Regional Modelling of Tropospheric Ozone

  • David Simpson
  • Jan Eiof Jonson

Abstract

Atmospheric transport and chemistry models are an essential part of assessing ozone abatement. Such models allow a quantification of both the levels of ozone concentration across the whole of Europe, and of the relative effectiveness of different control measures. In this study, two photochemical models of the European Monitoring and Evaluation Programme (EMEPl) have been used to investigate the effects of emission control scenarios and to assess the contribution of specific source sectors to ozone formation over Europe. In a first step, the status quo of ozone concentrations was calculated for the base year 1990 and the trend scenario 2010, showing that even though precursor emissions were reduced significantly, ozone thresholds were exceeded to a large extent. Data from these models were also used as inputs for the emission-optimisation (Chap. 7), economic evaluation (Chap.s 9 & 10), and for more local modelling (Chap. 8). An important application of the Lagrangian model was the provision of sourcereceptor-matrices for the optimisation by the means of calculating matrices to relate emissions to ozone formation for a 5-year average (see Sect. 6.5).

Keywords

Tropospheric Ozone Ozone Formation Lagrangian Model Eulerian Model Biogenic Emission 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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References

  1. Amann M et al (1999), Final report on work done under EU acidification and ozone strategy. International Institute for Applied Systems Analysis (IIASA), Laxenburg, AustriaGoogle Scholar
  2. Andersson-Sköld Y and Simpson D (1999), Comparison of the chemical schemes of the EMEP MSC-W and the IVL photochemical trajectory models. In: Atmospheric Environment, 33, 1111–1129CrossRefGoogle Scholar
  3. DeMore, W.B. et al. (1997) Chemical kinetics and photochemical data for use in stratospheric modelling, JPL Publication 97–4.Google Scholar
  4. Derwent, R.G., Jenkin, M.E., Saunders, S.M. (1996) Photochemical ozone creation potentialsfor a large number of reactive hydrocarbons under European conditions, Atmos. Environ., 30, 189–200.Google Scholar
  5. Eliassen, A., Hov, O., Isaksen, I.S.A., Saltbones, J. and Stordal, F. (1982) A Lagrangian long- range transport model with atmospheric boundary layer chemistry, J. Appl. Met., 21, 1645–1661.CrossRefGoogle Scholar
  6. EMEP MSC-W (1998) Transboundary photooxidant air pollution in Europe. Calculations of tropospheric ozone and comparison with observations. Norwegian Meteorological Institute, Oslo, NorwayGoogle Scholar
  7. Fuhrer, J., Skarby, L., and Ashmore, M.A. (1997) Critical levels for ozone effects on vegetation in Europe, 1997, Environ. Poll., pp 91–96.Google Scholar
  8. Friedrich, R. (1993) Generation of time-dependent emission data, In P. Borrel et al., editor, Transport and Transformation of Polluntants in the Troposphere, Proceedings EUROTRAC symposium 1992, pages 255–268Google Scholar
  9. Friedrich, R., Reis, S., Voehringer, F., Simpson, D., Moussiopoulos, N., Salmons, R., and Papameletiou, D. (1998) Efficient ozone abatement strategies in Europe, in Transport and Chemical Transformation of Pollutants in the Troposphere, Proceedings EUROTRAC symposium 1998.Google Scholar
  10. Hass, H., Builtjes, P.J.H., Simpson, D., and Stern, R. (1997) Comparison of model results obtained with several European regional air quality models, Atmos. Environ., 31, No. 19, 3259–3279CrossRefGoogle Scholar
  11. Jenkin, M.E., Saunders, S.M. and Pilling, M.J. (1997) The tropospheric degredation of volatile organic compounds: a protocol for mechanism development, Atmos. Environ., 31, 81–104.CrossRefGoogle Scholar
  12. Jonson, J.E., Jakobsen, H.A., and Berge, E. (1997) Status of the development of the regional scale photo-chemical multi-layer eulerian model, Norwegian Meteorological Institute, EMEP MSC-W Note 2/97Google Scholar
  13. Jonson, J.E., Tarrason, L., Sundet, J., Berntsen, T., and Unger, S. (1998) The Eulerian 3-D oxidant model: status and evaluation for summer 1996 results and case-studies, In EMEP MSC-W Report 2/98, Part IIGoogle Scholar
  14. Jonson, J.E., Tarrason, L., and Sundet, J. (1999) Calculation of ozone and other pollutants for the summer 1996, Env. Manage, and Health, in press Google Scholar
  15. Kuhn, M., Builtjes, P.J.H., Poppe, D., Simpson, D., Stockwell, W.R., Andersson-Skold, Y., Baart, A., Das, M., Fiedler, F., Hov, O., Kirchner, F., Makar, P.A., Milford, J.B., Roemer, M.G.M., Ruhnke, R., Strand, A., Vogel, B., and Vogel, H. (1998) Intercomparison of the gas- phase chemistry in several chemistry and transport models, Atmos. Environ., 32, No. 4, 693–709CrossRefGoogle Scholar
