Abstract
The magnetic and electroconducting properties of Nd1 − x Sr x MnO3 − y films with various thicknesses are studied. It is shown that all the films exhibit considerably high conductivity at a temperature of 300 K and that they are not a paramagnetic insulator as should be the case according to the phase diagram of this compound. The temperature dependence of the resistance exhibits a semiconductor behavior with decreasing temperature and has a maximum R max at the temperature T max being significantly different from the Curie point. A negative magnetic moment is observed in all the studied films at high temperatures. The possible causes of this phenomenon are discussed.
Similar content being viewed by others
References
Kawano, H., Kajimoto, R., Yashizawa, H., Tomioka, Y., Kuwahara, H., and Tokura, Y., Magnetic Ordering and Relation to the Metal-Insulator Transition in Pr1 − x SrxMnO3 and Nd1 − x SrxMnO3 with x ∼ 1/2, Phys. Rev. Lett., 1997, vol. 78, pp. 4253–4256.
Tokura, Y. and Tomioka, Y., Colossal Magnetoresistive Manganites, J. Magn. Magn. Mater., 1999, vol. 200, pp. 1–23.
Kajimoto, R., Yoshizawa, H., Kuwahara, H., Tokura, Y., Ohoyama, K., and Ohashi, M., Hole-Concentration-Induced Transformation of the Magnetic and Orbital Structures in Nd1 − x SrxMnO3, Phys. Rev. B, 1999, vol. 60, pp. 9506–9517.
Cui, C., Tyson, T.A., Chen, Zh., and Zhong, Zh., Transport and Structural Study of Pressure-Induced Magnetic States in Nd0.55Sr0.45MnO3 and Nd0.5Sr0.5MnO3, Phys. Rev. B, 2003, vol. 68, p. 214417.
Prokhorov, V.G., Kaminsky, G.G., Komashko, V.A., Lee, Y.P., Park, S.Y., Hyin, Y.H., Kim, J.B., Park, J.S., Svechnikov, V.L., Pashchenko, V.P., and Khokhlov, V.A., Nonclassical Magnetic Dynamics and Negative Exchange Bias in Nd0.5Sr0.5MnO3 Films, Fiz. Nizk. Temp,., 2007, vol. 33,no. 8, pp. 889–896.
Ogimoto, Y., Nakamura, M., Takubo, N., Tamaru, H., Izumi, M., and Miyano, K., Strain-Induced Crossover of the Metal-Isolator Transition in Perovskite Manganites, Phys. Rev. B, 2005, vol. 71, p. 060403(R).
Prellier, W., Biswas, A., Raeswari, M., Venkatesan, T., and Greene, R.G., Effect of Substrate-Induced Strain of the Charge-Ordering Transition in Nd0.5Sr0.5MnO3 Thin Films, Appl. Phys. Lett., 1999, vol. 75, no. 3, pp. 397–399.
Wang, Y.T., Pan, M.X., Zhao, D.Q., Wang, W.H., and Wang W.L., Unusual Diamagnetic Response in PrAlNiCuFe Metallic Glass, Appl. Phys. Lett., 2004, vol. 85, no. 14, pp. 2881–2883.
Marcovich, V., Fita, I., Ruznak, R., Martin, C., Kikoin, K., Wisniewski, A., Hebert, S., Maignan, A., and Gorodetsky, G., Metastable Diamagnetism in the Manganite Sm0.1Ca0.84Sr0.06MnO3, Phys. Rev. B, 2006, vol. 74, p. 174 408.
Onishchenko, T.A., Diamagnetism of Band Electrons in Macroscopically Inhomogeneous Crystals, Pis’ma Zh. Eksp. Teor. Fiz., 1981, vol. 33, no. 2, pp. 93–97.
Author information
Authors and Affiliations
Corresponding author
Additional information
Original Russian Text © V.A. Khokhlov, 2010, published in Elektronnaya Obrabotka Materialov, 2010, No. 2, pp. 67–71.
About this article
Cite this article
Khokhlov, V.A. Experimental studies of cation-anion-deficient Nd1 − x Sr x MnO3 − y (x = 0.45) films with various thicknesses. Surf. Engin. Appl.Electrochem. 46, 144–148 (2010). https://doi.org/10.3103/S1068375510020109
Received:
Published:
Issue Date:
DOI: https://doi.org/10.3103/S1068375510020109