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Ultrafast dynamics of photoinduced processes at surfaces and interfaces

  • Christian Frischkorn
  • Martin Wolf
  • Ulrich Höfer
  • Jens Güdde
  • Peter Saalfrank
  • Mathias Nest
  • Tillmann Klamroth
  • Frank Willig
  • Ralph Ernstorfer
  • Lars Gundlach
  • Volkhard May
  • Luxia Wang
  • Walter R. Duncan
  • Oleg V. Prezhdo
Part of the Chemical Physics book series (CHEMICAL, volume 87)

Abstract

While femtochemistry in the gas and solution phase has led to enormous progress in the understanding and even control of chemical reactions over the past decades, a comparable level of sophistication in the analysis of surface chemical reactions has not been achieved.

Keywords

Potential Energy Surface Second Harmonic Generation Anchor Group Second Harmonic Generation Signal Heterogeneous Electron Transfer 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.

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References

  1. 1.
    A.M. Wodtke, J.C. Tully, D.J. Auerbach, Int. Rev. Phys. Chem. 23, 513 (2004)Google Scholar
  2. 2.
    H. Nienhaus, Surf. Sci. Rep. 45, 1 (2002)CrossRefGoogle Scholar
  3. 3.
    W. Ho, Acc. Chem. Res. 31, 567 (1998)CrossRefGoogle Scholar
  4. 4.
    C. Frischkorn, M. Wolf, Chem. Rev. 106, 4207 (2006)CrossRefGoogle Scholar
  5. 5.
    D.N. Denzler, C. Hess, S. Funk, G. Ertl, M. Bonn, C. Frischkorn, M. Wolf, in Femtochemistry and Femtobiology - Ultrafast dynamics in molecular science, ed. by A. Douhal, J. Santamaria (World Scientific, Singapore, 2002), p. 653Google Scholar
  6. 6.
    M.I. Kaganov, I.M. Lifshitz, L.V. Tanatarov, Sov. Phys. JETP 4, 173 (1957)Google Scholar
  7. 7.
    S.I. Anisimov, B.L. Kapeliovich, T.L. Perel'man, Sov. Phys. JETP 39, 375 (1974)Google Scholar
  8. 8.
    J. Hohlfeld, S.S. Wellershoff, J. Güdde, U. Conrad, V. Jähnke, E. Matthias, Chem. Phys. 251, 237 (2000)CrossRefGoogle Scholar
  9. 9.
    J. Hohlfeld, PhD thesis, Freie Universität Berlin (1998)Google Scholar
  10. 10.
    M. Lisowski, P.A. Loukakos, U. Bovensiepen, J. Stähler, C. Gahl, M. Wolf, Appl. Phys. A 78, 165 (2004)CrossRefGoogle Scholar
  11. 11.
    F. Budde, T.F. Heinz, A. Kalamarides, M.M.T. Loy, J.A. Misewich, Surf. Sci. 283, 143 (1993)CrossRefGoogle Scholar
  12. 12.
    M. Brandbyge, P. Hedegard, T.F. Heinz, J.A. Misewich, D.M. Newns, Phys. Rev. B 52, 6042 (1995)CrossRefGoogle Scholar
  13. 13.
    D.M. Newns, T.F. Heinz, J.A. Misewich, Prog. Theor. Phys. 106, 411 (1991)Google Scholar
  14. 14.
    D.M. Newns, Phys. Rev. 178, 1123 (1969)CrossRefGoogle Scholar
  15. 15.
    J.A. Misewich, T.F. Heinz, D.M. Newns, Phys. Rev. Lett. 68, 3737 (1992)CrossRefGoogle Scholar
  16. 16.
    D. Menzel, R. Gomer, J. Chem. Phys. 41, 3311 (1964)CrossRefGoogle Scholar
  17. 17.
    P.A. Redhead, Can. J. Phys. 42, 886 (1964)Google Scholar
  18. 18.
    P.R. Antoniewicz, Phys. Rev. B 21, 3811 (1980)CrossRefGoogle Scholar
  19. 19.
    F. Budde, T.F. Heinz, M.M.T. Loy, J.A. Misewich, F. de Rougemont, H. Zacharias, Phys. Rev. Lett. 66, 3024 (1991)CrossRefGoogle Scholar
  20. 20.
    J.A. Misewich, T.F. Heinz, A. Kalamarides, U. Höfer, M.M.T. Loy, J. Chem. Phys. 100, 736 (1994)CrossRefGoogle Scholar
  21. 21.
    L.M. Struck, L.J. Richter, S.A. Buntin, R.R. Cavanagh, J.C. Stephenson, Phys. Rev. Lett. 77, 4576 (1996)CrossRefGoogle Scholar
  22. 22.
    J.C.Tully, M. Gomez, M. Head-Gordon, J. Vac. Sci. Technol. A 11, 1914 (1993)CrossRefGoogle Scholar
  23. 23.
    M. Head-Gordon, J.C. Tully, J. Chem. Phys. 103, 10137 (1995)CrossRefGoogle Scholar
  24. 24.
    A.C. Luntz, M. Persson, J. Chem. Phys. 123, 074704 (2005)CrossRefGoogle Scholar
  25. 25.
    D.N. Denzler, C. Frischkorn, M. Wolf, G. Ertl, J. Phys. Chem. B 108, 14503 (2004)CrossRefGoogle Scholar
  26. 26.
