Abstract
Single-crystalline DyFe1−x Mn x O3 perovskites with the nominal Mn contents of x = 0.2, 0.5, and 0.7 were grown successfully. The solid solutions have an orthorhombic structure with space group Pbnm. Magnetic susceptibilities at different crystallographic axes show a large magnetic anisotropy, primarily originating from the large spin-orbit coupling of the Dy moment. For DyFe0.8Mn0.2O3, a room-temperature weak ferromagnetism is confirmed along the c-axis. A spin reorientation transition occurs at T SR ≈ 225 K, below which the canted weak ferromagnetic moment disappears. The application of a high magnetic field (µ0H ≥ 6 T) along the c-axis at T = 200 K unveils a hidden field-induced weak ferromagnetism, which probably has the same spin configuration as that above T SR ≈ 225 K.
Similar content being viewed by others
References
Y. Tokunaga, S. Iguchi, T. Arima and Y. Tokura, Phys. Rev. Lett. 101, 097205 (2008).
A. Stroppa, M. Marsman, G. Kresse and S. Picozzi, New J. Phys. 12, 093026 (2010).
T. Goto, T. Kimura, G. Lawes, A. P. Ramirez and Y. Tokura, Phys. Rev. Lett. 92, 257201 (2004).
See, for example, S.-W. Cheong and M. Mostovoy, Nature Mater. 6, 13 (2007)
F.-K. Chiang, M-W. Chu, F. C. Chou, H. T. Jeng, H. S. Sheu, F. R. Chen and C. H. Chen, Phys. Rev. B 83, 245105 (2011).
F. Hong, Z. Cheng, H. Zhao, H. Kimura and X. Wang, Appl. Phys. Lett. 99, 092502 (2011).
P. Mandal, V. S. Bhadram, Y. Sundarayya, C. Narayana, A. Sundaresan and C. N. R. Rao, Phys. Rev. Lett. 107, 137202 (2011).
Y.-H. Huang, M. Karppinen, N. Imamura, H. Yamauchi and J. B. Goodenough, Phys. Rev. B 76, 174405 (2007).
Y. Nagata, S. Yashiro, T. Misuhashi, A. Koriyama, Y. Kawashima and H. Samata, J. Magn. Magn. Mater. 237, 250 (2001).
P. Mandal, C. R. Serrao, E. Suard, V. Caignaert, B. Raveau, A. Sundaresan and C. N. R. Rao, J. Solid State Chem. 197, 408 (2013).
I. Mikami, J. Phys. Soc. Jap. 34, 338 (1973).
R. D. Shannon, Acta Cryst. 32, 751 (1976).
A. H. Cooke, D. M. Martin and M. R. Wells, J. Phys. C: Solid State Phys. 7, 3133 (1974).
G. Gorodetsky, B. Sharon and S. Shtrikman, J. Appl. Phys. 39, 1371 (1968).
T. Skomski and D. J. Sellmyer, J. Rare Earths 27, 675 (2009).
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Cho, K., Park, S. Field-induced weak ferromagnetism in single-crystalline DyFe0.8Mn0.2O3 . Journal of the Korean Physical Society 63, 1–4 (2013). https://doi.org/10.3938/jkps.63.1
Received:
Published:
Issue Date:
DOI: https://doi.org/10.3938/jkps.63.1