Abstract
Nuclear data obtained in the neutron induced fission of 232Th nucleus are of great importance for advanced fast reactors based on Th fuel cycle. Fission cross sections, mass and charge distributions, prompt emission in fission including neutron multiplicities, yields and cross-sections of some isotopes of interest for applications, isomer ratios were obtained. This paper presents the theoretical predictions and the first results on 232Th(n,f) by applying Talys and the author’s computer code for modeling of nuclear reaction mechanisms and the fission process. Theoretical evaluations of fission observables and produced isotopes are compared with existing experimental data and with similar data for neutrons induced fission of 233U nucleus. The present researches on 232Th(n,f) reaction are realized in the frame of nuclear data program running at Joint Institute for Nuclear Research (Dubna) basic facilities, IREN, and MT-25 Microtron.
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REFERENCES
Meija, J., Coplen, T.B., Berglund, M., Brand, W.A., de Bièvre, P., Gröning, M., Holden, N.E., Irrgeher, J., Loss, R.D., Walczyk, T., and Prohaska, T., Pure Appl. Chem., 2016, vol. 88, no. 3, p. 265.
Hargraves, R. and Moir, R., Am. Sci., 2010, vol. 98, p. 304.
Krepel, J., Fission and transmutation, in Encyclopedia of Nuclear Energy, Amsterdam: Elsevier, 2021, vol. 1.
Waltar, A.E., Fission, in Encyclopedia of Nuclear Energy, Amsterdam: Elsevier, 2021, vol. 4.
Waltar, A.E., Medical, industrial and agricultural applications of nuclear technology, in Encyclopedia of Nuclear Energy, Amsterdam: Elsevier, 2021, vol. 4.
Koning, A.J., Hilaire, S., and Duijvestijn, M.C., TALYS-1.0., Proceedings of the International Conference on Nuclear Data for Science and Technology 2007, Bersillon, O., Gunsing, F., Bauge, E., Jacqmin, R., and Leray, S., Eds., Nice: EDP Sciences, 2008, p. 211.
Satchler, G.R., Direct Nuclear Reactions, New York: Oxford Univ. Press, 1983.
Koning, A.J. and Duijvestijn, M.C., Nucl. Phys. A, 2004, vol. 744, p. 15.
Hauser, W. and Feshbach, H., Phys. Rev., 1952, vol. 87, no. 2, p. 366.
Foderaro, A., The Neutron Interaction Theory, Cambridge: MIT Press, 1971.
Gledenov, Y.M., Sedysheva, M.V., Sedyshev, P.V., Oprea, A., Chen, Z., Chen, Y., Yuan, J., Zhang, G., Tang, G., Khuukhenkhuu, G., and Szalanski, P.J., Nucl. Sci. Technol., 2002, no. 2 (suppl.), p. 342.
Oprea, A.I., Oprea, C., Pirvutoiu, C., and Vladoiu, D., Rom. Rep. Phys., 2011, vol. 63, no. 1, p. 107.
Hill, D.L. and Wheeler, J.A., Phys. Rev., 1953, vol. 89, p. 1102.
Moldauer, P.A., Phys. Rev. B, 1964, vol. 135, p. 642.
Moldauer, P.A., Rev. Mod. Phys., 1964, vol. 36, p. 1079.
Brosa, U., Grossmann, S., and Müller, A., Phys. Rep., 1990, vol. 197, no. 4, p. 167.
Duijvestijn, M.C., Koning, A.J., and Hambsch, F.J., Phys. Rev. C, 2001, vol. 64, 014607.
Huizenga, J.R. and Vandenbosh, R., Phys. Rev., 1960, vol. 120, p. 1305.
Huizenga, J.R. and Vandenbosh, R., Phys. Rev., 1960, vol. 120, p. 1313.
Smith, A.B., Phys. Rev., 1962, vol. 127, p. 718.
Batchelor, R., Gilboy, W.B., and Towle, J.H., Nucl. Phys., 1965, vol. 65 p. 236.
Fursov, B.I., Baranov, Yu.M., Klemyshev, M.P., Samylin, B.F., Smirenkin, G.N., and Turchin, Yu.M., Sov. At. Energy, 1991, vol. 71, p. 827.
Karamian, S.A., Collins, C.B., Carroll, J.J., Adam, J., Belov, A.G., and Stegailov, V.I., Phys. Rev. C, 1999, vol. 59, p. 755.
Simutkin, V.D., Pomp, S., Blomgren, J., Osterlund, M., Bevilaqua, R., Andersson, P., Ryzhov, I.V., Tutin, G.A., Yavshits, S.G., Vaishene, L.A., Onegin, M.S., Meulders, J.P., and Prieels, R., arXiv:1304.2316v1 [nucl-ex], 2013. Accessed September 15, 2021.
Funding
The present work was realized with the financial and logistical support of the Flerov Laboratory of Nuclear Reactions, Joint Institute for Nuclear Research (Dubna) and the Annual Cooperation Program between the Joint Institute for Nuclear Research (Dubna) and Romanian Research Institutes for 2020 and 2021.
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Oprea, C., Mihul, A. & Oprea, A.I. Advances in Modelling of Fast Neutrons Induced Fission of 232Th. Bull. Russ. Acad. Sci. Phys. 86, 1418–1425 (2022). https://doi.org/10.3103/S106287382211020X
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DOI: https://doi.org/10.3103/S106287382211020X