud. J. Rad. Chem. 22, 147–155.CrossRefGoogle Scholar
  24. Folsom, T. R., and C. Sreekumarau. 1970. Some reference methods for determining radioactive and natural cesium for marine studies. In: Reference Methods for Marine Radioactivity Studies. Tech. Rep. Ser. No. 118, IAEA, Vienna, pp. 129–186.Google Scholar
  25. Garrett, C. 1979. Mixing in the ocean interior. Dynam. Atmos. Ocean 3, 239–265.CrossRefGoogle Scholar
  26. Goldberg, E. D., V. T. Bowen, J. W. Farrington, G. Harvey, J. M. Martin, P. L. Parker, R. W. Risebrough, W. Robertston, E. Schneider, and E. Gamble. 1978. The mussel watch. Environ. Conserv. 5, 101–125.CrossRefGoogle Scholar
  27. Hardy, E. P., P. W. Krey, and H. L. Volchok. 1973. Global inventory and distributions of fallout plutonium. Nature (London) 241, 444–445.CrossRefGoogle Scholar
  28. Hetherington, J. A. 1976. The behavior of plutonium radionuclides in the Irish Sea. In: Environmental Toxicity of Aquatic Radionuclides: Models and Mechanisms. Ann Arbor Science Publishers, Ann Arbor, Mich., pp. 81–106.Google Scholar
  29. Hetherington, J. A., D. F. Jefferies, and M. B. Lovett. 1976a. Some investigations into the behavior of plutonium in the marine environment. In: Radiological Impacts of Releases from Nuclear Facilities into Aquatic Environments. IAEA, Vienna, pp. 193–212.Google Scholar
  30. Hetherington, J. A., D. F. Jefferies, N. T. Mitchell, R. J. Pentreath, and D. S. Woodhead. 1976b. Environmental and public health consequences of the controlled disposal of transuranic elements to the marine environment. In: Transuranium Nuclides in the Environment. IAEA, Vienna, pp. 139–154.Google Scholar
  31. Holland, W. R., and P. B. Rhines. 1980. An example of eddy-induced ocean circulation. J. Phys. Oceanogr. 10, 1010–1031.CrossRefGoogle Scholar
  32. IAEA (International Atomic Energy Agency). 1970. Reference Methods for Marine Radioactivity Studies. Tech. Rep. Ser. No. 118, IAEA, Vienna.Google Scholar
  33. IAEA (International Atomic Energy Agency). 1976. Transuranium Nuclides in the Environment. IAEA, Vienna, IAEA-SM-199.Google Scholar
  34. IAEA (International Atomic Energy Agency). 1978. The radiological basis of the IAEA revised definition and recommendations concerning high level waste unsuitable for dumping at sea. Tech. Doc. 211, IAEA, Vienna.Google Scholar
  35. Jenkins, W. J. 1977. Tritium-helium dating in the Sargasso Sea: a measurement of oxygen utilization rates. Science 196, 291–292.CrossRefGoogle Scholar
  36. Jenkins, W. J. 1980. Tritium and 3He in the Sargasso Sea. J. Mar. Res. 38(3), 533–569.Google Scholar
  37. Jenkins, W. J., and W. B. Clarke. 1976. The distribution of 3He in the western Atlantic ocean. Deep-Sea Res. 23, 481–494.Google Scholar
  38. Jenkins, W. J., and P. B. Rhines. 1980. Tritium in the Deep North Atlantic Ocean. Nature 286(5776), 877–880.CrossRefGoogle Scholar
  39. Joseph, A. B., P. F. Gustafson, I. R. Russell, E. A. Schuert, H. L. Volchok, and A. Tamplin. 1971. Sources of radioactivity and their characteristics. In: Radioactivity in the Marine Environment (A. H. Seymour, Ed.). U.S. Natl. Acad. Sci., Natl. Res. Council, Washington, D.C., pp. 6–41.Google Scholar
  40. Kautsky, H. 1977. Stromungen in der Nordsee. Umschau Kurzberichte 77, 672–673.Google Scholar
  41. Kigoshi, K. 1962. Krypton-85 in the atmosphere. Bull. Chem. Soc. Japan 35, 1014–1016.CrossRefGoogle Scholar
  42. Koide, M., J. J. Griffin, and E. D. Goldberg. 1975. Records of plutonium fallout in marine and terrestrial samples. J. Geophys. Res. 30, 4153–4162.CrossRefGoogle Scholar
  43. Kuo, H. H., and G. Veronis. 1970. The distribution of tracers in the deep oceans of the world. Deep-Sea Res. 17, 29–46.Google Scholar