    G. Ertl, H. Knözinger (eds.), Handbook of heterogeneous catalysis (VCH, Weinheim, 1997)Google Scholar
  27. 27.
    C.G.V. de Walle, J. Neugebauer, Nature 423, 626 (2003)CrossRefGoogle Scholar
  28. 28.
    K. Christmann, Prog. Surf. Sci. 48, 15 (1995)CrossRefGoogle Scholar
  29. 29.
    G.A. Somorjai, J. Phys. Chem. B 106, 9201 (2002)CrossRefGoogle Scholar
  30. 30.
    K. Christmann, Surf. Sci. Rep. 9, 1 (1988)CrossRefGoogle Scholar
  31. 31.
    D.N. Denzler, C. Frischkorn, C. Hess, M. Wolf, G. Ertl, Phys. Rev. Lett. 91, 226102 (2003)CrossRefGoogle Scholar
  32. 32.
    C.M. Mate, G.A. Somorjai, Phys. Rev. B 34, 7417 (1986)CrossRefGoogle Scholar
  33. 33.
    N. Takagi, Y. Yasui, T. Takaoka, M. Sawada, H. Yanagita, T. Aruga, M. Nishijima, Phys. Rev. B 53, 13767 (1996)CrossRefGoogle Scholar
  34. 34.
    C. Frischkorn, Surf. Sci. 593, 67 (2005)CrossRefGoogle Scholar
  35. 35.
    M. Bonn, S. Funk, C. Hess, D.N. Denzler, C. Stampfl, M. Scheffler, M. Wolf, G. Ertl, Science 285, 1042 (1999)CrossRefGoogle Scholar
  36. 36.
    M. Yada, R.J. Madix, Surf. Sci. 328, 171 (1995)CrossRefGoogle Scholar
  37. 37.
    H. Eyring, M. Polanyi, Z. Phys. Chem. B 12, 279 (1931)Google Scholar
  38. 38.
    L. Diekhöner, L. Hornekaer, H. Mortensen, E. Jensen, A. Baurichter, V.V. Petrunin, A.C. Luntz, J. Chem. Phys. 117, 5018 (2002)CrossRefGoogle Scholar
  39. 39.
    S. Wagner, C. Frischkorn, M. Wolf, M. Rutkowski, H. Zacharias, A. Luntz, Phys. Rev. B 72, 205404 (2005)CrossRefGoogle Scholar
  40. 40.
    K.W. Kolasinski, W. Nessler, A. de Meijere, E. Hasselbrink, Phys. Rev. Lett. 72, 1356 (1994)CrossRefGoogle Scholar
  41. 41.
    E. Hasselbrink, in Laser spectroscopy and photochemistry on metal surfaces, ed. by H.L. Dai, W. Ho (World Scientific, Singapore, 1995), p. 685Google Scholar
  42. 42.
    A.C. Luntz, M. Persson, S. Wagner, C. Frischkorn, M. Wolf, J. Chem. Phys. 124, 244702 (2006)CrossRefGoogle Scholar
  43. 43.
    J.C. Tully, J. Chem. Phys. 73, 1975 (1995)CrossRefGoogle Scholar
  44. 44.
    P.N.J. Persson, Sliding friction: Physical principles and applications (Springer, Berlin, 1998)Google Scholar
  45. 45.
    K.P. Bohnen, M. Kiwi, H. Suhl, Phys. Rev. Lett. 34, 1512 (1975)CrossRefGoogle Scholar
  46. 46.
    A. Nourtier, Journal De Physique 38, 479 (1977)Google Scholar
  47. 47.
    L. Bartels, F.Wang, D. Moller, E. Knoesel, T.F. Heinz, Science 305, 648 (2004)CrossRefGoogle Scholar
  48. 48.
    K. Stépán, J. Güdde, U. Höfer, Phys. Rev. Lett. 94, 236103 (2005)CrossRefGoogle Scholar
  49. 49.
    K. Stépán, M. Dürr, J. Güdde, U. Höfer, Surf. Sci. 593, 54 (2005)CrossRefGoogle Scholar
  50. 50.
    E.H.G. Backus, A. Eichler, A.W. Kleyn, M. Bonn, Science 310, 1790 (2005)CrossRefGoogle Scholar
  51. 51.
    H. Wang, R.G. Tobin, D.K. Lambert, C.L. DiMaggio, G.B. Fisher, Surf. Sci. 372, 267 (1997)CrossRefGoogle Scholar
  52. 52.
    A.T. Gee, B.E. Hayden, J. Chem. Phys. 113, 10333 (2000)CrossRefGoogle Scholar
  53. 53.
    J.L. Gland, B.A. Sexton, G.B. Fisher, Surf. Sci. 95, 587 (1980)CrossRefGoogle Scholar
  54. 54.
    A. Winkler, X. Guo, H.R. Siddiqui, P.L. Hagans, J.T. Yates, Surf. Sci. 201, 419 (1988)CrossRefGoogle Scholar
  55. 55.
    P. Gambardella, Z. Sljivancanin, B. Hammer, M. Blanc, K. Kuhnke, K. Kern, Phys. Rev. Lett. 87, 056103 (2001)CrossRefGoogle Scholar
  56. 56.
    Y.R. Shen, Annu. Rev. Phys. Chem. 40, 327 (1989)CrossRefGoogle Scholar
  57. 57.
