Nonsequential Multiple Ionization in Strong Laser Fields

  • H. Rottke
Part of the Springer Series on Atomic, Optical, and Plasma Physics book series (SSAOPP, volume 35)

Abstract

In 1965, it was experimentally observed that photoionization of an atom through absorption of many photons with an energy fh smaller than the ionization threshold is possible if only the light intensity is chosen high enough [1] . The formation of doubly charged ions in multiphoton ionization was first observed for alkaline-earth atoms with two electrons outside of closed shells [2] and later also for rare-gas atoms irradiated with Nd:YAG laser light [3] . The light intensity necessary to observe multiple ionization is in the 1013 W/cm2 range and higher. This intensity corresponds to an electric field strength of at least 108 V/cm in the wave. At these field strengths, the light—atom interaction can no longer be characterized by perturbation theoretical methods since the external electric field approaches the Coulomb field the valence electrons are exposed to in an atom. Soon after its observation the question arose whether double ionization is a stepwise process [4]:
$$ A + {n_1}w \to {A^ + } $$
(18.1a)
$$ {A^ + } + {n_2}w \to {A^ + }^ + $$
(18.1b)
, or a direct one, where both electrons are removed simultaneously from the atom:
$$ A + nw \to {A^{ + + }} $$
(18.2)
.