  44. Labeyrie, L. D., H. D. Livingston, and V. T. Bowen. 1976. Comparison of the distributions in marine sediments of the fallout-derived nuclides 55Fe and 239–240pu a new approach to the chemistry of environmental radionuclides. In: Transuranium Nuclides in the Environment. IAEA, Vienna, pp. 121–137.Google Scholar
  45. Livingston, H. D., and V. T. Bowen. 1976. Americium in the marine environment—relationships to plutonium. In: Environmental Toxicity of Aquatic Radionuclides: Models and Mechanisms (M. W. Miller and J. N. Stannard, Eds.). Ann Arbor Science Publishers, Ann Arbor, Mich., pp. 107–130.Google Scholar
  46. Livingston, H. D., and V. T. Bowen. 1977. Windscale effluent in the sediments and waters of the Minch. Nature (London) 269, 586–588.CrossRefGoogle Scholar
  47. Livingston, H. D., and V. T. Bowen. 1979. Pu and 137Cs in coastal sediments. Earth Planet. Sci. Lett. 43, 29–45.CrossRefGoogle Scholar
  48. Livingston, H. D., D. L. Schneider, and V. T. Bowen. 1975. 241 Pu in the marine environment by a radiochemical procedure. Earth Planet. Sci. Lett. 25, 361–367.CrossRefGoogle Scholar
  49. Livingston, H. D., V. T. Bowen, and S. L. Kupferman. 1982. Radionuclides from Windscale discharges I: nonequilibrium experiments in high latitude oceanoggraphy. J. Mar. Res. 40, 253–271.Google Scholar
  50. Loosli, H. H., and H. Oeschger. 1978. 39Ar, 14C and 85Kr measurements in groundwater samples. In: Intl. Symp. Isotope Hydrology. IAEA-SM-228/50.Google Scholar
  51. Luykx, F., and G. Fraser. 1978. Radioactive effluents from nuclear power stations and nuclear fuel reprocessing plants in the European Community: discharge data 1972–76 radiological aspects. Health and Safety Directorate, Comm. Europ. Comm., Rep. EVR 6088, EN, RF.Google Scholar
  52. Mitchell, N. T. 1977. Radioactivity in surface and coastal waters of the British Isles, 1976. Pt. 1: The Irish Sea and its environs. Ministry Agr. Food and Fish., Fisheries Radiobiol. Lab. Lowestoft, Tech. Rep., FRL 13.Google Scholar
  53. Miyake, Y. 1963. Artificial radioactivity in the sea. In: The Sea, Vol. 2. Inter- science Publishers, New York, pp. 78–87.Google Scholar
  54. Munk, W. 1966. Abyssal recipes. Deep-Sea Res. 13, 707–730.Google Scholar
  55. Munnich, K. O., and W. Roether. 1967. Transfer of bomb C-14 and tritium from the atmosphere into the ocean: internal mixing of the ocean on the basis of tritium and C-14 profiles. In: Radioactive Dating and Methods of Low Level Counting. IAEA, Vienna, pp. 93–117.Google Scholar
  56. Murray, C. N., H. Kautsky, M. Hoppenheit, and M. Damian. 1978. Actinide activities in water entering the northern North Sea. Nature (London) 276, 225–230.CrossRefGoogle Scholar
  57. Needier, G. T. 1979. Comments on high latitude processes for ocean climate modelling. Dynam. Atmos. Oceans 3, 231–237.CrossRefGoogle Scholar
  58. Noshkin, V. E., and V. T. Bowen. 1973. Concentrations and distributions of long-lived fallout radionuclides in open-ocean sediments. In: Radioactive Contamination of the Marine Environment. IAEA, Vienna, pp. 671–686.Google Scholar
  59. Noshkin, V. E., K. M. Wong, R. J. Eagle, and C. Gatrousis. 1975. Transuranic and other radionuclides in Bikini Lagoon: concentration data retrieved from aged coral sections. Limnol. Oceanogr. 20, 729–742.CrossRefGoogle Scholar
  60. Noshkin, V. E., K. M. Wong, T. A. Jokela, R. J. Eagle, and J. L. Brunk. 1978. Radionuclides in the marine environment near the Farallon Islands. Lawrence Livermore Laboratory Report UCRL 52381, 1–17.Google Scholar
  61. Nozaki, Y., J. Thomson, and K. K. Turekian. 1976. The distributions of 210Pb and 210Po in the surface waters of the Pacific Ocean. Earth Planet. Sci. Lett. 32,304–321.CrossRefGoogle Scholar
