Modeling Heavy Metals in Europe’s Atmosphere: A Combined Trajectory-Climatologic Approach

  • Joseph Alcamo
  • Jerzy Bartnicki
  • Krzysztof Olendrzynski
Chapter
Part of the NATO · Challenges of Modern Society book series (NATS, volume 15)

Abstract

The long range transport of heavy metals in the atmosphere leads to low but steady deposition of heavy metals into soils, lakes and forests in Europe. Although their atmospheric fluxes are low, these metals can accumulate in the detritus of soils. This accumulated metal may be mobilized by acidification and may then disturb soil organisms, which in turn can lead to disturbance of organic matter decomposition and nutrient cycling (Ottar et al., 1989). Circumstantial evidence from wind sector analysis and trajectory modeling (Pacyna et al., 1984), and receptor modeling (Stevens et al., 1984) indicates that the deposition of metals may originate from sources many hundreds of kilometers away. It is thought that large particles (> 10 μ) settle out in the vicinity of the stacks but stack gases containing metals condense into small particles which then coalesce within hours into particles with diameters of 0.1 to 1.0 μ; particles of this size are too coarse to be efficiently removed by brownian diffusion yet too small to settle out by gravity. Hence these metal particles may travel long distances before being removed by precipitation or dry deposition.

Keywords

Heavy Metal Transport Distance Trajectory Model Brownian Diffusion Trace Model 
These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.
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References

  1. Chan, W.H., Tang, A.J.S., Chung, D.H.S., and Lusis, M.A., 1982, Concentration and deposition of trace metals in Ontario-1982, Water, Air, and Soil Pollution 29:373–389.Google Scholar
  2. Dulac, F., Buart-Menard, P., Ezat, U., Melki, S., and Bergametti, G., 1989, Atmospheric input of trace metals to the western Mediterranean: uncertainties in modelling dry deposition from cascade impactor data, Tellus, 41B:362–378.CrossRefGoogle Scholar
  3. Eliassen, A. and Saltbones, J., 1983, Modelling of long-range transport of sulphur over Europe: a two-year model run and some model experiments. Atmospheric Environment, 17:1457–1473.CrossRefGoogle Scholar
  4. Eliassen, A., Hov, O., Iversen, T., Saltbones, J., and Simpson, D., 1988, Estimates of airborne transboundary transport of sulphur and nitrogen over Europe, EMEP/MSC-W Report 1/88:1–79.Google Scholar
  5. Georgii, H.W., Perseke, C., and Rohbock, E., 1982, Feststellung der deposition von sauren und langzeitwirksamen luftverunreinigungen aus belastungsgebieten, Umweltforschungsplan des Bundesminiters des Innern, Luftreinhaltung Forschungsprojekt 104 02 600.Google Scholar
  6. Gatz, D.F., 1975, Pollutant aerosol deposition into southern lake Michigan, Water, Air and Soil Pollution 5:239–251.CrossRefGoogle Scholar
  7. Ottar, B., Lindberg, S.E., Voldner, E., Lingqvist, O., Mayer, R., Semb, A., Steinnes, E., and Watt, J., 1989, Special topics concerning interactions of heavy metals with the environment, in: Control and Fate of Atmospheric Trace Metals: 365-372, J.M. Pacyna and B. Ottar, ed., Kluwer Academic Publishers.Google Scholar
  8. Pacyna, J.M., Semb, A., and Hanssen, J.E., 1984, Emission and long-range transport of trace elements in Europe, Tellus 36B:163–178.CrossRefGoogle Scholar
  9. Pacyna, J.M., 1988, Atmospheric lead emissions in Europe in 1985, NILU OR:19/88:1–10.Google Scholar
  10. Pacyna, J.M., and Münch, J., 1987, Atmospheric emissions of As, Cd, Pb and Zn from industrial sources in Europe, in: S.E. Lindberg, and T.C. Hutchinson, ed., Heavy Metals in the Environment, Vol.1, New Orleans, CEP Consultants, Edinburgh.Google Scholar
  11. Pacyna, J.M., and Münch, J., 1988, Atmospheric emissions of arsenic, cadmium, mercury and zinc in Europe in 1982, NILU OR:17/83:1–33.Google Scholar
  12. Rühling, A., Rasmussen, L., Pilegaard, K., Mäkinen, A., and Steinnes, E., 1987, Survey of atmospheric heavy metal deposition, Report prepared for The Steering Body for Environmental Monitoring, The Nordic Council of Ministers. NORD 1987:21:1–44.Google Scholar
  13. Sehmel, G.A., 1980, Particle and gas dry deposition: a review, Atmospheric Environment, 14:983–1011.CrossRefGoogle Scholar
  14. Seinfeld, J.H., 1986, Atmospheric chemistry and physics of air pollution, John Wiley & Sons, New York.Google Scholar
  15. Semb, A., and Pacyna, J.M., 1988, Toxic trace elements and chlorinated hydrocarbons: sources, atmospheric transport and deposition, Miljørapport, NORD 1988:74. pp. 1–96.Google Scholar
  16. Slinn, W.G.N., 1984, Precipitation scavenging, in: Atmospheric Science and Power Production, D. Randerson, ed., Technical Information Center, Office of Scientific and Technical Information, United States Department of Energy.Google Scholar
  17. Stevens, R.K., Dzubay, T.G., Lewis, C.W., and Shaw Jr., R.W., 1984, Source apportionment methods applied to the determination of the origin of ambient aerosols that affect visibility in forested areas, Atmospheric Environment Vol. 18, No. 2:261–272.CrossRefGoogle Scholar
  18. WMO, 1989, Air Quality Guidelines, Review Draft, Vol. 11, World Health Organization, Regional Office for Europe, Copenhagen, Denmark.Google Scholar

Copyright information

© Springer Science+Business Media New York 1991

Authors and Affiliations

  • Joseph Alcamo
    • 1
  • Jerzy Bartnicki
    • 1
  • Krzysztof Olendrzynski
    • 1
  1. 1.International Institute for Applied Systems AnalysisLaxenburgAustria

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