    G.A. Reider, T.F. Heinz, in Photonic probes of surfaces, ed. by P. Halevi (North-Holland, Amsterdam, 1995), pp. 3–66Google Scholar
  58. 58.
    G. Lüpke, D.J. Bottomley, H.M. van Driel, J. Opt. Soc. Am. B 11, 33 (1994)CrossRefGoogle Scholar
  59. 59.
    P. Kratzer, E. Pehlke, M. Scheffer, M.B. Raschke, U. Höfer, Phys. Rev. Lett. 81, 5596 (1998)CrossRefGoogle Scholar
  60. 60.
    M.B. Raschke, U. Höfer, Phys. Rev. B 59, 2783 (1999)CrossRefGoogle Scholar
  61. 61.
    J.E. Reutt-Robey, D.J. Doren, Y.J. Chabal, S.B. Christman, J. Chem. Phys. 93, 9113 (1990)CrossRefGoogle Scholar
  62. 62.
    J. Güdde, U. Höfer, J. Phys.: Condens. Matter 18, S1409 (2006)CrossRefGoogle Scholar
  63. 63.
    P.J. Feibelman, S. Esch, T. Michely, Phys. Rev. Lett. 77, 2257 (1996)CrossRefGoogle Scholar
  64. 64.
    C.T. Campbell, G. Ertl, H. Kuipers, J. Segner, Surf. Sci. 107, 220 (1981)CrossRefGoogle Scholar
  65. 65.
    S. Deliwala, R.J. Finlay, J.R. Goldman, T.H. Her, W.D. Mieher, E. Mazur, Chem. Phys. Lett. 242, 617 (1995)CrossRefGoogle Scholar
  66. 66.
    D.G. Busch, W. Ho, Phys. Rev. Lett. 77, 1338 (1996)CrossRefGoogle Scholar
  67. 67.
    J.A. Prybyla, T.F. Heinz, J.A. Misewich, M.M.T. Loy, J.H. Glownia, Phys. Rev. Lett. 64, 1537 (1990)CrossRefGoogle Scholar
  68. 68.
    F.J. Kao, D.G. Busch, D. Cohen, D.G. Dacosta, W. Ho, Phys. Rev. Lett. 71, 2094 (1993)CrossRefGoogle Scholar
  69. 69.
    X.Y. Zhu, S.R. Hatch, A. Campion, J.M. White, J. Chem. Phys. 91, 5011 (1989)CrossRefGoogle Scholar
  70. 70.
    K. Watanabe, K. Sawabe, Y. Matsumoto, Phys. Rev. Lett. 76, 1751 (1996)CrossRefGoogle Scholar
  71. 71.
    M. Bauer, S. Pawlik, R. Burgermeister, M. Aeschlimann, Surf. Sci. 404, 62 (1998)CrossRefGoogle Scholar
  72. 72.
    S. Ogawa, H. Nagano, H. Petek, Phys. Rev. Lett. 82, 1931 (1999)CrossRefGoogle Scholar
  73. 73.
    M. Wolf, A. Hotzel, E. Knoesel, D. Velic, Phys. Rev. B 59, 5926 (1999)CrossRefGoogle Scholar
  74. 74.
    C. Lei, M. Bauer, K. Read, R. Tobey, Y. Liu, T. Popmintchev, M.M. Murnane, H.C. Kapteyn, Phys. Rev. B 66, 245420 (2002)CrossRefGoogle Scholar
  75. 75.
    K. Stépán, PhD thesis, Philipps-Universität Marburg (2006)Google Scholar
  76. 76.
    J. Wintterlin, R. Schuster, G. Ertl, Phys. Rev. Lett. 77, 123 (1996)CrossRefGoogle Scholar
  77. 77.
    A. Bogicevic, J. Stromquist, B.I. Lundqvist, Phys. Rev. B 57, R4289 (1998)CrossRefGoogle Scholar
  78. 78.
    U. Engström, R. Ryberg, Phys. Rev. Lett. 82, 2741 (1999)CrossRefGoogle Scholar
  79. 79.
    C. Puglia, A. Nilsson, B. Hernnas, O. Karis, P. Bennich, N. Martensson, Surf. Sci. 342, 119 (1995)CrossRefGoogle Scholar
  80. 80.
    A.C. Luntz, private communicationsGoogle Scholar
  81. 81.
    M. Bonn, D.N. Denzler, S. Funk, M. Wolf, S.S. Wellershoff, J. Hohlfeld, Phys. Rev. B 61, 1101 (2000)CrossRefGoogle Scholar
  82. 82.
    T. Komeda, Y. Kim, M. Kawai, B.N.J. Persson, H. Ueba, Science 295, 2055 (2002)CrossRefGoogle Scholar
  83. 83.
    J.I. Pascual, N. Lorente, Z. Song, H. Conrad, H.P. Rust, Nature 423, 525 (2003)CrossRefGoogle Scholar
  84. 84.
    B.N.J. Persson, H. Ueba, Surf. Sci. 502, 18 (2002)CrossRefGoogle Scholar
  85. 85.
    H. Ueba, T. Mii, N. Lorente, B.N.J. Persson, J. Chem. Phys. 123, 084707 (2005)CrossRefGoogle Scholar
  86. 86.
    B.N.J. Persson, R. Ryberg, Phys. Rev. Lett. 54, 2119 (1985)CrossRefGoogle Scholar
  87. 87.