  62. Oeschger, H., U. Sieganthaler. U. Schotterer, and A. Gugelmann. 1975. A box diffusion model to study the carbon dioxide exchange in nature. Tellers 27, 168–192.Google Scholar
  63. Östlund, H. G., and M. Stuiver. 1980. GEOSECS Pacific radiocarbon. Radiocarbon 22, 25–53Google Scholar
  64. Östlund, H. G., H. G. Dorsey, and C. G. Rooth. 1974. GEOSECS North Atlantic radiocarbon and tritium results. Earth Planet Sci. Lett. 23, 69–86.CrossRefGoogle Scholar
  65. Östlund, H. G., H. G. Dorsey, R. Brescher, and W. H. Peterson. 1977. Tritium Laboratory Data Report No. 6. University of Miami, RSMAS.Google Scholar
  66. Rooth, C. G., and H. G. Östlund. 1972. Penetration of tritium into the Atlantic thermocline. Deep-Sea Res. 19, 481–492.Google Scholar
  67. Pannetier, R. 1970. Original use of the radioactive tracer gas krypton-85 to study meridian atmospheric flow. J. Geophys. Res. 75, 2985–2989.CrossRefGoogle Scholar
  68. Schroder, J. 1975. Krypton-85 in the ocean. Z. Naturforsch. 30a, 962–967.Google Scholar
  69. Stuiver, M., and H. G. Östlund. 1980. GEOSECS Atlantic radiocarbon. Radiocarbon 22, 1–24.Google Scholar
  70. Stuiver, M., and P. D. Quay. 1980. Changes in atmospheric carbon-14 attributed to a variable sun. Science 207, 11–19.CrossRefGoogle Scholar
  71. Sugihara, T. T., and V. T. Bowen. 1962. Radioactive rare earths from fallout for study of particle movement in the sea. In: Radioisotopes in the Physical Sciences and Industry. IAEA, Vienna, pp. 57–65.Google Scholar
  72. Telegadas, K., and G. J. Ferber. 1975. Atmospheric concentrations and inventory of krypton-85 in 1973. Science 190, 882–883.Google Scholar
  73. Templeton, W. L. 1980. Artificial radionuclides in the oceans. In: Oceanography, The Past (M. Sears and D. Merriman, Eds.). Springer-Verlag, New York, pp.420–437.Google Scholar
  74. Toonkel, L. E. 1980. Quarterly 90Sr deposition at world land sites. Appendix A, in Environmental Quarterly Report EML-370, Environmental Measurements Laboratory, U.S. Department of Energy, New York, A-3.Google Scholar
  75. Volchok, H. L., V. T. Bowen, T. R. Folsom, W. S. Broecker, E. A. Schuert, and G. S. Bien. 1971. Oceanic distributions of radionuclides from nuclear explosions. In: Radioactivity in the Marine Environment (A. H. Seymour, Ed.). U.S. Natl. Acad. Sci., Natl. Res. Council, Washington, D.C., pp. 42–89.Google Scholar
  76. Weiss, W. M., K-H. Fischer, B. Kromer, W. Roether, H. Lehn, W. B. Clarke, and Z. Top. 1978. Gas exchange with the atmosphere and internal mixing of Lake Constance (Obersee). Verhandlungen der Gesellschaft für Ökologie, Keil, pp. 153–161.Google Scholar
  77. Weiss, W. M., W. Roether, and E. Dreisigacker. 1979. Tritium in the North Atlantic Ocean-Inventory, input and transfer into deep water. In: Behavior of Tritium in the Environment. IAEA-SM-232/98, Vienna, pp. 315–336.Google Scholar
  78. Williams, P. M., M. C. Stenhouse, E. M. Druffel, and M. Koide. 1978. Organic 14C activity in an abyssal marine sediment. Nature (London) 276, 698–701.CrossRefGoogle Scholar
  79. Wong, K. M., C. S. Brown, and V. E. Noshkin. 1978. A rapid procedure for plu- tonium separation in large volumes of fresh and saline water by manganese dioxide co-precipitation. J. Radioanal. Chem. 42, 7–15.CrossRefGoogle Scholar
  80. Zander, I., and R. Araskog. 1973. Nuclear explosions 1945–1972, basic data. Res. Inst, of National Defense, Sweden FOA4, Rep. A4505-A1, 56 pp.Google Scholar

Copyright information

© Springer-Verlag New York Inc. 1983

Authors and Affiliations

  • Hugh D. Livingston
  • William J. Jenkins

There are no affiliations available

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