Heterodyne 2D-IR Photon Echo Spectroscopy of Multi-Level OH Stretching Coherences in Hydrogen Bonds

  • N. Huse
  • B. D. Bruner
  • M. L. Cowan
  • J. Dreyer
  • E. T. J. Nibbering
  • T. Elsaesser
  • R. J. D. Miller
Part of the Springer Series in Chemical Physics book series (CHEMICAL, volume 79)

Abstract

We explore the multilevel structure and vibrational couplings of hydrogen bonded O-H stretching transitions in acetic acid dimer using femtosecond 2D-IR photon echo spectroscopy. Anharmonic coupling with low-frequency modes and Fermi resonances with overtone/combination levels dominate the complex ultrafast dynamics.

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Copyright information

© Springer-Verlag Berlin Heidelberg 2005

Authors and Affiliations

  • N. Huse
    • 1
  • B. D. Bruner
    • 2
  • M. L. Cowan
    • 2
  • J. Dreyer
    • 1
  • E. T. J. Nibbering
    • 1
  • T. Elsaesser
    • 1
  • R. J. D. Miller
    • 2
  1. 1.Max Born Institut fuer Nichtlineare Optik und KurzzeitspektroskopieBerlinGermany
  2. 2.Departments of Physics and ChemistryUniversity of TorontoTorontoCanada

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