  16. LAT (1997) Laboratory of Applied Thermodynamicy, University of Thessaloniki, Methodologies for Estimating Air Pollutant Emissions from Transport—Road Traffic Composition, Task 2.2/Deliverable 16, LAT Report No. 9718, Thessaloniki, August 1997Google Scholar
  17. LAT (1998) Laboratory of Applied Thermodynamicy, University of Thessaloniki, Methodologies for Estimating Air Pollutant Emissions from Transport—Emission Factors and Traffic Characteristics Data Set, Deliverable 21, LAT Report No. 9802 Thessaloniki, January 1998Google Scholar
  18. Middleton, P., Stockwell, W.R. and Carter, W.P.L. (1990) Aggregation and analysis of volatile organic compound emissions for regional modeling, Atmos. Environ., 24A, No. 5, 1107–1133.Google Scholar
  19. Moussiopoulos, N., S ahm P., Tourlou, M., Friedrich, R., Simpson, D., Lutz, M. (1999) Development and evaluation of ozone abatement strategies on urban scale air quality, 8th International Symposium Transport and Air Pollution, Graz, Austria.Google Scholar
  20. Pleim, J. E. and Ching, J.K.S. (1993) Interpretative analysis of observed and modeled mesoscale ozone photochemistry in area with numerous point sources, Atmos. Environ., 27A, 999–1017.Google Scholar
  21. Reis, S., Simpson, D., Friedrich, R., Jonson, J.E., Unger, S., and Obermeier, A. (1999) Road traffic emissions—predictions of future contributions to regional ozone levels in Europe, 8th International Symposium Transport and Air Pollution, Graz, Austria.Google Scholar
  22. Sillman, S., Logan, A., and Wofsy, S.C. (1990) The sensitivity of ozone to nitrogen oxides and hydrocarbons in regional ozone episodes, J. Geophys. Res., 20, 1837–1851.CrossRefGoogle Scholar
  23. Simpson, D. (1992a) Long period modelling of photochemical oxidants in Europe. Calculations for July 1985, Atmos. Environ., 26A, No. 9, 1609–1634.Google Scholar
  24. Simpson, D. (1992b) Long period modelling of photochemical oxidants in Europe. A) Hydrocarbon reactivity and ozone formation in Europe. B) On the linearity of country-to-country ozone calculations in Europe, EMEP MSC-W Note 1/92, Norwegian Meteorological Institute, Oslo.Google Scholar
  25. Simpson, D. (1993) Photochemical model calculations over Europe for two extended summer periods: 1985 and 1989. Model results and comparisons with observations, Atmos. Environ., 21 A, No. 6, 921–943Google Scholar
  26. Simpson, D. (1995) Biogenic emissions in Europe 2: Implications for ozone control strategies, J. Geophys. Res., 100, No. Dil, 22891–22906.Simpson, D. and Andersson-Sköld, Y. (1997) Regional and local scale modelling of ozone in Europercalculations for the EU Auto/Oil Programme. Norwegian Meteorological Institute, Research Report No. 47, Oslo, Norway.CrossRefGoogle Scholar
  27. Simpson, D. and Jonson, J.E. (1998) Comparison of Lagrangian and Eulerian models for the summer of 1996, In EMEP MSC-W Report 2/98, Part III, Transboundary photooxidant air pollution in Europe. Calculations of tropospheric ozone and comparison with observations. Norwegian Meteorological Institute, Oslo, NorwayGoogle Scholar
  28. Simpson, D. and Malik, S. (1996) Photochemical oxidant modelling and source-receptor relationships for ozone, In EMEP MSC-W Report 1/96, Norwgian Meteorological Institute, Oslo, Norway.Google Scholar
  29. Simpson, D., Guenther, A., Hewitt, C.N., and Steinbrecher, R. (1995) Biogenic emissions in Europe 1. Estimates and uncertainties, J. Geophys. Res., 100, No. Dil, 22875–22890CrossRefGoogle Scholar
  30. Simpson, D., Olendrzynski, K., Semb, A., Stören, E., and Unger, S. (1997) Photochemical oxidant modelling in Europe: multi-annual modelling and source-receptor relationships, Norwegian Meteorological Institute, EMEP MSC-W Report 3/97.Google Scholar
  31. Simpson, D., Altenstedt, J., and Hjellbrekke, A.G. (1998) The Lagrangian oxidant model: status and multi-annual evaluation, Part I in MSC-W (1998).Google Scholar
  32. Solberg, S., Dye, C., Schmidbauer, N., and Simpson, D. (1995) Evaluation of the VOC measurement programme within EMEP, Kjeller, Norway, Norwegian Institute for Air Research (NILU) Report 5/95.Google Scholar
  33. UN-ECE (1997) Health-effects of Ozone and Nitrogen Oxides in an Integrated Assessment of Air Pollution, Institute for Environment and Health, University of Leicester, Leicester, UK.Google Scholar

Copyright information

© Springer-Verlag Berlin Heidelberg 2000

Authors and Affiliations

  • David Simpson
  • Jan Eiof Jonson

There are no affiliations available

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