    U. Engström, R. Ryberg, J. Chem. Phys. 112, 1959 (2000)CrossRefGoogle Scholar
  88. 88.
    W.S. Fann, R. Storz, H.W.K. Tom, J. Bokor, Phys. Rev. Lett. 68, 2834 (1992)CrossRefGoogle Scholar
  89. 89.
    F. Weik, A. de Meijere, E. Hasselbrink, J. Chem. Phys. 99, 682 (1993)CrossRefGoogle Scholar
  90. 90.
    R. Knorren, G. Bouzerar, K.H. Bennemann, Phys. Rev. B 63, 094306 (2001)CrossRefGoogle Scholar
  91. 91.
    M. Nest, P. Saalfrank, J. Chem. Phys. 116, 7189 (2002)CrossRefGoogle Scholar
  92. 92.
    S. Gao, B.I. Lundquist, W. Ho, Surf. Sci. 341, L1031 (1995)CrossRefGoogle Scholar
  93. 93.
    J.C.Tully, M. Gomez, M. Head-Gordon, J. Vac. Sci. Technol.A11, 1914 (1993)CrossRefGoogle Scholar
  94. 94.
    M. Morin, N.J. Levinos, A.L. Harris, J. Chem. Phys. 96, 3950 (1992)CrossRefGoogle Scholar
  95. 95.
    S. Gao, Phys. Rev. B 55, 1876 (1997)CrossRefGoogle Scholar
  96. 96.
    P.W. Anderson, Phys. Rev. 124, 41 (1961)CrossRefGoogle Scholar
  97. 97.
    P. Saalfrank, R. Baer, R. Kosloff, Chem. Phys. Lett. 230, 463 (1994)CrossRefGoogle Scholar
  98. 98.
    P. Saalfrank, R. Kosloff, J. Chem. Phys. 105, 2441 (1996)CrossRefGoogle Scholar
  99. 99.
    S.A. Buntin, L.J. Richter, R.R. Cavanagh, D.S. King, Phys. Rev. Lett. 61, 1321 (1988)CrossRefGoogle Scholar
  100. 100.
    M. Nest, P. Saalfrank, Phys. Rev. B 69, 235405 (2004)CrossRefGoogle Scholar
  101. 101.
    L. Cai, X. Xiao, M.M.T. Loy, Surf. Sci. 464, L727 (2000)CrossRefGoogle Scholar
  102. 102.
    M. Kampling, K. Al-Shamery, H.J. Freund, M. Wilde, K. Fukutani, Y. Murata, Phys. Chem. Chem. Phys. 4, 2629 (2002)CrossRefGoogle Scholar
  103. 103.
    G. Boendgen, P. Saalfrank, J. Phys. Chem. B 102, 8029 (1998)CrossRefGoogle Scholar
  104. 104.
    P. Saalfrank, G. Boendgen, C. Corriol, T. Nakajima, Faraday Discuss. 117, 65 (2000)CrossRefGoogle Scholar
  105. 105.
    K. Nakagami, Y. Ohtsuki, Y. Fujimura, Chem. Phys. Lett. 360, 91 (2002)CrossRefGoogle Scholar
  106. 106.
    V.S. Letokhov, Science 180, 451 (1973)CrossRefGoogle Scholar
  107. 107.
    F.F. Crim, Science 249, 1387 (1990)CrossRefGoogle Scholar
  108. 108.
    A. Abe, K. Yamashita, P. Saalfrank, Phys. Rev. B 67, 235411 (2003)CrossRefGoogle Scholar
  109. 109.
    G.K. Paramonov, P. Saalfrank, Chem. Phys. Lett. 301, 509 (1999)CrossRefGoogle Scholar
  110. 110.
    G.K. Paramonov, P. Saalfrank, J. Chem. Phys. 110, 6500 (1999)CrossRefGoogle Scholar
  111. 111.
    J.K. Vincent, R.A. Olsen, G.J. Kroes, M. Luppi, E.J. Baerends, J. Chem. Phys. 122, 044701 (2005)CrossRefGoogle Scholar
  112. 112.
    T. Vazhappilly, T. Klamroth, P. Saalfrank, (to be published)Google Scholar
  113. 113.
    H. Shi, K. Jacobi, Surf. Sci. 313, 289 (1994)CrossRefGoogle Scholar
  114. 114.
    S. Beyvers, Y. Ohtsuki, P. Saalfrank, J. Chem. Phys. 124, 234706 (2006)CrossRefGoogle Scholar
  115. 115.
    Y. Ohtsuki, W. Zhu, H. Rabitz, J. Chem. Phys. 110, 9825 (1999)CrossRefGoogle Scholar
  116. 116.
    J.W. Gadzuk, L.J. Richter, S.A. Buntin, D.S. King, R.R. Cavanagh, Surf. Sci. 235, 317 (1990)CrossRefGoogle Scholar
  117. 117.
    P. Saalfrank, Chem. Phys. 211, 265 (1996)CrossRefGoogle Scholar
  118. 118.
    K.F. und P. Saalfrank, Chem. Phys. Lett. 268, 291 (1997)CrossRefGoogle Scholar
  119. 119.
    P. Saalfrank, G. Boendgen, K. Finger, L. Pesce, Chem. Phys. 251, 51 (2000)CrossRefGoogle Scholar
  120. 120.
    N.A. Besley, Chem. Phys. Lett. 390, 124 (2004)CrossRefGoogle Scholar
  121. 121.
