The Role of Convection in the Vertical Distribution of Ozone and Precursors in the Troposphere

  • Øystein Hov
  • Frode Flatøy
  • Asbjørn Strand
Conference paper
Part of the NATO ASI Series book series (volume 32)

Abstract

Strand and Hov (1994b) have estimated that the amount of NOx injected in the free troposphere by rapid transport from the planetary boundary layer in connection with convective clouds and frontal circulation is about 0.6 TgN/yr, and in addition about the same amount of other NOy compounds is injected. For comparison, the various sources at the ground total 34 TgN/yr of NOx. The strength of the lightning source was assumed to be 3 TgN/yr. The total release of NOx from aircraft is reported to be 0.58 TgN/yr. NOx transported downwards from the stratosphere where it is formed through the decomposition of N2O has been estimated to contribute about 0.34 TgN/yr. In a 3-D mesoscale chemistry model for Europe during the time period July 1 to 10, 1991, NOx brought to the upper troposphere by convective transport was calculated to be the dominant contributor to the chemical formation of ozone there, while aircraft emissions of NOx also made a significant contribution. Without aircraft or convective NOx in the upper troposphere the in-situ ozone formation was calculated to be modest.

Keywords

Atmospheric Boundary Layer Planetary Boundary Layer Lower Troposphere Convective Cloud Tropospheric Ozone 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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References

  1. Flatøy, F., Ø. Hov and H. Smit (1994) 3-D model studies of vertical exchange processes of ozone in the troposphere over Europe. Submitted to J. Geophys. Res.Google Scholar
  2. Grennfelt, P., Ø. Hov and R. G. Derwent (1994) Second generation abatement strategies for Nox, NH3, SO2 and VOC. Ambio 23, 425–433.Google Scholar
  3. Holton, J. R. (1992) An introduction to dynamic meteorology, 3rd edition. Academic Press, New York, 511 pp.Google Scholar
  4. Iversen, T., N. E. Halvorsen, S. Mylona and H. Sandnes (1991) Calculated budgets for airborne acidifying components in Europe. EMEP/MSC-W Report 1/91, The Norwegian Meteorological Institute, P.O. Box 43-Blindern, N-0313 Oslo, Norway.Google Scholar
  5. Mahlman, J. D. and W. J. Moxim (1978) Tracer Simulation using a global general circulation model: results from a midlatitude instantaneous source experiment. J. Atmos. Sci., 35, 1340–1374.CrossRefGoogle Scholar
  6. McInnes, G. and C. T. Walker (1992) The global distribution of aircraft air pollutant emissions. Warren Spring Laboratory, report LR 872 (AP), Stevenage Hertfordshire SG1 2BX, England.Google Scholar
  7. Pleim, P. E. and J. S. Chang (1992) A non-local closure model for vertical mixing in the convective boundary layer. Atmospheric Environment, 26, 965–981.CrossRefGoogle Scholar
  8. Plumb, R. A. and J. D. Mahlman (1987) The zonally averaged transport characteristics of the GFDL general circulation/transport model. J. Atmos. Sci., 44, 298–327.CrossRefGoogle Scholar
  9. Strand, A. and Ø. Hov (1993) A two-dimensional zonally averaged transport model including convective motions and a new strategy for the numerical Solution. J. Geophys. Res., 98, 9023–9037.CrossRefGoogle Scholar
  10. Strand, A. and Ø. Hov (1994a) Two-dimensional global study of the tropospheric ozone produetion. J. Geophys. Res., 99D, 22877–22895.CrossRefGoogle Scholar
  11. Strand, A. and Ø. Hov (1994b) The impact of man-made and natural Nox on Upper tropospheric ozone: A two-dimensional model study. Submitted to Atmospheric Environment.Google Scholar
  12. WMO (1994) WMO-UNEP Ozone assessment.Google Scholar

Copyright information

© Springer-Verlag Berlin Heidelberg 1995

Authors and Affiliations

  • Øystein Hov
    • 1
    • 2
  • Frode Flatøy
    • 1
  • Asbjørn Strand
    • 1
    • 2
  1. 1.Geophysics InstituteBergenNorway
  2. 2.Nansen Environmental and Remote Sensing CenterSolheimsvik-BergenNorway

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