About this book
This thesis describes significant advances in experimental capabilities using ultracold polar molecules. While ultracold polar molecules are an idyllic platform for quantum chemistry and quantum many-body physics, molecular samples prior to this work failed to be quantum degenerate, were plagued by chemical reactions, and lacked any evidence of many-body physics. These limitations were overcome by loading molecules into an optical lattice to control and eliminate collisions and hence chemical reactions. This led to observations of many-body spin dynamics using rotational states as a pseudo-spin, and the realization of quantum magnetism with long-range interactions and strong many-body correlations.
Further, a 'quantum synthesis' technique based on atomic insulators allowed the author to increase the filling fraction of the molecules in the lattice to 30%, a substantial advance which corresponds to an entropy-per-molecule entering the quantum degenerate regime and surpasses the so-called percolations threshold where long-range spin propagation is expected.
Lastly, this work describes the design, construction, testing, and implementation of a novel apparatus for controlling polar molecules. It provides access to: high-resolution molecular detection and addressing; large, versatile static electric fields; and microwave-frequency electric fields for driving rotational transitions with arbitrary polarization. Further, the yield of molecules in this apparatus has been demonstrated to exceed 10^5, which is a substantial improvement beyond the prior apparatus, and an excellent starting condition for direct evaporative cooling to quantum degeneracy.
ultracold polar molecule experiment quantum synthesis atomic insulator quantum degenerate bulk gas polar molecules highly-filled 3D optical lattice quantum-state controlled chemical reaction quantum magnetism polar molecules low entropy quantum gas polar molecules new apparatus controlling polar molecules many-body spin dynamics ultracold polar molecules quantum degenerate bulk gas
- DOI https://doi.org/10.1007/978-3-319-98107-9
- Copyright Information Springer Nature Switzerland AG 2018
- Publisher Name Springer, Cham
- eBook Packages Physics and Astronomy Physics and Astronomy (R0)
- Print ISBN 978-3-319-98106-2
- Online ISBN 978-3-319-98107-9
- Series Print ISSN 2190-5053
- Series Online ISSN 2190-5061
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