    V. Mohan, N. Sathyamurthy, Comput. Phys. Rep. 48, 213 (1988)CrossRefGoogle Scholar
  122. 122.
    U. Thumm, P. Kürpick, U. Wille, Phys. Rev. B 61, 3067 (2000)CrossRefGoogle Scholar
  123. 123.
    W. Ho, Surf. Sci. 363, 166 (1996)CrossRefGoogle Scholar
  124. 124.
    P.B. Corkum, F. Brunel, N.K. Sherman, T. Srinivasan-Rao, Phys. Rev. Lett. 61, 2886 (1988)CrossRefGoogle Scholar
  125. 125.
    A. Abe, K. Yamashita, J. Chem. Phys. 119, 9710 (2003)CrossRefGoogle Scholar
  126. 126.
    D. DeVault, Quantum–mechanical tunneling in biological systems, (Cambridge Univ. Press: London, 1984)Google Scholar
  127. 127.
    E.G. Petrov, Physics of charge transfer in biosystems (Naukowa Dumka: Kiev, 1984) (in Russian)Google Scholar
  128. 128.
    R.A. Marcus, N. Sutin, Biochim. Biophys. Acta 811, 265 (1985)Google Scholar
  129. 129.
    J. Jortner, M. Bixon, Adv. Chem. Phys. 106, 35 (1999)CrossRefGoogle Scholar
  130. 130.
    V. May, O. Kühn, Charge and energy transfer dynamics in molecular systems (Wiley–VCH, Berlin, 2004)Google Scholar
  131. 131.
    F.L. Carter (ed.) Molecular electronic devices (Marcel Dekker, New York, 1982).Google Scholar
  132. 132.
    A. Nitzan, Mark A. Ratner. Science, 300, 1384 (2003)CrossRefGoogle Scholar
  133. 133.
    B. O'Regan, M. Grätzel, Nature 353, 737 (1991).CrossRefGoogle Scholar
  134. 134.
    R.J.D. Miller, G. McLendon, A. Nozik, W. Schmickler, F. Willig, Surface electron transfer processes (VCH Publishers, New York, 1995)Google Scholar
  135. 135.
    J.B. Asbury, E. Hao, T. Wang, H. N. Ghosh, T. Lian, J. Phys. Chem. B 105, 4545 (2001)CrossRefGoogle Scholar
  136. 136.
    J. Kallioinen, G. Benkö, V. Sundström, J.E.I. Korppi-Tommola, A.P. Yartsev, J. Phys. Chem. B 106, 4396 (2002)CrossRefGoogle Scholar
  137. 137.
    A. Hagfeldt, M. Grätzel, Chem. Rev. 95, 49 (1995)CrossRefGoogle Scholar
  138. 138.
    K. Schwarzburg, R. Ernstorfer, S. Felber, F. Willig, Coord. Chem. Rev. 248, 1259 (2004)CrossRefGoogle Scholar
  139. 139.
    B. Burfeindt, T. Hannappel, W. Storck, F. Willig, J. Phys. Chem. 100, 16463, (1996)CrossRefGoogle Scholar
  140. 140.
    C. Zimmermann, F. Willig, S. Ramakrishna, B. Burfeindt, B. Pettinger, R. Eichberger, W. Storck, J. Phys. Chem. B 105, 9245, (2001)CrossRefGoogle Scholar
  141. 141.
    R. Huber, J.-E. Moser, M. Grätzel, J. Wachtveitl, J. Phys. Chem. B 106, 6494 (2002)CrossRefGoogle Scholar
  142. 142.
    T.H. James (ed.) The theory of the photographic process (McMillan Publishing Co., New York, 1977)Google Scholar
  143. 143.
    V. Shklover, M.-K. Nazeeruddin, S. M. Zakeeruddin, C. Barbe, A. Kay, T. Haibach, W. Steurer, R. Hermann, H.-U. Nissen, M. Grätzel, Chem. Mater. 9, 430 (1997)CrossRefGoogle Scholar
  144. 144.
    R. Ernstorfer, PhD Thesis, Free University Berlin, (2004)Google Scholar
  145. 145.
    L. Gundlach, PhD Thesis, Free University Berlin, (2005)Google Scholar
  146. 146.
    A. Hermann, W.G. Schmidt, F. Bechstedt, J. Phys. Chem. B 109, 7928 (2005)CrossRefGoogle Scholar
  147. 147.
    J. Moser, S. Punchihewa, P.P. Infelta, M. Grätzel, Langmuir 7, 3012 (1991)CrossRefGoogle Scholar
  148. 148.
    L. Wang, R. Ernstorfer, F. Willig, V. May, J. Phys. Chem. B 109, 9589 (2005)CrossRefGoogle Scholar
  149. 149.
    L. Wang, F. Willig, V. May, J. Chem. Phys. 124, 014712 (2006)CrossRefGoogle Scholar
  150. 150.
    W.R. Duncan, O.V. Prezhdo, J. Phys. Chem. B 109, 17998 (2005), and references given in this paper.CrossRefGoogle Scholar
  151. 151.
    P. Persson, M.J. Lundqvist, R. Ernstorfer, W.A. Goddard III, F. Willig, J. Chem. Theory. Comput. 2, 441 (2006), and references given in this paper.CrossRefGoogle Scholar
  152. 152.
    J.P. Muscat, D.M. Newns, Prog. Surf. Sci. 9, 1 (1978)CrossRefGoogle Scholar
  153. 153.
