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Two Dimensional Fourier Transform Electronic Spectroscopy: Evolution of Cross Peaks in the Fenna-Matthews-Olson Complex

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Ultrafast Phenomena XV

Part of the book series: Springer Series in Chemical Physics ((CHEMICAL,volume 88))

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Abstract

Two dimensional femtosecond Fourier transform electronic spectroscopy is used to study the evolution of cross peaks in the Fenna-Matthews-Olson complexes isolated from Chlorobium tepidum and Pelodictyon phaeum. Evidence for quantum beating is observed, and a technique for eliminating the signal from the main diagonal peaks using polarization rotation of the input pulses is demonstrated.

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Author information

Authors and Affiliations

  1. Department of Chemistry, University of California, Berkeley

    G. S. Engel, E. L. Read, T. R. Calhoun, T. K. Ahn, T. Mančál & G. R. Fleming

  2. Physical Biosciences Division, Lawrence Berkeley National Laboratory, Berkeley, California, 94720-1460, USA

    G. S. Engel, E. L. Read, T. R. Calhoun, T. K. Ahn, T. Mančál & G. R. Fleming

  3. Department of Chemistry and Biochemistry, Arizona State University, Tempe, Arizona, 85287-1604, USA

    R. E. Blankenship

Authors
  1. G. S. Engel
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  2. E. L. Read
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  3. T. R. Calhoun
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  4. T. K. Ahn
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  5. T. Mančál
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  6. R. E. Blankenship
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  7. G. R. Fleming
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Editor information

Editors and Affiliations

  1. Steacie Institute for Molecular Sciences, National Research Council Canada, 100 Sussex Drive, Rm 2063, Ottawa, ON, K1A 0R6, Canada

    Paul Corkum

  2. Department of Chemistry & Biochemistry 215 UCB, University of Colorado, Boulder, Boulder, CO, 80309-0215, USA

    David M. Jonas

  3. Department of Chemistry, University of Toronto, 80 St. George Street, Toronto, ON, M5S 3H6, Canada

    R. J. Dwayne. Miller

  4. School of Electrical & Computer Engineering, Purdue University, 1285 Elec. Eng. Bldg., West Lafayette, IN, 47907-1285, USA

    Andrew M. Weiner

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© 2007 Springer-Verlag Berlin Heidelberg

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Cite this paper

Engel, G.S. et al. (2007). Two Dimensional Fourier Transform Electronic Spectroscopy: Evolution of Cross Peaks in the Fenna-Matthews-Olson Complex. In: Corkum, P., Jonas, D.M., Miller, R.J.D., Weiner, A.M. (eds) Ultrafast Phenomena XV. Springer Series in Chemical Physics, vol 88. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-540-68781-8_127

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