Keywords

Momentum Distribution Light Wave Atomic Beam Double Ionization Multiple Ionization 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  1. 1.
    G.S. Voronov, N.B. Delone: Zh. Eksp. Teor. Fiz. 1, 42 (1965) [Sov. Phys. JETP 23, 54 (1966)]Google Scholar
  2. 2.
    I. Aleksakhin, N. Delone, I. Zapesochnyi, V. Suran: Zh. Eksp. Teor. Fiz. 76, 887 (1979) [Sov. Phys. JETP 49, 447 (1979)]ADSGoogle Scholar
  3. 3.
    A. l’Huillier, L.A. Lompre, G. Mainfray, C. Manus: Phys. Rev. Lett. 48, 1814 (1982)ADSCrossRefGoogle Scholar
  4. 4.
    A. l’Huillier, L.A. Lompre, G. Mainfray, C. Manus: Phys. Rev. A 27, 2503 (1983)ADSCrossRefGoogle Scholar
  5. 5.
    D.N. Fittinghoff, P.R. Bolton, B. Chang, K.C. Kulander: Phys. Rev. Lett. 69, 2642 (1992)ADSCrossRefGoogle Scholar
  6. 6.
    B. Walker, B. Sheehy, L.F. DiMauro, P. Agostini, K.J. Schafer, K.C. Kulander: Phys. Rev. Lett. 73, 1227 (1994) 7. V. Schmidt: Electron Spectrometry of Atoms using Synchrotron Radiation (Cambridge University Press, Cambridge 1997)Google Scholar
  7. 8.
    U. Eichmann, M. Dörr, H. Maeda, W. Becker, W. Sandner: Phys. Rev. Lett. 84, 3550 (2000)ADSCrossRefGoogle Scholar
  8. 9.
    P.B. Corkum: Phys. Rev. Lett. 71, 1994 (1993)ADSCrossRefGoogle Scholar
  9. 10.
    B. Walker, E. Mevel, B. Yang, P. Breger, J.P. Chambaret, A. Antonetti, L.F. DiMauro, P. Agostini: Phys. Rev. A 48, R894 (1993)ADSCrossRefGoogle Scholar
  10. 11.
    T. Weber, M. Weckenbrock, A. Staudte, O. Jagutzki, V. Mergel, F. Afaneh, G. Urbasch, M. Vollmer, H. Giessen, R. Dörner: Phys. Rev. Lett. 84, 443 (2000)ADSCrossRefGoogle Scholar
  11. 12.
    R. Moshammer, B. Feuerstein, W. Schmitt, A. Dorn, C.D. Schröter, J. Ullrich, H. Rottke, C. Trump, M. Wittmann, G. Korn, K. Hoffmann, W. Sandner: Phys. Rev. Lett. 84, 447 (2000)ADSCrossRefGoogle Scholar
  12. 13.
    T. Weber, H. Giessen, M. Weckenbrock, G. Urbasch, A. Staudte, L. Spielberger, O. Jagutzki, V. Mergel, M. Vollmer, R. Dörner: Nature 405, 658 (2000)ADSCrossRefGoogle Scholar
  13. 14.
    B. Feuerstein, R. Moshammer, D. Fischer, A. Dorn, C.D. Schröter, J. Deipenwisch, J.R. Crespo Lopez-Urrutia, C. Höhr, P. Neumayer, J. Ullrich, H. Rottke, C. Trump, M. Wittmann, G. Korn, W. Sandner: Phys. Rev. Lett. 87, 043003 (2001)Google Scholar
  14. 15.
    B. Witzel, N.A. Papadogiannis, D. Charalambidis: Phys. Rev. Lett. 85, 2268 (2000)ADSCrossRefGoogle Scholar
  15. 16.
    R. Lafon, J.L. Chaloupka, P.M. Paul, P. Agostini, K.C. Kulander, L.F. DiMauro: Phys. Rev. Lett. 86, 2762 (2001)ADSCrossRefGoogle Scholar
  16. 17.
    E.R. Peterson, P.H. Bucksbaum: Phys. Rev. A 64, 053405 (2001)Google Scholar
  17. 18.
    L.V. Keldysh: Zh. Éksp. Teor. Fiz. 47, 1945 (1964) [Sov. Phys. JETP 20, 1307 (1965)]Google Scholar
  18. 19.
    R.R. Freeman, P.H. Buchsbaum, H. Milchberg, S. Darack, D. Schumacher, M.E. Geusic: Phys. Rev. Lett. 59, 1092 (1987)ADSCrossRefGoogle Scholar
  19. 20.
    H. Rottke, B. Wolff, M. Brickwedde, D. Feldmann, K.H. Welge: Phys. Rev. Lett. 64, 404 (1990)ADSCrossRefGoogle Scholar
  20. 21.
    P. Agostini, F. Fabre, G. Mainfray, G. Petite, N.K. Rahman: Phys. Rev. Lett. 42, 1127 (1979) ,)ADSCrossRefGoogle Scholar
  21. 22.
    A.M. Perelomov, V.S. Popov, M.V. Terent’ev: Zh. Eksp. Teor. Fiz. 50, 1393 (1966) [Sov. Phys. JETP 23, 924 (1966)] ,)Google Scholar
  22. 23.
    A.M. Perelomov, V.S. Popov, M.V. Terent’ev: Zh. Eksp. Teor. Fiz. 51, 309 (1966) [Sov. Phys. JETP 24, 207 (1967)];Google Scholar
  23. 23a.
    A.M. Perelomov, V.S. Popov: Zh. Eksp. Teor. Fiz. 52, 514 (1967) [ibid. 25, 336 (1967)];Google Scholar
  24. 23b.
    V.S. Popov, V.P. Kuznetsov, A.M. Perelomov: Zh. Eksp. Teor. Fiz. 53, 331 (1967) [ibid. 26, 222 (1967)]Google Scholar
  25. 24.
    G.L. Yudin, M.Y. Ivanov: Phys. Rev. A 63, 033404 (2001); M.V. Ammosov, N.B. Delone, V.P. Krainov: Zh. Eksp. Teor. Fiz. 91, 2008 (1986) [Sov. Phys. JETP 64, 1191 (1986)];Google Scholar
  26. 24a.
    N.B. Delone, V.P. Krainov: J. Opt. Soc. Am. B 8, 1207 (1991)ADSCrossRefGoogle Scholar
  27. 25.
    G.L. Yudin, M.Y. Ivanov: Phys. Rev. A 64, 013409 (2001)Google Scholar
  28. 26.
    G.G. Paulus, W. Nicklich, H. Xu, P. Lambropoulos, H. Walther: Phys. Rev. Lett. 72, 2851 (1994)ADSCrossRefGoogle Scholar
  29. 27.