    G. Benkö, J. Kallioinen, J.E.I. Korppi-Tommola, A.P. Yartsev, V. Sundström, J. Am. Chem. Soc. 124, 489 (2002)CrossRefGoogle Scholar
  154. 154.
    P. C. Redfern, P. Zapol, L. A. Curtiss, T. Rajh, M. C. Thurnauer, J. Phys. Chem. B 107, 11419 (2003)CrossRefGoogle Scholar
  155. 155.
    S. G. Abuabara, L.G.C. Rego, V.S. Batista, J. Am. Chem. Soc. 127, 18234 (2005), and references given in this paper.CrossRefGoogle Scholar
  156. 156.
    W.R. Duncan, W.M. Stier, O.V. Prezhdo, J. Am. Chem. Soc. 127, 7941 (2005)CrossRefGoogle Scholar
  157. 157.
    C. Zimmermann, F. Willig, S. Ramakrishna, B. Burfeindt, B. Pettinger, R. Eichberger, W. Storck, J. Phys. Chem. B 105, 9245 (2001)CrossRefGoogle Scholar
  158. 158.
    L. Gundlach, S. Felber, W. Storck, E. Galoppini, Q. Wei, F. Willig, Res. Chem. Intermed. 31, 39 (2005)CrossRefGoogle Scholar
  159. 159.
    B. Trösken, F. Willig, K. Schwarzburg, A. Ehert, M. Spitler, J. Phys. Chem. 99, 5152 (1995)CrossRefGoogle Scholar
  160. 160.
    L. Gundlach, R. Ernstorfer, F. Willig, Phys. Rev. B 74, 035324 (2006)CrossRefGoogle Scholar
  161. 161.
    L. Gundlach, J. Szarko, L. D. Socaciu-Siebert, A. Neubauer, R. Ernstorfer, F. Willig. Phys. Rev. B (submitted)Google Scholar
  162. 162.
    S. Ramakrishna, F. Willig, J. Phys. Chem. B 104, 68, (2000)CrossRefGoogle Scholar
  163. 163.
    S. Ramakrishna, F. Willig, V. May, Phys. Rev. B 62, R16330, (2000)CrossRefGoogle Scholar
  164. 164.
    S. Ramakrishna, F. Willig, V. May, J. Chem. Phys. 115, 2743, (2001)CrossRefGoogle Scholar
  165. 165.
    S. Ramakrishna, F. Willig, V. May, Chem. Phys. Lett. 351, 242 (2002)CrossRefGoogle Scholar
  166. 166.
    S. Ramakrishna, F. Willig, V. May, A. Knorr, J. Phys. Chem. B 107, 607 (2003)CrossRefGoogle Scholar
  167. 167.
    L. Wang, V. May, J. Chem. Phys. 121, 8039 (2004)CrossRefGoogle Scholar
  168. 168.
    L. Wang, F. Willig, V. May, in Molecular simulation, special issue on Electron Transfer, ed. by D.N. Beratan, S.S. Skourtis (in press)Google Scholar
  169. 169.
    M. Thoss, I. Kondov, H. Wang, Chem. Phys. 304, 169 (2004)CrossRefGoogle Scholar
  170. 170.
    I. Kondov, M. Thoss, H. Wang, J. Phys. Chem. A 110, 1364 (2006)CrossRefGoogle Scholar
  171. 171.
    P. Persson, R. Bergström, S. Lunell, J. Phys. Chem. B 104, 10348, (2000)CrossRefGoogle Scholar
  172. 172.
    L.G.C. Rego, V.S. Batista, J. Am. Chem. Soc. 125, 7989, (2003)CrossRefGoogle Scholar
  173. 173.
    W. R. Duncan, O. V. Prezhdo, J. Phys. Chem. B 109, 365 (2005)CrossRefGoogle Scholar
  174. 174.
    P. Persson, M.J. Lundqvist, R. Ernstorfer, W.A. Goddard III, F. Willig, J. Chem. Theory Comp. 2, 441, (2006)CrossRefGoogle Scholar
  175. 175.
    M. Nilsing, S. Lunell, P. Persson, L. Ojamäe, Surf. Sci. 582, 49 (2005)CrossRefGoogle Scholar
  176. 176.
    F. Willig, C. Zimmermann, S. Ramakrishna, W. Storck, Electrochim. Acta 45, 4565 (2000)CrossRefGoogle Scholar
  177. 177.
    B. Burfeindt, C. Zimmermann, S. Ramakrishna, T. Hannappel, B. Meißner, W. Storck, F. Willig, Z. Phys. Chem. 212, 67 (1999)Google Scholar
  178. 178.
    P.C. Redfern, P. Zapol, L.A. Curtiss, T. Rajh, M.C. Thurnauer, J. Phys. Chem. B 107, 11419 (2003)CrossRefGoogle Scholar
  179. 179.
    P.H. Hahn, W.G. Schmidt, Surf. Rev. Lett. 10, 163 (2003)CrossRefGoogle Scholar
  180. 180.
    W.G. Schmidt, P.H. Hahn, F. Bechstedt, N. Esser, P. Vogt, A. Wange, W. Richter. Phys. Rev. Lett. 90, 126101 (2003)CrossRefGoogle Scholar
  181. 181.
    T. Letzig, H.-J. Schimper, T. Hannappel, F. Willig, Phys. Rev. B, 71, 033308 (2005)CrossRefGoogle Scholar
  182. 182.