    G.G. Paulus, W. Becker, W. Nicklich, H. Walther: J. Phys. B: At. Mol. Opt. Phys. 27, L703 (1994)ADSCrossRefGoogle Scholar
  30. 28.
    W. Becker, A. Lohr, M. Kleber: J. Phys. B: At. Mol. Opt. Phys. 27, L325 (1994)ADSCrossRefGoogle Scholar
  31. 29.
    B. Yang, K.J. Schafer, B. Walker, K.C. Kulander, P. Agostini, L.F. DiMauro: Phys. Rev. Lett. 71, 3770 (1993)ADSCrossRefGoogle Scholar
  32. 30.
    A. McPherson, G. Gibson, H. Jara, U. Johann, T.S. Luk, I. McIntyre, K. Boyer, C.K. Rhodes: J. Opt. Soc. Am. B 4, 595 (1987)ADSCrossRefGoogle Scholar
  33. 31.
    M. Ferray, A. L’Huillier, X.F. Li, L.A. Lompré, G. Mainfray, C. Manus: J. Phys. B: At. Mol. Opt. Phys. 21, L31 (1988)ADSCrossRefGoogle Scholar
  34. 32.
    M. Lewenstein, P. Balcou, M.Y. Ivanov, A. L’Huillier, P.B. Corkum: Phys. Rev. A 49, 2117 (1994)ADSCrossRefGoogle Scholar
  35. 33.
    J.D. Jackson: Classical Electrodynamics, 3rd edn. (John Wiley & Sons, Inc., New York 1999) p. 580MATHGoogle Scholar
  36. 34.
    T.W.B. Kibble: Phys. Rev. Lett. 16, 1054 (1966)ADSCrossRefGoogle Scholar
  37. 35.
    P. Mulser: J. Opt. Soc. Am. B 2, 1814 (1985)ADSCrossRefGoogle Scholar
  38. 36.
    W. Becker, R.R. Schlicher, M.O. Scully, K. Wódkiewicz: J. Opt. Soc. Am. B 4, 743 (1987)ADSCrossRefGoogle Scholar
  39. 37.
    P.H. Bucksbaum, R.R. Freeman, M. Bashkansky, T.J. Mcllrath: J. Opt. Soc. Am. B 4, 760 (1987)ADSCrossRefGoogle Scholar
  40. 38.
    R. Moshammer, B. Feuerstein, D. Fischer, A. Dorn, C.D. Schröter, J. Deipenwisch, J.R. Crespo Lopez-Urrutia, C. Höhr, P. Neumayer, J. Ullrich, H. Rottke, C. Trump, M. Wittmann, G. Korn, W. Sandner: Opt. Express 8, 358 (2001)ADSCrossRefGoogle Scholar
  41. 39.
    D.R. Miller: Free Jet Sources. In: Atomic and Molecular Beam Methods, Vol. 1, ed. by G. Scoles (Oxford University Press, Oxford 1988)Google Scholar
  42. 40.
    F. Lindner et al.: submittedGoogle Scholar
  43. 41.
    E. Eremina, H. Rottke, W. Sandner, A. Dreischuh, F. Lindner, F. Grasbon, G.G. Paulus, H. Walther, R. Moshammer, B. Feuerstein, J. Ullrich: submitted for publicationGoogle Scholar
  44. 42.
    T. Weber, M. Weckenbrock, A. Staudte, L. Spielberger O. Jagutzki, V. Mergel, F. Afaneh, G. Urbasch, M. Vollmer, H. Giessen, R. Dörner: J. Phys. B: Atomic, Molec. Opt.Phys. 33, L127 (2000)ADSCrossRefGoogle Scholar
  45. 43.
    M. Weckenbrock, M. Hattass, A. Czasch, O. Jagutzki, L. Schmidt, T. Weber, H. Roskos, T. Löffler, M. Thomson, R. Dörner: J. Phys. B: Atomic, Molec. Opt. Phys. 34, L449 (2001)ADSCrossRefGoogle Scholar
  46. 44.
    R. Moshammer, B. Feuerstein, J. Crespo Lopez-Urrutia, J. Deipenwisch, A. Dorn, D. Fischer, C. Höhr, P. Neumayer, C. D. Schröter, J. Ullrich, H. Rottke, C. Trump, M. Wittmann, G. Korn, W. Sandner: Phys. Rev. A65, 035401 (2992)Google Scholar
  47. 45.
    D.N. Fittinghoff, P.R. Bolton, B. Chang, K.C. Kulander: Phys. Rev. A 49, 2174 (1994)ADSCrossRefGoogle Scholar
  48. 46.
    P. Dietrich, N.H. Burnett, M. Ivanov, P.B. Corkum: Phys. Rev. A50, R3585 (1994)ADSCrossRefGoogle Scholar
  49. 47.
    V.R. Bhardwaj, S.A. Aseyev, G.L. Yudin, D.M. Villeneuve, D.M. Rayner, M.Yu. Ivanov, P.B. Corkum: Phys. Rev. Lett. 86, 3522 (2001)ADSCrossRefGoogle Scholar
  50. 48.
    N.B. Delone, V.P. Krainov: Uspekhi Fiz. Nauk 168, 531 (1998) [Physics— Uspekhi 41, 469 (1998)]CrossRefGoogle Scholar
  51. 49.
    A.I. Nikishov, V.I. Ritus: Zh. Eksp. Teor. Fiz. 50, 255 (1966) [Sov. Phys. JETP 23, 162 (1966)]Google Scholar
  52. 50.
    R. Kopold, W. Becker, H. Rottke, W. Sandner: Phys. Rev. Lett. 85, 3781 (2000)ADSCrossRefGoogle Scholar
  53. 51.
    S.P. Goreslavskii S.V. Popruzhenko, R. Kopold, W. Becker: Phys. Rev. A 64, 053402 (2001)Google Scholar
  54. 52.
    S.P. Goreslavskii, S.V. Popruzhenko: Opt. Express 8, 395 (2001)ADSCrossRefGoogle Scholar
  55. 53.
    A. Talebpour, S. Larochelle, S.L. Chin: J. Phys. B: Atomic, Molec. Opt. Phys. 30, L245 (1997)ADSCrossRefGoogle Scholar
  56. 54.
    C. Cornaggia, P. Hering: J. Phys. B: Atomic, Molec. Opt. Phys. 31, L503 (1998)ADSCrossRefGoogle Scholar
  57. 55.
    C. Cornaggia, P. Hering: Phys. Rev. A 62, 023403 (2000)Google Scholar

Copyright information

© Springer-Verlag Berlin Heidelberg 2003

Authors and Affiliations

  • H. Rottke

There are no affiliations available

Personalised recommendations