    T.M. Halasinski, J.L. Weisman, R. Ruiterkamp, T.J. Lee, F. Salama, M. Head-Gordon, J. Phys. Chem. A 107, 3660 (2003)CrossRefGoogle Scholar
  183. 183.
    K. K. Ong, J.O. Jensen, H.F. Hameka, J. Mol. Str. (Theochem). 459, 131 (1999)CrossRefGoogle Scholar
  184. 184.
    R. Ernstorfer, L. Gundlach, S. Felber, W. Storck, R. Eichberger, F. Willig, J. Phys. Chem. B (accepted)Google Scholar
  185. 185.
    R. Rodriguez, M.A. Blesa, A.E. Regazzoni, J. Coll. Int. Sci. 177, 122, (1996)CrossRefGoogle Scholar
  186. 186.
    J.L. Herek (ed.), Coherent control of photochemical and photobiological processes, special issue, J. Photochem. Photobiol. (2006)Google Scholar
  187. 187.
    T. Halfmann (ed.), Quantum control of light and matter, special issue, Opt. Comm. (2006).Google Scholar
  188. 188.
    A. P. Pierce, M.A. Dahleh, H. Rabitz, Phys. Rev. A 37, 4950 (1988)CrossRefGoogle Scholar
  189. 189.
    S.G. Abuabara, L.G.C. Rego, V.S. Batista, J. Am. Chem. Soc. 127, 18234 (2005)CrossRefGoogle Scholar
  190. 190.
    W. Stier, O.V. Prezhdo, J. Phys. Chem. B 106, 8047 (2002)CrossRefGoogle Scholar
  191. 191.
    W. Stier, O.V. Prezhdo, Isr. J. Chem. 42, 213 (2003)CrossRefGoogle Scholar
  192. 192.
    W. Stier, W.R. Duncan, O.V. Prezhdo, SPIE Proc. 5223, 132 (2003)CrossRefGoogle Scholar
  193. 193.
    W. Stier, W.R. Duncan, O.V. Prezhdo, Adv. Mat. 16, 240 (2004)CrossRefGoogle Scholar
  194. 194.
    W.R. Duncan, O.V. Prezhdo, J. Phys. Chem. B 109, 17998 (2005)CrossRefGoogle Scholar
  195. 195.
    C.F. Craig, W.R. Duncan, O.V. Prezhdo, Phys. Rev. Lett. 95, 163001 (2005)CrossRefGoogle Scholar
  196. 196.
    R. Argazzi, N.Y.M. Iha, H. Zabri, F. Odobel, C.A. Bignozzi, Coord. Chem. Rev. 248, 1299 (2004)CrossRefGoogle Scholar
  197. 197.
    Y. Wang, K. Hang, N.A. Anderson, T. Lian, J. Phys. Chem. B 107, 9434 (2003)CrossRefGoogle Scholar
  198. 198.
    J.B. Asbury, R.J. Ellingson, H.N. Ghosh, S. Ferrere, A.J. Nozik, T.Q. Lian, J. Phys. Chem. B 103, 3110 (1999)CrossRefGoogle Scholar
  199. 199.
    J.B. Asbury, E.C. Hao, Y.Q. Wang, H.N. Ghosh, T.Q. Lian, J. Phys. Chem. B 105, 4545 (2001)CrossRefGoogle Scholar
  200. 200.
    R. Memming, Semiconductor Electrochemistry (Wiley-VCH, Weinheim, 2001)Google Scholar
  201. 201.
    C. Kittel, Introduction to solid state Physics (Wiley, New York, 1996)Google Scholar
  202. 202.
    W. Kohn, L.J. Sham, Phys. Rev. A 4, 1133 (1965)Google Scholar
  203. 203.
    T. Frauenheim, G. Seifert, M. Elstner, T. Niehaus, C. Köhler, M. Amkreutz, M. Sternberg, Z. Hajnal, A. DiCarlo, S. Suhai, J. Phys.: Condens. Matter 14, 3015 (2002)CrossRefGoogle Scholar
  204. 204.
    M.A.L. Marques, E.K.U. Gross, Annu. Rev. Phys. Chem. 55, 427 (2004)CrossRefGoogle Scholar
  205. 205.
    R. Baer, T. Seideman, S. Ilani, D. Neuhauser, J. Chem. Phys. 120, 3387 (2004)CrossRefGoogle Scholar
  206. 206.
    I. Franco, S. Tretiak, J. Am. Chem. Soc. 126, 12130 (2004)CrossRefGoogle Scholar
  207. 207.
    M.A.L. Marques, X. López, D. Varsano, A. Castro, A. Rubio, Phys. Rev. Lett. 90, 258101 (2003)CrossRefGoogle Scholar
  208. 208.
    J.P. Perdew, K. Burke, M. Ernzerhof, Phys. Rev. Lett. 77, 3685 (1996)CrossRefGoogle Scholar
  209. 209.
    G. Kresse, J. Furthmüller, Comput. Mater. Sci. 6, 15 (1996)CrossRefGoogle Scholar
  210. 210.
    G. Kresse, J. Furthmüller, Phys. Rev. B 54, 11169 (1996)CrossRefGoogle Scholar
  211. 211.
    S. Hammes-Schiffer, J.C. Tully, J. Chem. Phys. 101, 4657 (1994)CrossRefGoogle Scholar
  212. 212.
    G.D. Billing, Int. Rev. Phys. Chem. 13, 309 (1994)CrossRefGoogle Scholar
  213. 213.
    J.C. Tully, in Classical and quantum dynamics in condensed phase simulations, ed. by B.J. Berne, G. Ciccotti, D.F. Coker (World Scientific, Singapore, 1998), pp. 489–514Google Scholar
  214. 214.
    P. Ehrenfest, Z. Physik 45, 455 (1927)CrossRefGoogle Scholar
  215. 215.
    J.C. Tully, R.K. Preston, J. Chem. Phys. 55, 562 (1971)CrossRefGoogle Scholar
  216. 216.
    J.C. Tully, J. Chem. Phys. 93, 1061 (1990)CrossRefGoogle Scholar
  217. 217.
    P.V. Parahdekar, J. C. Tully, J. Chem. Phys. 122, 094102 (2005)CrossRefGoogle Scholar
  218. 218.
    T.N. Todorov, J. Hoekstra, A.P. Sutton, Phys. Rev. Lett. 86, 3606 (2001)CrossRefGoogle Scholar
  219. 219.
    A.P. Horsfield, D.R. Bowler, A.J. Fisher, T.N. Todorov, C.G. Sanchez, J. Phys. Cond. Mat. 16, 8251 (2004)CrossRefGoogle Scholar
  220. 220.
    O.V. Prezhdo, Y.V. Pereverzev, J. Chem. Phys. 113, 6557 (2000)CrossRefGoogle Scholar
  221. 221.
    C. Brooksby, O.V. Prezhdo, Chem. Phys. Lett. 346, 463 (2001)CrossRefGoogle Scholar
  222. 222.
    O.V. Prezhdo, Y.V. Pereverzev, J. Chem. Phys. 116, 4450 (2002)CrossRefGoogle Scholar
  223. 223.
    E. Pahl, O.V. Prezhdo, J. Chem. Phys. 116, 8704 (2002)CrossRefGoogle Scholar
  224. 224.
    O.V. Prezhdo, J. Chem. Phys. 117, 2995 (2002)CrossRefGoogle Scholar
  225. 225.
    C. Brooksby, O.V. Prezhdo, Chem. Phys. Lett. 378, 533 (2003)CrossRefGoogle Scholar
  226. 226.
    D. Kilin, Y.V. Pereverzev, O.V. Prezhdo, J. Chem. Phys. 120, 11209 (2004).CrossRefGoogle Scholar
  227. 227.
    E. Heatwole, O.V. Prezhdo, J. Chem. Phys. 121, 10967 (2004).CrossRefGoogle Scholar
  228. 228.
    E. Heatwole, O.V. Prezhdo, J. Chem. Phys. 122, 234109 (2005)CrossRefGoogle Scholar
  229. 229.
    O.V. Prezhdo, P.J. Rossky, Phys. Rev. Lett. 81, 5294 (1998)CrossRefGoogle Scholar
  230. 230.
    O.V. Prezhdo, J. Chem. Phys. 111, 8366 (1999)CrossRefGoogle Scholar
  231. 231.
    O.V. Prezhdo, Phys. Rev. Lett. 85, 4413 (2000)CrossRefGoogle Scholar
  232. 232.
    A. Luis, Phys. Rev. A 67, 062113 (2003)CrossRefGoogle Scholar
  233. 233.
    P. Exner, J. Phys. A: Math. Gen. 38, L449 (2005)CrossRefGoogle Scholar
  234. 234.
    S. Ramakrishna, F. Willig, A. Knorr, Surf. Sci 558, 159 (2004)CrossRefGoogle Scholar
  235. 235.
    L. Toben, L. Gundlach, R. Ernstorfer, R. Eichberger, T. Hannappel, F. Willig, A. Zeiser, J. Forstner, A. Knorr, P. H. Hahn, M.G. Schmidt, Phys. Rev. Lett. 94, 067601 (2005)CrossRefGoogle Scholar
  236. 236.
    P. Nuernberger, D. Wolpert, H. Weiss, G. Gerber, in Ultrafast Phenomena XV, ed. by P.B. Corkum, D.M. Jonas, R.J.D. Miller, and A.M. Weiner (Springer Series of Chemical Physics, Springer, Berlin,) Vol. 88Google Scholar

Copyright information

© Springer 2007

Authors and Affiliations

  • Christian Frischkorn
    • 1
  • Martin Wolf
    • 1
  • Ulrich Höfer
    • 2
  • Jens Güdde
    • 2
  • Peter Saalfrank
    • 3
  • Mathias Nest
    • 3
  • Tillmann Klamroth
    • 3
  • Frank Willig
    • 4
  • Ralph Ernstorfer
    • 4
  • Lars Gundlach
    • 4
  • Volkhard May
    • 5
  • Luxia Wang
    • 5
  • Walter R. Duncan
    • 6
  • Oleg V. Prezhdo
    • 6
  1. 1.Fachbereich PhysikFreie Universität BerlinGermany
  2. 2.Fachbereich PhysikPhilipps-UniversitätMarburgGermany
  3. 3.Institut für ChemieUniversität PotsdamGermany
  4. 4.Hahn-Meitner-InstitutBerlinGermany
  5. 5.Institut für PhysikHumboldt Universität zu BerlinGermany
  6. 6.Department of ChemistryUniversity of WashingtonSeattleUSA

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